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成果及论文

    代表性论文 (#共同一作; *通讯作者)

1. Bu, F.; Deng, Y.; Xu, J.; Yang, D.; Li, Y.; Li, W.* and Lei, A.*, Electrocatalytic reductive deuteration of arenes and heteroarenes. Nature 2024. doi.org/10.1038/s41586-024-07989-7.

2. LiW.; Rabeah, J.; Bourriquen, F.; Yang, D.; Kreyenschulte, C.; Rockstroh, N.; Lund, H.; Bartling, S.; Surkus, A-E.; Junge, K.; Brückner, A.*; Lei, A.*; and Beller, M.*, Scalable and selective deuteration of (hetero)arenes, Nature Chem., 2022, 14, 334–341 (Highlighted in “Synfacts”).

3.  Li, Y.#; Peng, Y.#; Dong, W.#; Jiang, X.; Lu, L.; Yang, D.; Hsu, L-C.; LiW.*; Su, B-L.* and Lei, A.*, Multiscale Anion-Hybrid in Atomic Ni Sites for High-Rate Water Electrolysis: Insights into the Charge Accumulation Mechanism, J. Am. Chem. Soc. 2024146, 14194–14202.

4. Li, H.#; Li, Y.#; Chen, J; Lu, L.; Wang, P.; Hu, J.; Ma, R.; Gao, Y.; Yi, H.*; LiW.* and Lei, A.*, Scalable and Selective Electrochemical Hydrogenation of Polycyclic Arenes, Angew. Chem. Int. Ed. 2024, doi.org/10.1002/anie.202407392.

5. Qiu, F.+; Chen, Y.+; Liao, P.; Gao, Y.; Guo, M.*; Zhang, H.*; Lei, A.* and LiW.*, Electrochemical selective deuterium labelling of N-heteroarenes, Green Synth. Catal. 2024, doi. org/10.1016/j.gresc.2024.06.003.

6. Li, H.; Shabbir, M.; Li, W.* and Lei, A.*, Recent Advances in Deuteration Reactions, Chin. J. Chem. 2024, 42, 11451156.

7. Cui, X.#; Li, W.#; (co-first author), Junge, K.; Fei, Z.; Beller, M.* and Dyson, P. J.*, Selective Acceptorless Dehydrogenation of Primary Amines to Imines by Core–Shell Cobalt Nanoparticles, Angew. Chem. Int. Ed. 2020, 59, 7501–7507.

8. Li, W.; Liu, W.; Leonard, D. K.; Rabeah, J.; Junge, K.; Brückner A. and Beller, M.*, Practical Catalytic Cleavage of C(sp3)−C(sp3) Bonds in Amines, Angew. Chem. Int. Ed., 2019, 58, 10693–10697. (Hot Paper)

9. Li, W.; Duan, Z.; Zhang, X.; Zhang, H.; Wang, M.; Jiang, R.; Zeng, H.; Liu, C. and Lei, A.*, From Anilines to Isatins: Palladium-Catalyzed Oxidative C−H Double Carbonylation, Angew. Chem. Int. Ed., 2015, 54, 18931896.

10. Li, W.; Liu, C.; Zhang, H.; Ye, K.-Y.; Zhang, G.; Zhang, W.; Duan, Z.; You, S.-L.*; and Lei, A.*, Palladium-Catalyzed Oxidative Carbonylation of N-Allylamines for the Synthesis of beta-Lactams, Angew. Chem. Int. Ed., 2014, 53, 2443–2446. (Highlighted in “Synfacts” and “Organic Chemistry”)

11. Li, W.; Cui, X.; Junge, K.; Surkus, A.-E.; Kreyenschulte, C.; Bartling, S.; Beller, M.*, General and Chemoselective Copper Oxide Catalysts for Hydrogenation Reactions, ACS Catal., 2019, 9, 4302–4307. 

12. Li, W.; Qu, R.; Liu, W.; Bourriquen, F.; Bartling, S.; Rockstroh, N.; Junge, K.*; and Beller, M.*, Copper-catalysed low-temperature water-gas shift reaction for selective deuteration of aryl halides, Chem. Sci., 2021, doi.org/10.1039/D1SC04259A.

13. Li, W.#; Artz, J.#; (co-first author), Broicher, C.; Junge, K.; Palkovits, R.* and Beller, M.*, Superior Activity and Chemoselectivity of Heterogenized Cobalt Catalysts for Nitroarene Reduction under Mild Conditions, Catal. Sci. & Technol., 2019, 9, 157–162.

