Murakami, Masahiro - Kyoto University - Department of Synthetic Chemistry and Biological Chemistry

个人简介

Education 1979 B. Sc. The University of Tokyo 1981 M. Sc.The University of Tokyo 1984 D. Sc. The University of Tokyo (Prof. Mukaiyama) Professional Career 1984-1987 Assistant, The University of Tokyo 1987-1993 Assistant, Kyoto University 1991-1992 Postdoctoral Fellow, ETH Zürich, Switzerland (Prof. Eschenmoser) 1993-2001 Associate Professor, Kyoto University 2002- Professor, Kyoto University Honors: The Chemical Society of Japan Award for Young Chemists, 1989 The Chemical Society of Japan Award for Creative Work, 2004 Nagoya Silver Medal, 2008 Synthetic Organic Chemistry Award, Japan, 2013

研究领域

Organometalic chemistry is one of the fundamental research area with great potential; Innumerable combinations of elements and bonding modes are possible, and therefore, it still has a lot of room which has been still unexplored. In addition, development of organometalic chemistry enables to synthesize new compounds, which can lead to development of vairous fields including molecular catalysts, functional materials, polymer synthesis, and pharmaceuticals. Our research project is based on organic synthesis, but our goal is "innovative discovery" which would stimulate the related sciences. 1. Synthetic Transformations Exploiting Light as the Energy Source 2. Synthetic Transformations Based on Cleavage of Unreactive Bonds 3. Multiple Functionailzation of Terminal Alkynes in One-pot

