• Open Access

Dynamical phase shift in x-ray absorption and ionization spectra by two delayed x-ray laser fields

Viktoriia Savchenko, Faris Gel'mukhanov, Tim Laarmann, Sergey P. Polyutov, and Victor Kimberg
Phys. Rev. A 104, 013114 – Published 26 July 2021

Abstract

We study theoretically x-ray absorption and ionization spectra of an atom or molecule by two coherent x-ray pulses that show a relative phase shift resulting in a time delay of the pulse envelopes. We demonstrate that the phase modulation of the spectra is shifted with respect to the phase oscillation comb of the x-ray double pulse. The reason for this shift is the dynamics of the process defined by the interplay of the delay time, the pulse width, the detuning, and the lifetime of the core-excited state.

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  • Received 24 March 2021
  • Revised 4 May 2021
  • Accepted 2 July 2021

DOI:https://doi.org/10.1103/PhysRevA.104.013114

Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article's title, journal citation, and DOI. Funded by Bibsam.

Published by the American Physical Society

Physics Subject Headings (PhySH)

Atomic, Molecular & Optical

Authors & Affiliations

Viktoriia Savchenko1,2, Faris Gel'mukhanov1,2,3, Tim Laarmann4,5, Sergey P. Polyutov1,6, and Victor Kimberg1,2,*

  • 1International Research Center of Spectroscopy and Quantum Chemistry–IRC SQC, Siberian Federal University, 660041 Krasnoyarsk, Russia
  • 2Department of Theoretical Chemistry and Biology, KTH Royal Institute of Technology, 10691 Stockholm, Sweden
  • 3Institute for Methods and Instrumentation in Synchrotron Radiation Research FG-ISRR, Helmholtz-Zentrum Berlin für Materialien und Energie, Albert-Einstein-Strasse 15, 12489 Berlin, Germany
  • 4Deutsches Elektronen-Synchrotron DESY, Notkestr. 85, 22607 Hamburg, Germany
  • 5The Hamburg Centre for Ultrafast Imaging CUI, Luruper Chaussee 149, 22761 Hamburg, Germany
  • 6Kirensky Institute of Physics, Federal Research Center KSC SB RAS, 660036 Krasnoyarsk, Russia

  • *kimberg@kth.se

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Issue

Vol. 104, Iss. 1 — July 2021

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