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Quantifying F and Cl concentrations in granitic melts from apatite inclusions in zircon

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Abstract

Apatite inclusions hosted by zircon offer a means to probe the magmatic history of granitic rocks and better constrain the volatile budgets of crystallising granitic melts. Building on recently developed F–Cl–OH partitioning models for apatite and coexisting melt, we outline an approach for estimating the melt concentrations of F and Cl from the composition of apatite inclusions in zircon, constrained by Ti-in-zircon crystallisation temperatures. The melts in equilibrium with apatite inclusions in zircon for the ‘I-type’ Jindabyne, Why Worry and Cobargo granitic suites of the Lachlan Orogen (eastern Australia), have Cl concentrations of 20–2880 ppm and F concentrations of 65–575 ppm. Variations in melt Cl and F concentrations between the granitic suites is attributed to differences in source compositions, specifically the relative contribution of F-rich turbiditic sediments and Cl-rich juvenile arc magmas. Within individual granitic suites, the calculated melt F and Cl concentrations decrease with magmatic differentiation and falling melt temperatures, and this appears to reflect the partitioning of Cl and F into biotite and hornblende, and into exsolving aqueous fluids. This study demonstrates that apatite-melt exchange coefficients for F, Cl and OH can be applied to apatite inclusions in zircon to quantify the F and Cl content of the melt, without additional context from the host rock samples.

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Acknowledgements

LKL gratefully acknowledges the financial support of the Society of Economic Geologists Foundation, through a Hugo Dummett Mineral Discovery Fund student research grant. CJH acknowledges a Robert and Maude Gledden Senior Visiting Fellowship at the University of Western Australia in 2019, and an Emeritus Fellowship from the Leverhulme Trust EM-2017-047\4. We are grateful to J. Craven, R. Hinton and C. Talavera for their assistance with secondary ion mass spectrometry analysis at the Edinburgh Ion Microprobe Facility. We also thank J. Hammerli for assistance with LA-ICPMS analyses, conducted at The University of Western Australia with instrumentation part funded by the Australian Research Council (LE100100203 and LE150100013). We acknowledge the facilities, and the scientific and technical assistance of the Australian Microscopy & Microanalysis Research Facility at the Centre for Microscopy, Characterisation & Analysis, The University of Western Australia, a facility funded by the University, State and Commonwealth Governments.

Funding

This research was supported by a grant from the Hugo Dummett Mineral Discovery Fund, awarded by the Society of Economic Geologists Foundation.

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  1. Centre for Exploration Targeting, School of Earth Sciences, University of Western Australia, 35 Stirling Hwy, Crawley, 6009, Australia

    Lillian A. Kendall-Langley & Anthony I. S. Kemp

  2. School of Earth Sciences, University of Bristol, Wills Memorial Building, Queen’s Road, Bristol, BS8 1RJ, UK

    Chris J. Hawkesworth

  3. Centre for Microscopy, Characterisation and Analysis, University of Western Australia, 35 Stirling Hwy, Crawley, 6009, Australia

    Malcolm P. Roberts

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Kendall-Langley, L.A., Kemp, A.I.S., Hawkesworth, C.J. et al. Quantifying F and Cl concentrations in granitic melts from apatite inclusions in zircon. Contrib Mineral Petrol 176, 58 (2021). https://doi.org/10.1007/s00410-021-01813-5

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