Structural extracellular polymeric substances (SEPS) as valuable biopolymers, can be extracted from waste activated sludge (WAS). However, the extraction yield is typically low, and detailed information on SEPS characterizations, as well as proper treatment of the sludge after SEPS extraction, remains limited. This study aimed to optimize the conditions of heating-NaCO extraction process to increase

The occurrence and risk of N-(1,3-dimethylbutyl)-N′-phenyl--phenylenediamine-quinone (6PPD-Q), derived from the oxidation of the tire antidegradant 6PPD, has raised significant concern since it was found to cause acute mortality in coho salmon when exposed to urban runoff. Given the short half-life period and low solubility of 6PPD-Q, reliable in situ measurement techniques are required to accurately

In mining regions, flotation reagents can interact with heavy metals, thereby increasing the complexity of their migration. However, most current studies solely focus on the migration of heavy metals, neglecting the influence of flotation reagents in their models concerning mining area pollution. This study developed the reactive transport model, Multisurface Speciation Model (MSM), which integrated

Frequent occurrence of trace antibiotics in reclaimed water is concerning, which inevitably causes aquifer contamination in the case of managed aquifer recharge (MAR). Global governments have formulated strict reclaimed water standards to ensure the safety of water reuse. Recent studies have found that improved antibiotics removal is intimately associated with high ammonia-oxidizing activity. However

Selective lithium (Li) recovery from unconventional water sources (UWS) (e.g., shale gas waters, geothermal brines, and rejected seawater desalination brines) using inorganic lithium-ion sieve (LIS) materials can address Li supply shortages and distribution issues. However, the development of high-performance LIS materials and the optimization of recovery-related operating parameters are hampered by

The iron redox cycle can enhance anammox in treating low-strength ammonia wastewater. However, maintaining an effective iron redox cycle and suppressing nitrite-oxidizing bacteria in a one-stage partial nitritation and anammox (PN/A) process poses challenges during long-term aeration. We proposed a novel and simple strategy to achieve an efficient iron redox cycle in an iron-mediated anoxic-microaerobic

Chemical moderate preoxidation for algae-laden water is an economical and prospective strategy for controlling algae and exogenous pollutants, whereas it is constrained by a lack of effective on-line evaluation and quick-response feedback method. Herein, excitation-emission matrix parallel factor analysis (EEM-PARAFAC) was used to identify cyanobacteria fluorophores after preoxidation of sodium hypochlorite

The presence of antibiotics in wastewater poses significant threat to our ecosystems and health. Traditional biological wastewater treatment technologies have several limitations in treating antibiotic-contaminated wastewaters, such as low removal efficiency and poor process resilience. Here, a novel electrochemical-coupled sulfur-mediated biological system was developed for treating wastewater co-contaminated

A new aeration device based on Bernoulli's principle, Jetventrumixer (JVM), was introduced into an aeration tank in denitrification process, which involved an automatic split injection system (ASIS) into two denitrification tanks every 10 minutes. Real-time monitoring of influent water allowed the calculation of the C/N ratio, enhancing the utilization efficiency of internal carbon sources while reducing

Dewatering is an indispensable link in sludge treatment, but its effect on the microplastics (MPs) remains inadequately understood. This study investigated the physicochemical changes and leaching behavior of MPs during the mechanical dewatering of sludge, as well as the impact of MP leachates on activated sludge (AS). After sludge dewatering, MPs exhibit rougher surfaces, decreased sizes and altered

Microbial amino acid composition (AA) reflects adaptive strategies of cellular and molecular regulations such as a high proportion of acidic AAs, including glutamic and aspartic acids in alkaliphiles. It remains understudied how microbial AA content is linked to their pH adaptation especially in natural environments. Here we examined prokaryotic communities and their AA composition of genes with metagenomics

The solid pore characteristics are commonly considered as the important influential factors on waste-activated sludge (WAS) dewaterability, and should be related to the cohesive force of bio-flocs dominated by cation-organic interactions at solid-water interface. This study aimed to establish an approach for regulating the solid pore structure of WAS by cationic regulation. The influential mechanism

