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Rational Design of Flexible Two-Dimensional MXenes with Multiple Functionalities
Chemical Reviews ( IF 54.301 ) Pub Date : 2019-11-11 , DOI: 10.1021/acs.chemrev.9b00348
Zhongheng Fu, Ning Wang, Dominik Legut, Chen Si, Qianfan Zhang, Shiyu Du, Timothy C. Germann, Joseph S. Francisco, Ruifeng Zhang

In the past decade, two-dimensional (2D) transition metal carbides, nitrides, and carbonitrides (MXenes) have attracted attention and interest from the scientific community due to their superior mechanical strength and flexibility, physical/chemical properties, and multiple exciting functionalities. Among these materials, the ingenious and effective combination of the mechanical and functional properties of MXenes provides a promising opportunity for designing flexible and wearable devices. This review summarizes the recent research progress in the structural stabilities, mechanical strength and deformation mechanism, strain-tunable energy storages, and catalytic and thermoelectric properties along with certain strain modifications and strain-controllable electronic/topological properties of MXenes from a combined theoretical and experimental perspective and illustrates their electronic origins. Taking the design principles as a focus, the theoretical predictions provide guidance, while the experimental work gives a thorough validation, thus setting the foundation for the current scientific achievements, challenges, and prospects in the field of MXenes.
更新日期:2019-11-13

 

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