Optical investigation of the heavy-fermion normal state in superconducting UTe2

Sirak M. Mekonen, Chang-Jong Kang, Dipanjan Chaudhuri, David Barbalas, Sheng Ran, Gabriel Kotliar, Nicholas P. Butch, and N. P. Armitage
Phys. Rev. B 106, 085125 – Published 16 August 2022

Abstract

The recently discovered superconductor, UTe2, has attracted immense scientific interest due to observations that suggest odd-parity superconductivity. It is believed that the material is a heavy-fermion metal at low temperatures although details of the normal state are unclear. Using Fourier transform infrared spectroscopy, we investigated the normal state electronic structure of UTe2 at zero applied magnetic field. Combining the measured reflectivity with the dc resistivity, the complex optical conductivity was obtained over a large frequency range. The frequency dependence of the real part of the optical conductivity exhibits a MIR peak around 4000 cm1 and a narrow Drude peak that develops below 40 K. A combination of density functional and dynamic mean-field theory gives spectra in close correspondence to the experiment. Via this comparison we attribute the prominent MIR peak to interband transitions involving a narrow U 5f feature that develops near the Fermi level. In this regard, this comparison along with data that shows the scale of the low-temperature mass renormalization gives spectroscopic evidence for the existence of a low-energy Kondo resonance at temperatures just above the onset of superconductivity and implicates heavy electrons in the formation of the superconducting state. We find that the coherent Kondo resonance is primarily associated with a collapse of scattering and less with a transfer of spectral weight.

  • Figure
  • Figure
  • Figure
  • Figure
  • Figure
  • Figure
  • Received 7 May 2021
  • Revised 31 May 2022
  • Accepted 18 July 2022

DOI:https://doi.org/10.1103/PhysRevB.106.085125

©2022 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

Sirak M. Mekonen1, Chang-Jong Kang2,3, Dipanjan Chaudhuri1, David Barbalas1, Sheng Ran4,5,6, Gabriel Kotliar2,7, Nicholas P. Butch4,8,6, and N. P. Armitage1

  • 1The Institute for Quantum Matter, Department of Physics and Astronomy, The Johns Hopkins University, Baltimore, Maryland 21218, USA
  • 2Department of Physics and Astronomy, Rutgers University, Piscataway, New Jersey 08856, USA
  • 3Department of Physics, Chungnam National University, Daejeon 34134, South Korea
  • 4Center for Nanophysics and Advanced Materials, Department of Physics, University of Maryland, College Park, Maryland 20742, USA
  • 5NIST Center for Neutro Research, National Institute of Standards and Technology, Gaithersburg, Maryland 20742, USA
  • 6Department of Materials Science and Engineering, University of Maryland, College Park, Maryland 20742, USA
  • 7Department of Condensed Matter Physics and Materials Science, Brookhaven National Laboratory, Upton, New York 11973, USA
  • 8NIST Center for Neutro Research, National Institute of Standards and Technology, Gaithersburg, Maryland 20899, USA

Article Text (Subscription Required)

Click to Expand

References (Subscription Required)

Click to Expand
Issue

Vol. 106, Iss. 8 — 15 August 2022

Reuse & Permissions
Access Options
CHORUS

Article Available via CHORUS

Download Accepted Manuscript
Author publication services for translation and copyediting assistance advertisement

Authorization Required


×
×

Images

×

Sign up to receive regular email alerts from Physical Review B

Log In

Cancel
×

Search


Article Lookup

Paste a citation or DOI

Enter a citation
×