Nitrogen compounds in current seawater treatment processes typically are converted to nitrate, threatening seawater quality and marine ecology. Electrochemical denitrification is a promising technique, but its efficiency is severely limited by the presence of excess chloride ions. In this work, a flow-through cell went through an on-demand chlorine-mediated electrochemical-chemical tandem reaction

Due to the high moisture, strong hydrophilicity, and hard compressibility of sewage sludge (SS), it is difficult to realize the high-efficiency drying. Herein, a novel SS drying technology was developed to quickly and deeply reduce the moisture of SS from 75.6% to 38.5% in 1 h. During the process, secondary aluminum ash (SAA), a solid waste, was added to SS and acted as skeletons to form plenty of

Benzothiazoles (BTHs), benzotriazoles (BTRs), and benzotriazole ultraviolet absorbers (BUVs) have garnered significant attention owing to their persistent nature in the environment and adverse impacts on aquatic organisms. However, there remains a dearth of investigations and studies conducted in tropical marine environments. In this study, we undertook the inaugural distributional survey and ecotoxicological

Ambient operation and large-scale demonstration have limited the implementation and evaluation of anaerobic membrane bioreactors (AnMBRs) for low-strength wastewater treatment. Here, we studied these issues at an AnMBR demo plant that treats domestic wastewater and food waste together at ambient temperatures (7–28 °C). At varied hydraulic retention times (HRTs, 8–42 h), the AnMBR achieved a COD removal

Microbial chain elongation integrating innovative bioconversion technologies with organic waste utilization can transition current energy-intensive n-caproic acid production to sustainable circular bioeconomy systems. However, ammonia-rich waste streams, despite their suitability, pose inhibitory challenges to these bioconversion processes. Herein, biochar was employed as an additive to enhance the

Highly hydrophilic extracellular polymeric substance (EPS) with gel-like structure seriously plagues the development of sludge deep dewatering. Oxysulfur radicals-based oxidation driven by iron-bearing mineral proposes a promising strategy for effective EPS decomposition. However, the transformation and involved interaction mechanisms of aromatic proteins are still controversial due to the complex

Given the significance of HCO for autotrophic anammox bacteria (AnAOB), excessive HCO was always provided in anammox-related systems and engineering applications. However, its impact mechanism on anammox process at genome-level remains unknown. This study firstly established an anammox-centered coupling system that entails heterotrophic partial denitrification (PD) and hydrolytic acidification (A-PDHA)

Liquid-liquid extraction (LLE) combined with the N blow-down method is a promising tool for bioanalysis of drinking water. However, detailed information on which disinfection byproduct (DBP) classes are retained in LLE extracts is currently unavailable. In this study, the recovery of seven classes of volatile DBPs and total adsorbable organic halogens (TOX) during the LLE method, combined with three

Faecal contamination of freshwater and marine environments represents a significant risk for public health, recreational activity and food safety, and tools for evaluating complex multi-source contamination remain largely in the development phase. We evaluated the efficacy of the Fast Expectation Maximization (FEAST) microbial source tracking (MST) algorithm to apportion sources of faecal contamination

While forward osmosis (FO) and reverse osmosis (RO) processes have been proven effective in rejecting organic pollutants, the rejection rate is highly dependent on compound and membrane characteristics, as well as operating conditions. This study aims to establish machine learning (ML) models for predicting the rejection of organic pollutants by FO and RO and providing insights into the underlying

This paper examines the acid leaching efficiencies of Fe and P from vivianite slurry (VS, Fe(PO)·8HO), which is magnetically separated from anaerobic digested sludge, and elaborates on Fe and P reuse routes. The characteristics and dissolution behavior of raw VS in hydrochloric, sulfuric, phosphoric, oxalic, and citric acids are investigated. Results reveal that the primary impurities in VS are organic

Freeze-thaw (FT) events profoundly perturb the biochemical processes of soil and water in mid- and high-latitude regions, especially the riparian zones that are often recognized as the hotspots of soil-water interactions and thus one of the most sensitive ecosystems to future climate change. However, it remains largely unknown how the heterogeneously composed and progressively discharged meltwater

