Two deep-ultraviolet nonlinear optical monolayers obtained by a template-optimized design strategy

Abudukadi Tudi; Shujuan Han; Zhihua Yang; Shilie Pan

doi:10.1039/D1QI00945A

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Two deep-ultraviolet nonlinear optical monolayers obtained by a template-optimized design strategy†

Abudukadi Tudi,

^ab Shujuan Han,

^ab Zhihua Yang

*^ab and Shilie Pan

*^ab

Author affiliations

* Corresponding authors

^a CAS Key Laboratory of Functional Materials and Devices for Special Environments; Xinjiang Technical Institute of Physics & Chemistry, CAS; Xinjiang Key Laboratory of Electronic Information Materials and Devices, 40-1 South Beijing Road, Urumqi 830011, China
E-mail: zhyang@ms.xjb.ac.cn, slpan@ms.xjb.ac.cn

^b Center of Materials Science and Optoelectronics Engineering, University of Chinese Academy of Sciences, Beijing 100049, China

Abstract

Two-dimensional (2D) nonlinear optical monolayers are brilliant candidates for future nanoscale laser devices, typically within the deep ultraviolet (DUV) region. In our work, we propose a material template-optimized design strategy to obtain two 2D materials BOF and B₃O₃F₃. Both of them show extremely large band gaps (10.76 and 9.25 eV) and a proper second harmonic generation (SHG) response. The BOF and B₃O₃F₃ layers also show SHG anisotropy.

This article is part of the themed collection: 2021 Inorganic Chemistry Frontiers HOT articles

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Article information

DOI: https://doi.org/10.1039/D1QI00945A
Article type: Research Article
Submitted: 29 Jul 2021
Accepted: 02 Sep 2021
First published: 03 Sep 2021

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Inorg. Chem. Front., 2021,8, 4791-4795

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Two deep-ultraviolet nonlinear optical monolayers obtained by a template-optimized design strategy

A. Tudi, S. Han, Z. Yang and S. Pan, Inorg. Chem. Front., 2021, 8, 4791 DOI: 10.1039/D1QI00945A

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Inorganic Chemistry Frontiers

Two deep-ultraviolet nonlinear optical monolayers obtained by a template-optimized design strategy†

Abstract

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Two deep-ultraviolet nonlinear optical monolayers obtained by a template-optimized design strategy

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