Abstract
Quantum networks enable a broad range of practical and fundamental applications spanning from distributed quantum computing to sensing and metrology. A cornerstone of such networks is an interface between telecom photons and quantum memories, which has proven challenging for the case of spin-mechanical memories. Here we demonstrate a novel approach based on cavity optomechanics that utilizes the susceptibility of spin qubits to strain. We use it to control electronic spins of nitrogen vacancy centres in diamond with photons in the 1,550 nm telecommunication wavelength band. This method does not involve qubit optical transitions and is insensitive to spectral diffusion. Furthermore, our approach can be applied to solid-state qubits in a wide variety of materials, expanding the toolbox for quantum information processing.
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Source data are provided with this paper. All other data that support the plots within this paper and other findings of this study are available from the corresponding author upon reasonable request.
References
Degen, C. L., Reinhard, F. & Cappellaro, P. Quantum sensing. Rev. Mod. Phys. 89, 35002 (2017).
Gisin, N., Ribordy, G., Tittel, W. & Zbinden, H. Quantum cryptography. Rev. Mod. Phys. 74, 145–195 (2002).
Ladd, T. D. et al. Quantum computers. Nature 464, 45–53 (2010).
Kimble, H. J. The quantum internet. Nature 453, 1023–1030 (2008).
Awschalom, D. D., Hanson, R., Wrachtrup, J. & Zhou, B. B. Quantum technologies with optically interfaced solid-state spins. Nat. Photon. 12, 516–527 (2018).
Hensen, B. et al. Loophole-free Bell inequality violation using electron spins separated by 1.3 kilometres. Nature 526, 682–686 (2015).
Togan, E. et al. Quantum entanglement between an optical photon and a solid-state spin qubit. Nature 466, 730–734 (2010).
Faraon, A., Santori, C., Huang, Z., Acosta, V. M. & Beausoleil, R. G. Coupling of nitrogen-vacancy centers to photonic crystal cavities in monocrystalline diamond. Phys. Rev. Lett. 109, 033604 (2012).
Ruf, M., Weaver, M. J., van Dam, S. B. & Hanson, R. Resonant excitation and Purcell enhancement of coherent nitrogen-vacancy centers coupled to a Fabry-Pérot micro-cavity. Phys. Rev. Appl. 15, 024049 (2021).
Wang, H. & Lekavicius, I. Coupling spins to nanomechanical resonators: toward quantum spin-mechanics. Appl. Phys. Lett. 117, 230501 (2020).
Lee, D., Lee, K. W., Cady, J. V., Ovartchaiyapong, P. & Jayich, A. C. B. Topical review: spins and mechanics in diamond. J. Opt. 19, 33001 (2017).
Aspelmeyer, M., Kippenberg, T. J. & Marquardt, F. Cavity optomechanics. Rev. Mod. Phys. 86, 1391–1452 (2014).
Delsing, P. et al. The 2019 surface acoustic waves roadmap. J. Phys. D 52, 353001 (2019).
Leibfried, D., Blatt, R., Monroe, C. & Wineland, D. Quantum dynamics of single trapped ions. Rev. Mod. Phys. 75, 281–324 (2003).
Bienfait, A. et al. Phonon-mediated quantum state transfer and remote qubit entanglement. Science 364, 368–371 (2019).
Macquarrie, E. R., Gosavi, T. A., Jungwirth, N. R., Bhave, S. A. & Fuchs, G. D. Mechanical spin control of nitrogen-vacancy centers in diamond. Phys. Rev. Lett. 111, 227602 (2013).
Golter, D. A. et al. Coupling a surface acoustic wave to an electron spin in diamond via a dark state. Phys. Rev. X 6, 41060 (2016).
Whiteley, S. J. et al. Spin-phonon interactions in silicon carbide addressed by Gaussian acoustics. Nat. Phys. 15, 490–495 (2019).
Maity, S. et al. Coherent acoustic control of a single silicon vacancy spin in diamond. Nat. Commun. 11, 193 (2020).
Meesala, S. et al. Enhanced strain coupling of nitrogen-vacancy spins to nanoscale diamond cantilevers. Phys. Rev. Appl. 5, 34010 (2016).