The consistent presence of -chloronitrobenzene (-CNB) in groundwater has raised concerns regarding its potential harm. In this study, we developed a biocathode-anode cascade system in a permeable reactive barrier (BACP), integrating biological electrochemical system (BES) with permeable reactive barrier (PRB), to address the degradation of -CNB in the groundwater. BACP efficiently accelerated the formation

In this study, the transformation mechanisms of extracellular polymeric substances (EPS) during ultraviolet/peracetic acid (UV/PAA) disinfection were elucidated based on multiple molecular-level analyses. After UV/PAA disinfection, the contents of soluble EPS (S-EPS), loosely bound EPS (LB-EPS) and tightly bound EPS (TB-EPS) were reduced by 70.47 %, 57.05 % and 47.46 %, respectively. Fluorescence excitation-emission

Optimizing nitrogen removal is crucial for ensuring the efficient operation of wastewater treatment plants (WWTPs), but it is susceptible to variations in influent conditions and operational parameter constraints, and conflicts with the energy-saving and carbon emission reduction goals. To address these issues, this study proposes a hybrid framework integrating process simulation, machine learning

This study investigated a sustainable approach through dielectric barrier discharge (DBD) enhanced Fenton technology coupling nanofiltration (NF) process for landfill leachate treatment. The DBD/Fe(II)/HO system exhibited significant synergistic effects, removing 55.07 % of TOC and 53.79 % of UV within 60 min, respectively. Additionally, the DBD/Fe(II)/HO system demonstrated exceptional performance

The advanced oxidation process is an efficient technology for the degradation and detoxification of refractory organics to ensure water safety. However, most researches focus on improving pollutant degradation but overlook carbon emission and resource utilization. In this study, a flow-through electrochemical integrated system was constructed to simultaneously realize bisphenol A (BPA) oxidation into

Despite widespread deployment and investigation of ultrafiltration (UF) for secondary effluent purification, the challenge of membrane fouling due to effluent organic matter (EfOM) remains formidable. This study introduced a novel pretreatment method utilizing Co nanoparticles-encapsulated carbon nanotubes activated peroxymonosulfate (Co@CNT/PMS) to degrade EfOM and mitigate membrane fouling. Characterization

In a membrane bioreactor (MBR) system, sludge reduction techniques induce membrane fouling. To address this challenge, we incorporated a rotating mesh carrier, which can adsorb organic matter and provide a habitat for metazoans, into the anoxic tank of a conventional anoxic/oxic-MBR (A/O-MBR) system, termed rotating biological contactor-MBR (RBC-MBR), and evaluated treatment performance. Over 151 days

Research on the microbial community and function of the anammox process for environmentally friendly wastewater treatment has achieved certain success, which may mean more universal insights are needed. However, the comprehensive understanding of the anammox process is constrained by the limited taxonomic assignment and functional characterization of anammox microbiota, primarily due to the scarcity

Rivers play a pivotal role in global carbon (C) and nitrogen (N) biogeochemical cycles. Urbanized rivers are significant hotspots of greenhouse gases (GHGs, NO, CO and CH) emissions. This study examined the GHGs distributions in the Guanxun River, an effluents-receiving subtropical urbanized river, as well as the key environmental factors and processes affecting the pattern and emission characteristics

Lakes play a crucial role in the nitrogen (N) cycle, and eutrophication disrupts the balance of the nitrogen cycle within lakes, including both the N removal process and the N supplement process. However, the mechanisms by which different nutrient levels affect seasonal nitrogen variations in the water columns are not clear, especially for long-term and large- scale studies. In this study, we used

Antimicrobial resistance (AMR) is a global challenge that has impacted aquaculture and surrounding marine environments. In this study, a year-long monitoring program was implemented to evaluate AMR in two different aquaculture settings (i.e., open cage farming, recirculating aquaculture system (RAS)) and surrounding marine environment within a tropical coastal region. The objectives of this study are

