Abstract
The direct aqueous mineral carbonation of carbide slag was investigated. The flow characteristics of carbide slag-CO2-water reaction system in a bubble column were studied, which included the bubble Sauter mean diameter, gas holdup, bubble residence time, and the gas-liquid interfacial area. Bubble flow behaviors in the reactor were characterized by analyzing the bed pressure signals. The effects of the gas velocity (U g ) and liquid to solid ratio (L/S ratio) were discussed and analyzed. The results showed that the larger bubbles were easy to form at the larger L/S ratio, which indicated that the bubble coalescence was promoted. The gas holdup was larger when increasing U g or reducing the L/S ratio. The better gas-liquid interfacial areas were found in a wide range of L/S ratio at U g = 0.082 m/s. The optimum conditions were found at U g = 0.082 m/s and L/S ratio = 15–30 mL/g for the better gas-liquid interfacial area and the higher carbide slag conversion. The work provided the theoretical basis for the direct aqueous carbonation of the carbide slag and the operation condition optimization.
Funding source: National Natural Science Foundation of China
Award Identifier / Grant number: 51706108
Funding source: Nanjing Normal University
Award Identifier / Grant number: 184080H202B73
Funding source: National Natural Science Foundation of China
Award Identifier / Grant number: 5210060338
Funding source: Jiangsu Natural Science Foundation BK20200731
Nomenclature
- Symbols
- a int
-
gas-liquid interfacial area
- d 32
-
Sauter mean diameter
- F
-
dimensionless number
- Mo
-
Morton number
- U g
-
superficial gas velocity
- U b
-
bubble rise velocity
- t
-
bubble residence time
- Greek symbols
- ε g
-
gas holdup
- ρ
-
density
- σ
-
Surface tension
- μ
-
Viscosity
-
Author contributions: All the authors have accepted responsibility for the entire content of this submitted manuscript and approved submission.
-
Research funding: This study was financially supported by the National Natural Science Foundation of China (51706108), Natural Science Foundation of Jiangsu Higher Education Institutions of China (17KJB470008), and Research Startup Project of Nanjing Normal University (184080H202B73).
-
Conflict of interest statement: The authors have declared no conflict of interest.
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