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High-field dielectric properties and high-power performance of Fe-modified PZN–PMS–PZT piezoelectric ceramics

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Abstract

In this work, the 0.04Pb(Zn1/3Nb2/3)O3-0.05Pb(Mn1/3Sb2/3)O3–xPbZrO3–(0.91−x)PbTiO3 + ymol%Fe2O3 (xPZ-PZNMST + y%Fe; x = 0.440–0.460, y = 0.00–0.15) piezoelectric ceramics were synthesized by solid-state reaction method. The 0.45PZ-PZNMST + 0.10%Fe ceramic with morphotropic phase boundary shows optimum comprehensive electromechanical properties with d33 = 401 pC/N, kp=0.6, tan δ = 0.39%, Qm=921, and Tc = 314 °C. In addition, a low high-field tan δ of 0.78% at 200 V/mm is achieved in the 0.45PZ-PZNMST + 0.10%Fe ceramic. Therefore, a high vibration velocity of 0.80 m/s is obtained in 0.45PZ-PZNMST + 0.10%Fe ceramic. The maximum mechanical energy density of 0.45PZ-PZNMST + 0.10%Fe ceramic reaches 2500 J/m3, which is about four times that of commercial PZT4 ceramics (620 J/m3). The 0.45PZ-PZNMST + 0.10%Fe ceramic with good high-power performance shows a potential application in high-power ultrasonic transducers.

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Funding

The work was supported by the National Natural Science Foundation of China (Grant No. 92263105, U2037603 and 62374090) and the Fundamental Research Funds for the Central Universities (Grant No. 30921013108).

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Authors and Affiliations

  1. Hangzhou Applied Acoustics Research Institute, Hangzhou, 310023, China

    Guanglei Xiang, Yuequn Wang & Xuezhou Gai

  2. School of Material Science and Engineering, Nanjing University of Science and Technology, Nanjing, 210094, China

    Wenbin Tang & Guoliang Yuan

  3. State Key Laboratory of Mechanics and Control of Mechanical Structures, Nanjing University of Aeronautics and Astronautics, Nanjing, 210016, China

    Yiping Wang

Authors
  1. Guanglei Xiang
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  2. Yuequn Wang
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  4. Wenbin Tang
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  6. Guoliang Yuan
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Contributions

GX: conceptualization, investigation, data curation, formal analysis, writing—original draft, YW: investigation, data curation, formal analysis, XG: investigation, formal analysis, conceptualization, WT: conceptualization, supervision, writing—review & editing, YW: investigation, formal analysis, conceptualization, GY: conceptualization, supervision, writing—review & editing.

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Correspondence to Wenbin Tang.

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Xiang, G., Wang, Y., Gai, X. et al. High-field dielectric properties and high-power performance of Fe-modified PZN–PMS–PZT piezoelectric ceramics. J Mater Sci: Mater Electron 35, 809 (2024). https://doi.org/10.1007/s10854-024-12603-7

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