Many researchers have addressed the challenge of optimal pressure sensor placement for different purposes, such as leakage detection, model calibration, state estimation, etc. However, pressure data often need to serve multiple purposes, and a method to optimize sensor locations with versatility for various objectives is still lacking. In this paper, a graph-based optimal sensor placement (GOSP) framework

In recent decades, global aquaculture has expanded rapidly, raising concerns about coastal environmental degradation due to unregulated or poorly regulated discharge of aquaculture tailwater. Despite the crucial role of dissolved organic matter (DOM) in biogeochemical processes and aquatic biodiversity, the influence of aquaculture type on the molecular characteristics of DOM remains largely unexplored

Urban water systems in China are facing multiple challenges, including rapid urbanisation, climate change and infrastructure ageing. It is crucial to evaluate their environmental performance from a holistic perspective in planning and management processes. To the best of our knowledge, there is a lack of nationwide life cycle assessment (LCA) studies on China's urban water systems that cover all system

Nanofiltration (NF) is being increasingly applied to produce high-quality drinking water; however, its cost-effective operation remains challenging due to the perennial membrane fouling. On account of the low tolerance of common NF membranes to chemical oxidants, this study proposed high-dose UV irradiation as a pretreatment strategy for organic fouling mitigation. Results showed that the permeate

Water quality degradation by decommissioned mining sites is an environmental issue recognized globally. In the Ore mountains of Central Europe, a wide array of contaminants is released by abandoned under- and aboveground mining sites threatening the quantity and quality of surface and groundwater resources. Here, we focus on the less-explored internal pollution processes within these mines involving

Phytoremediation is an effective solution to treat pollution with antibiotic compounds in aquatic environments; however, the underlying mechanisms for plants to cope with antibiotic pollutants are obscure. Here we used cell suspension culture to investigate the distribution and transformation of ciprofloxacin (CIP) in common reed () plants, as well as the accompanying phenotypic and metabolic responses

Drinking water distribution systems are increasingly vulnerable to sewage intrusion due to aging water infrastructure and intensifying water stress. While the health risks associated with sewage intrusion have been extensively studied, little is known about the impacts of intruded bacteria and dissolved organic matter (DOM) on microbiology in drinking water. In this dynamic study, we demonstrate that

As the size of water distribution network (WDN) models continues to grow, developing and applying real-time models or digital twins to simulate hydraulic behaviors in large-scale WDNs is becoming increasingly challenging. The long response time incurred when performing multiple hydraulic simulations in large-scale WDNs can no longer meet the current requirements for the efficient and real-time application

Antimicrobial resistance (AMR) is one of the greatest threats to human health with a growing body of evidence demonstrating that selection for AMR can occur at environmental antimicrobial concentrations. Understanding the concentrations at which selection for resistance may occur is critical to help inform environmental risk assessments and highlight where mitigation strategies are required. A variety

The microalgal-bacterial granular sludge (MBGS) process, enhanced with sodium bicarbonate (NaHCO), offers a sustainable alternative for wastewater treatment aiming for carbon neutrality. This study demonstrates that NaHCO, which can be derived from the flue gases and alkaline textile wastewater, significantly enhances pollutant removal and biomass production. Optimal addition of NaHCO was found to

Extensive studies on improving anammox performance have taken place for decades with particular focuses on its operational and environmental factors, but such parameter-based optimization is difficult, because of the sheer number of possible combinations and multidimensional arrays of these factors. Utilizing machine-learning algorithm and published anammox data, Bayesian nonparametric general regression

Microplastics have attracted considerable attention as emerging contaminants that threaten water bodies. The removal of microplastics from a mini-hydrocyclone, enhanced by air flotation, was studied numerically. The three-phase flow was modeled using the Eulerian-Eulerian model coupled with interphase interactions. The characteristics of the flow field and distribution of microplastics and microbubbles

Disinfection is critical for ensuring water safety; however, the potential risks posed by disinfection byproducts (DBPs) have raised public concern. Previous studies have largely focused on low-molecular-weight DBPs with one or two carbon atoms, leaving the formation of high-molecular-weight DBPs (HMW DBPs, with more than two carbon atoms) less understood. This study explores the formation of HMW DBPs