14. Li, W.; Werner, T.*, B(C6F5)3-Catalyzed Michael Reactions: Aromatic C–H as Nucleophiles, Org. Lett., 2017, 19, 2568–2571. (Selected to be featured in ACS Editors' Choice)

15. Li, W.; Wang, M.-M. Hu, Y.; Werner, T.*, B(C6F5)3-Catalyzed Regioselective Deuteration of Electron-Rich Aromatic and Heteroaromatic Compounds, Org. Lett., 2017, 19, 5768–5771.

16. Li, W.; Duan, Z.; Jiang, R.; and Lei, A.*, Palladium/Copper-Catalyzed Aerobic Oxidative C–H Carbonylation for the Synthesis of o-Aminobenzoates, Org. Lett., 2015, 17, 1397-1400.

17. Li, W.; Xu, Z.; Sun, P.*; Jiang, X. and Fang, M.; Synthesis of Biphenyl-2-carbonitrile Derivatives via a Palladium-Catalyzed sp2 C-H Bond Activation Using Cyano as Directing Group, Org. Lett., 2011, 13, 1286–1289.

18. Li, W.; Sun, P.*, Pd(OAc)2-Catalyzed Alkoxylation of Arylnitriles via sp2 C-H Bond Activation Using Cyano as the Directing,  J. Org. Chem., 2012, 77, 8362–8366.

19. Li, W.; Yin, Z.; Jiang, X. and Sun, P.*, Palladium-Catalyzed Direct ortho C-H Arylation of 2-Arylpyridine Derivatives with Aryltrimethoxysilane, J. Org. Chem., 2011, 76, 8543–8548.

20. Duan, Z.; Li, W.* and Lei, A.*, Nickel-Catalyzed Reductive Cross-Coupling of Aryl Bromides with alkyl Bromides: Et3N as the Terminal Reductant, Org. Lett., 2016, 18, 40124015.

21. Liu, W.; Li, W.; Spannenberg, A.; Junge, K.; Beller, M.*, Iron-catalysed regioselective hydrogenation of terminal epoxides to alcohols under mild conditions, Nat. Catal., 2019, 2, 523–528. 

22. Chen, F.; Li, W.; Sahoo, B.; Kreyenschulte, C.; Agostini, G.; Lund, H.; Junge, K.; Beller, M.*, Hydrogenation of Pyridines Using a NitrogenModified Titania-Supported Cobalt Catalyst, Angew. Chem. Int. Ed., 2018, 57, 1448814492.

23. Liu, W.#; Leischner, T.#; (co-first author), Li, W.; Junge, K.; Beller, M.*, A General Regioselective Synthesis of Alcohols by Cobalt-Catalyzed Hydrogenation of Epoxides, Angew. Chem. Int. Ed., 2020, 59, 11321–11324

24. Leonard, D. K.; Li, W.; Junge K.; Beller, M.*, Improved Bimetallic Cobalt–Manganese Catalysts for Selective Oxidative Cleavage of Morpholine Derivatives, ACS Catal, 2019, 9, 1112511129.

25. Leonard, D. K.; Li, W.; Rockstroh, N.; Junge, K.; Beller, M.*, Aerobic iron-catalyzed site-selective C(sp3)–C(sp3) bond cleavage in N-heterocycles,. Catal. Commun., 2021, 157, 10633322.

26. Cui, X.; Li, W.; Ryabchuk, P.; Junge, K.; Beller, M.*, Bridging Homogeneous and Heterogeneous Catalysis by Heterogeneous Single-metal-site Catalysts, Nat. Catal., 2018, 1, 385–397.

27. Liu, C.; Yuan, J.; Gao, M.; Tang, S.; Li, W.; Shi R.; Lei, A.*, Oxidative Coupling between Two Hydrocarbons: An Update of Recent C–H Functionalizations, Chem. Rev., 2015, 115, 1213812204.

28. Hao, W.; Tian, J.; Li, W.; Shi, R.; Huang, Z.; Lei, A.*, Nickel-Catalyzed Oxidative C−H/N−H Isocyanide Insertion: An Efficient Synthesis of Iminoisoindolinone Derivatives, Chem. Asian J., 2016, 11, 16641667.