Ovartchaiyapong, P., Lee, K. W., Myers, B. A. & Jayich, A. C. B. Dynamic strain-mediated coupling of a single diamond spin to a mechanical resonator. Nat. Commun. 5, 4429 (2014).
Barfuss, A., Teissier, J., Neu, E., Nunnenkamp, A. & Maletinsky, P. Strong mechanical driving of a single electron spin. Nat. Phys. 11, 820–824 (2015).
Arcizet, O. et al. A single nitrogen-vacancy defect coupled to a nanomechanical oscillator. Nat. Phys. 7, 879–883 (2011).
Pigeau, B. et al. Observation of a phononic Mollow triplet in a multimode hybrid spin-nanomechanical system. Nat. Commun. 6, 8603 (2015).
Ohta, R. et al. Rare-earth-mediated optomechanical system in the reversed dissipation regime. Phys. Rev. Lett. 126, 47404 (2021).
Burek, M. J. et al. Diamond optomechanical crystals. Optica 3, 1404–1411 (2016).
Mitchell, M. et al. Single-crystal diamond low-dissipation cavity optomechanics. Optica 3, 963–970 (2016).
Cohen, J. D. et al. Phonon counting and intensity interferometry of a nanomechanical resonator. Nature 520, 522–525 (2015).
Wallucks, A., Marinković, I., Hensen, B., Stockill, R. & Gröblacher, S. A quantum memory at telecom wavelengths. Nat. Phys. 16, 772–777 (2020).
Regal, C. A. & Lehnert, K. W. From cavity electromechanics to cavity optomechanics. J. Phys. Conf. Ser. 264, 12025 (2011).
Mirhosseini, M., Sipahigil, A., Kalaee, M. & Painter, O. Superconducting qubit to optical photon transduction. Nature 588, 599–603 (2020).
Forsch, M. et al. Microwave-to-optics conversion using a mechanical oscillator in its quantum ground state. Nat. Phys. 16, 69–74 (2020).
Lauk, N. et al. Perspectives on quantum transduction. Quantum Sci. Technol. 5, 020501 (2020).
Doherty, M. W. et al The nitrogen-vacancy colour centre in diamond. https://doi.org/10.1016/j.physrep.2013.02.001 (2013).
Soykal, Ö. O., Ruskov, R. & Tahan, C. Sound-based analogue of cavity quantum electrodynamics in silicon. Phys. Rev. Lett. 107, 235502 (2011).
Yeo, I. et al. Strain-mediated coupling in a quantum dot-mechanical oscillator hybrid system. Nat. Nanotechnol. 9, 106–110 (2014).
Mitchell, M., Lake, D. P. & Barclay, P. E. Realizing Q > 300 000 in diamond microdisks for optomechanics via etch optimization. APL Photon. 4, 16101 (2019).
Rokhsari, H., Kippenberg, T. J., Carmon, T. & Vahala, K. J. Radiation-pressure-driven micro-mechanical oscillator. Opt. Express 13, 5293–5301 (2005).
Hossein-Zadeh, M. & Vahala, K. J. Observation of injection locking in an optomechanical rf oscillator. Appl. Phys. Lett. 93, 191115 (2008).
Hong, B. & Hajimiri, A. A general theory of injection locking and pulling in electrical oscillators–part II: amplitude modulation in LC oscillators, transient behavior, and frequency division. IEEE J. Solid State Circuits 54, 2122–2139 (2019).
Gruber, A. et al. Scanning confocal optical microscopy and magnetic resonance on single defect centers. Science 276, 2012–2014 (1997).
Udvarhelyi, P., Shkolnikov, V. O., Gali, A., Burkard, G. & Pályi, A. Spin–strain interaction in nitrogen-vacancy centers in diamond. Phys. Rev. B 98, 75201 (2018).
MacQuarrie, E. R. et al. Coherent control of a nitrogen-vacancy center spin ensemble with a diamond mechanical resonator. Optica 2, 233–238 (2015).
Hong, S. et al. Coherent, mechanical control of a single electronic spin. Nano Lett. 12, 3920–3924 (2012).