Substantial volumes of hazardous shale gas produced water (SGPW) generated in unconventional natural gas exploration. Membrane distillation (MD) is a promising approach for SGPW desalination, while membrane fouling, wetting, and permeate deterioration restrict MD application. The integration of gravity-driven membrane (GDM) with MD process was proposed to improve MD performance, and different pretreatment

Freshwater ecosystems, such as urban lake sediments, have been identified as important sources of greenhouse gases (GHGs) to the atmosphere, as well as persistent sinks for ubiquitous microplastics due to the high population density and frequent anthropogenic activity. The potential impacts of microplastics on GHG production, however, remain underexplored. In this study, four types of common biodegradable

To reduce the harm of water contamination incidents in drinking water source areas (DWSAs) and explore feasible approaches, the research developed a hydrodynamic water quality model for DWSAs based on two dimensional water quality and quantity equations, Geographic Information System (GIS), and Digital Elevation Model (DEM). The Heshangshan Drinking Water Source Area (HDWSA) in the Three Gorges Reservoir

Urban stormwater management systems, particularly storm sewers, are critical for managing runoff in urban areas. These systems are designed to function during wet weather events; however, field-based observations of these systems suggest that they may also be active flow pathways in dry weather conditions, ultimately contributing to streamflow. Unlike dry weather flow in wastewater systems, storm sewer

CrAssphage has been recognized as the most abundant and human-specific bacteriophage in the human gut. Consequently, crAssphage has been used as a microbial source tracking (MST) marker to monitor human fecal contamination. Many crAss-like phages (CLPs) have been recently discovered, expanding the classification into the new order Crassvirales. This study aims to assess CLP prevalence in South Korea

Ultrafiltration technology (UF) is efficient in surface water treatment, but its development and widespread application are limited by membrane fouling. Herein, an efficient and stable polymerized ferric titanium coagulant (PFTC) was synthesized and used as a UF pretreatment agent in actual lake water treatment. The control mechanism of PFTC on membrane fouling was investigated from the perspective

The enhancement of electron or proton transfer between syntrophic microbes has been widely recognised as a means for improving methane generation. However, the uncoupled supplementation of electrons and protons in multiphase anaerobic environment hinders the balanced uptake of electrons and protons in the cytoplasm of methanogens, limiting methanogenesis efficiency. Herein, the cooperative effect of

Ultraviolet light-emitting diodes (UV-LEDs) have demonstrated the ability to inactivate microorganisms in water, offering an environmentally safer alternative to the conventional mercury lamp, in UV applications. While several studies have explored the microbiological effect of UVC-LEDs (200nm-280nm), limited information exists regarding their effects on waters with critical qualities. These critical

Accurately predicting the concentration of organochlorine pesticides (OCPs) presents a challenge due to their complex sources and environmental behaviors. In this study, we introduced a novel and advanced model that combined the power of three distinct techniques: Complete Ensemble Empirical Mode Decomposition with Adaptive Noise (CEEMDAN), Variational Mode Decomposition (VMD), and a deep learning

The efficient capture of uranium from wastewater is crucial for environmental remediation and the sustainable development of nuclear energy, yet it poses considerable challenges. In this study, amphiphilic ionic covalent organic framework intercalated into graphene oxide (GO) nanosheets functionalized with polyethyleneimine (PEI) were used to construct hybrid membranes with ultrafast uranium adsorption

Dual electron donor bioretention systems have emerged as a popular strategy to enhance dissolved nitrogen removal from stormwater runoff. Pyrite-woodchip mixotrophic bioretention systems showed a promoted and stabilized removal of dissolved nutrients under complex rainfall conditions, but the sulfate reduction process that can induce iron sulfide generation and reuse was overlooked. In this study,

Submerged macrophytes remediation is a commonly used technique for improving water quality and restoring habitat in aquatic ecosystems. However, the drivers of success in the submerged macrophytes assembly process and their specific impacts on methane emissions are poorly understood. Thus, we conducted a mesocosm experiment to test the growth plasticity and carbon fixation of widespread submerged macrophytes