Abstract
Engineering quantum phases using light is a novel route to designing functional materials, where light-induced superconductivity is a successful example. Although this phenomenon has been realized experimentally, especially for the high- cuprates, the underlying mechanism remains mysterious. Using the recently developed variational non-Gaussian exact diagonalization method, we investigate a particular type of photoenhanced superconductivity by suppressing a competing charge order in a strongly correlated electron-electron and electron-phonon system. We find that the -wave superconductivity pairing correlation can be enhanced by a pulsed laser, consistent with recent experiments based on gap characterizations. However, we also find that the pairing correlation length is heavily suppressed by the pump pulse, indicating that light-enhanced superconductivity may be of fluctuating nature. Our findings also imply a general behavior of nonequilibrium states with competing orders, beyond the description of a mean-field framework.
1 More- Received 9 January 2021
- Revised 17 July 2021
- Accepted 9 September 2021
DOI:https://doi.org/10.1103/PhysRevX.11.041028
Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article’s title, journal citation, and DOI.
Published by the American Physical Society
Physics Subject Headings (PhySH)
Popular Summary
Superconductivity, in which electricity flows with zero resistance below some critical temperature, has a wide range of potential applications. Progress is hampered, however, by the need for impractically low temperatures. Cuprate superconductors, made from a type of copper oxide, hold the record for high superconducting temperature without the need for extreme pressure. Strong laser pulses can trigger transient superconductivity at even higher temperatures, though the underlying mechanism remains elusive. Using a new computational method, we explore what drives this phenomenon.
Tackling the theoretical side of this problem is challenging because of the strong correlations among electrons, coupling with phonons (quanta of lattice vibrations), as well as additional complications from the ultrafast laser. Our approach separates the electronic wave function, the phonon wave function, and the entanglement between them. This allows us to solve the dynamics of each component using different techniques and self-consistently evolve the entire wave function.
Consistent with recent experiments, our method finds that a pulse laser can enhance the strength of an unconventional pairing symmetry known as -wave pairing, which manifests as an increase of electron Cooper pairs responsible for superconductivity. However, the pairing is not sustained over relatively long distances, indicating that the induced Cooper pairs are essentially local. Therefore, light-induced superconductivity may be of a fluctuating nature.
Our method will initiate various revolutionary opportunities in simulating nonequilibrium experiments, such as pump-probe and x-ray scattering, on strongly correlated materials. Our study also represents the first important step toward understanding ultrafast light-induced phenomena in correlated materials with evident lattice effects.