MacQuarrie, E. R., Gosavi, T. A., Bhave, S. A. & Fuchs, G. D. Continuous dynamical decoupling of a single diamond nitrogen-vacancy center spin with a mechanical resonator. Phys. Rev. B 92, 224419 (2015).
Chen, H. Y., MacQuarrie, E. R. & Fuchs, G. D. Orbital state manipulation of a diamond nitrogen-vacancy center using a mechanical resonator. Phys. Rev. Lett. 120, 167401 (2018).
Lee, K. W. et al. Strain coupling of a mechanical resonator to a single quantum emitter in diamond. Phys. Rev. Appl. 6, 34005 (2016).
Poot, M., Fong, K. Y., Bagheri, M., Pernice, W. H. P. & Tang, H. X. Backaction limits on self-sustained optomechanical oscillations. Phys. Rev. A 86, 53826 (2012).
Lake, D. P., Mitchell, M., Sukachev, D. D. & Barclay, P. E. Processing light with an optically tunable mechanical memory. Nat. Commun. 12, 663 (2021).
Neuman, T. et al. A phononic interface between a superconducting quantum processor and quantum networked spin memories. npj Quantum Inf. 7, 121 (2021).
Meesala, S. et al. Strain engineering of the silicon-vacancy center in diamond. Phys. Rev. B 97, 205444 (2018).
MacCabe, G. S. et al. Nano-acoustic resonator with ultralong phonon lifetime. Science 370, 840–843 (2020).
Li, P.-B., Zhou, Y., Gao, W.-B. & Nori, F. Enhancing spin–phonon and spin–spin interactions using linear resources in a hybrid quantum system. Phys. Rev. Lett. 125, 153602 (2020).
Chamberland, C. et al. Building a fault-tolerant quantum computer using concatenated cat codes. Preprint at https://arxiv.org/abs/2012.04108 (2020).
MacQuarrie, E. R., Otten, M., Gray, S. K. & Fuchs, G. D. Cooling a mechanical resonator with nitrogen-vacancy centres using a room temperature excited state spin-strain interaction. Nat. Commun. 8, 14358 (2017).
Kettler, J. et al. Inducing micromechanical motion by optical excitation of a single quantum dot. Nat. Nanotechnol. https://doi.org/10.1038/s41565-020-00814-y (2020)
Ghobadi, R., Wein, S., Kaviani, H., Barclay, P. & Simon, C. Progress toward cryogen-free spin-photon interfaces based on nitrogen-vacancy centers and optomechanics. Phys. Rev. A 99, 53825 (2019).
Acknowledgements
This work was supported by the Alberta Innovates Strategic Research Project (G2018000888), the Canada Foundation for Innovation (CGI Project 36130), the National Research Council Nanotechnology Research Centre, the NSERC Discovery Grant (RGPIN/04535-2016), Strategic Partnership Grant (STPGP/521536-2018, STPGP/493807-2016), Accelerator, CREATE and RTI programmes. We thank H. Jayakumar, J. P. Hadden, T. Masuda and B. Khanaliloo for contributions to the initial setup of the experimental apparatus.
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P.K.S., D.P.L. and D.D.S. set up and optimized the experiment. P.K.S. and D.P.L. measured the experimental data. P.K.S. and D.D.S. analysed the data and independently simulated the results in discussion with P.E.B. P.K.S., D.P.L. and M.J.M. prepared the sample for the experiment. P.E.B. was responsible for experimental infrastructure. P.K.S., D.D.S. and P.E.B. wrote the manuscript with input from and discussion with the co-authors. P.E.B. supervised the overall project and its direction. All the authors critically read the manuscript and approved it.
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Extended data
Extended Data Fig. 1 Experimental setup.
a) Image of the inside of the sample chamber. b) Widefield optical image of fiber taper coupled microdisk. c) Schematic of the basic setup.
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Source Data Fig. 4
All the final experimental data plotted in Fig. 4.
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Shandilya, P.K., Lake, D.P., Mitchell, M.J. et al. Optomechanical interface between telecom photons and spin quantum memory. Nat. Phys. 17, 1420–1425 (2021). https://doi.org/10.1038/s41567-021-01364-3
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DOI: https://doi.org/10.1038/s41567-021-01364-3
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