Issue 9, 2021

Dimensionality control of magnetic coupling at interfaces of cuprate–manganite superlattices

Abstract

The dimensionality of the crystal structure plays a vital role in artificial heterostructures composed of different transition metal oxides. Nonlinear layer-thickness dependence of the exchange bias effect was observed in high-quality SrCuO2/La0.7Sr0.3MnO (LSMO) superlattices induced in the present work by dimensional evolution. In the SCO(n)/LSMO(8) superlattices with thickness below the critical value (5 u.c.), the exchange bias effect decreased and the saturated magnetization increased with increase in SCO thickness. By contrast, the exchange bias effect increased and the saturated magnetization decreased in S(n)L(8) superlattices with thickness above the critical value. This is because the lattice SCO material underwent a breathing-like structural transformation from the planar to a chain-like structure. The results indicate the interfacial superexchange coupling mainly present in the chain-like S(n)L(8) superlattices through X-ray absorption spectroscopy and first principles calculations. This superexchange coupling generated a weak localized magnetic moment to pin the adjacent ferromagnetic layer. However, in the thicker S(n)L(8) superlattices, evolution of magnetic properties was induced by the long-range antiferromagnetic order in the planar SCO layer. Our findings demonstrate that the dimensionality driven structural variation is an effective method to manipulate the electronic reconstruction and the associated physical properties, paving a pathway for the advancement of strongly correlated materials.

Graphical abstract: Dimensionality control of magnetic coupling at interfaces of cuprate–manganite superlattices

Supplementary files

Article information

Article type
Communication
Submitted
18 May 2021
Accepted
16 Jun 2021
First published
19 Jun 2021

Mater. Horiz., 2021,8, 2485-2493

Dimensionality control of magnetic coupling at interfaces of cuprate–manganite superlattices

G. Zhou, H. Ji, Z. Yan, P. Kang, Z. Li and X. Xu, Mater. Horiz., 2021, 8, 2485 DOI: 10.1039/D1MH00790D

To request permission to reproduce material from this article, please go to the Copyright Clearance Center request page.

If you are an author contributing to an RSC publication, you do not need to request permission provided correct acknowledgement is given.

If you are the author of this article, you do not need to request permission to reproduce figures and diagrams provided correct acknowledgement is given. If you want to reproduce the whole article in a third-party publication (excluding your thesis/dissertation for which permission is not required) please go to the Copyright Clearance Center request page.

Read more about how to correctly acknowledge RSC content.

Social activity

Spotlight

Advertisements