近期论文

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C-1 Oxidation/C-2 Reduction Isomerization of Unprotected Aldoses Induced by Light/Ketone Yusuke Masuda, Hiromu Tsuda, and Masahiro Murakami Angew. Chem., Int. Ed., in press; (Communication) DOI: 10.1002/anie.201914242 10.1002/anie.201914242 Carboxylation of Benzylic and Aliphatic C-H Bonds with CO2 Induced by Light/Ketone/Nickel Naoki Ishida, Yusuke Masuda, Yuuya Imamura, Katsushi Yamazaki, and Masahiro Murakami J. Am. Chem. Soc., 2019, 141, 19611-19615; (Communication) DOI: 10.1021/jacs.9b12529 One of the Most Read Articles in JACS, December 2019.10.1021/jacs.9b12529 Synthesis of Tofisopam by Way of Photoinduced CO2 Fixation Yusuke Masuda, Katsuhiko Makita, Naoki Ishida, and Masahiro Murakami Chem. Asian J., 2019, 14, 4189-4192; (Communication) DOI: 10.1002/asia.201901431 This article appears in 100th Annual Meeting of the Chemical Society of Japan 10.1002/asia.201901431 Asymmetric Synthesis and Stereochemical Assignment of 12C/13C Isotopomers Tomoya Miura, Takayuki Nakamuro, Yuuya Nagata, Daisuke Moriyama, Scott G. Stewart, and Masahiro Murakami J. Am. Chem. Soc., 2019, 141, 13341-13345; (Communication) DOI: 10.1021/jacs.9b07181 10.1021/jacs.9b07181 Photo-Assisted Fixation of CO2 onto Aryl Bromides Producing Aromatic Esters Naoki Ishida, Yusuke Masuda, Wenqing Liao, and Masahiro Murakami Chem. Lett., 2019, 48, 1316-1318; (Letter) DOI: 10.1246/cl.190563 10.1246/cl.190563 Diastereo- and Enantioselective Synthesis of (E)-δ-Boryl-Substituted anti-Homoallylic Alcohols in Two Steps from Terminal Alkynes Tomoya Miura, Naoki Oku, and Masahiro Murakami Angew. Chem., Int. Ed., 2019, 58, 14620-14624; (Communication) DOI: 10.1002/anie.201908299 10.1002/anie.201908299 A Strained Vicinal Diol as a Reductant for Coupling of Organyl Halides Naoki Ishida, Yusuke Masuda, Fangzhu Sun, Yoshiki Kamae, and Masahiro Murakami Chem. Lett., 2019, 48 1042-1045; (Letter) DOI: 10.1246/cl.190403 Selected as an Editor's Choice.10.1246/cl.190403 Generation of Boron Aza-Enolates by a Nickel-Catalyzed Reaction of Triazoles with Pinacolborane and Their Addition to Aldehydes Tomoya Miura, Sho Miyakawa, Takayuki Nakamuro, and Masahiro Murakami Chem. Lett., 2019, 48 965-967; (Letter) DOI: 10.1246/cl.190290 10.1246/cl.190290 Cyclization Reaction of 4-Acyl-1,2,3-triazoles Possessing Phenyl Rings through Generation of Electron-Deficient Carbenoids Qiang Zhao, Tomoya Miura, and Masahiro Murakami Chem. Lett., 2019, 48, 510-512; (Letter) DOI: 10.1246/cl.190074 10.1246/cl.190074 Preparation of Ni(cod)2 Using Light as the Source of Energy Naoki Ishida, Yoshiki Kamae, and Masahiro Murakami Organometallics, 2019, 38, 1413-1416; (Communication) DOI: 10.1021/acs.organomet.9b00057 One of the Most Read Articles in Organometallics, March-April 2019.10.1021/acs.organomet.9b00057 Photoinduced 1,2-Hydro(cyanomethylation) of Alkenes with a Cyanomethylphosphonium Ylide Tomoya Miura, Daisuke Moriyama, Yuuta Funakoshi, and Masahiro Murakami Synlett, 2019, 30, 511-514; (Letter) DOI: 10.1055/s-0037-1612230 Published as part of 30 Years SYNLETT – Pearl Anniversary Issue 10.1055/s-0037-1612230 Light/Palladium-Promoted Benzylic C–H Acylation Using a Benzoyl Group as the Photo-Directing Group Yusuke Masuda, Naoki Ishida, and Masahiro Murakami Chem. Asian J., 2019, 14, 403-406; (Communication) DOI: 10.1002/asia.201801881 10.1002/asia.201801881 Synthesis of γ-Boryl-Substituted Homoallylic Alcohols with Anti Stereochemistry Based on a Double-Bond Transposition Protocol Tomoya Miura, Junki Nakahashi, Takanori Sasatsu, and Masahiro Murakami Angew. Chem., Int. Ed., 2019, 58, 1138-1142; (Communication) DOI: 10.1002/anie.201811205 10.1002/anie.201811205 Synthesis of 2-Aryloxy-1,3-Dienes from Phenols and Propargyl Carbonates Naoki Ishida, Yusaku Hori, Shintaro Okumura, and Masahiro Murakami J. Am. Chem. Soc., 2019, 141, 84-88; (Communication) DOI: 10.1021/jacs.8b11159 One of the Most Read Articles in JACS, December 2018.10.1021/jacs.8b11159 Light/Copper Relay for Aerobic Fragmentation of Lignin Model Compounds Wang Zhou, Junki Nakahashi, Tomoya Miura, and Masahiro Murakami Asian J. Org. Chem., 2018, 7, 2431-2434; (Communication) DOI: 10.1002/ajoc.201800520 10.1002/ajoc.201800520 Synthesis of Fused and Linked Benzofurans from 2-Alkynylphenol Derivatives through Rhodium(I)-catalyzed Domino-type Addition Reactions Takanori Matsuda, Shinya Abe, Hirotaka Ito, Tomoya Tsuboi, Haruki Kirikae, and Masahiro Murakami Chimia, 2018, 72, 888-891;10.1002/ajoc.201800520 Synthesis of Elongated Esters from Alkenes Tomoya Miura, Yuuta Funakoshi, Junki Nakahashi, Daisuke Moriyama, and Masahiro Murakami Angew. Chem., Int. Ed., 2018, 57, 15455-15459; (Communication) DOI: 10.1002/anie.201809115 10.1002/anie.201809115 2-Arylsilacyclobutane as a Latent Carbanion Reacting with CO2 Naoki Ishida, Shintaro Okumura, Tairin Kawasaki, and Masahiro Murakami Angew. Chem., Int. Ed., 2018, 57, 11399-11403; (Communication) DOI: 10.1002/anie.201805333 10.1002/anie.201805333 Enantioselective Denitrogenative Annulation of 1H-Tetrazoles with Styrenes Catalyzed by Rhodium Takayuki Nakamuro, Kohei Hagiwara, Tomoya Miura, and Masahiro Murakami Angew. Chem., Int. Ed., 2018, 57, 5497-5500; (Communication) DOI: 10.1002/anie.201801283 10.1002/anie.201801283 Photo-Catalyzed Ortho-Alkylation of Pyridine N-Oxides through Alkene Cleavage Wang Zhou, Tomoya Miura, and Masahiro Murakami Angew. Chem., Int. Ed., 2018, 57, 5139-5142; (Communication) DOI: 10.1002/anie.201801305