Register      Login
Marine and Freshwater Research Marine and Freshwater Research Society
Advances in the aquatic sciences
RESEARCH ARTICLE

Potential water pollution from recycled concrete aggregate material

K. Purdy A , J. K. Reynolds A and I. A. Wright https://orcid.org/0000-0002-8567-4797 A B
+ Author Affiliations
- Author Affiliations

A School of Science, Western Sydney University, Locked Bag 1797, Penrith, NSW 2751, Australia.

B Corresponding author. Email: i.wright@westernsydney.edu.au

Marine and Freshwater Research 72(1) 58-65 https://doi.org/10.1071/MF19354
Submitted: 10 November 2019  Accepted: 2 April 2020   Published: 26 May 2020

Abstract

Recycled concrete aggregates (RCA) are a widely used recycled building material. RCA materials have many uses such as a road base or backfilling trenches. Our study investigated the potential water-contamination risks of water exposed to RCA materials. We recirculated water for 60 min through four different treatments. Two treatments were a PVC gutter filled with different size grades of RCA material (20 mm and 45 mm), the third treatment was a clean PVC gutter and the fourth and final treatment was an unused concrete water pipe. Results showed that RCA material exposed to water released a suite of contaminants that could be ecologically hazardous to aquatic species. RCA leached metals over the 60-min recirculation (aluminium, arsenic, barium, chromium, lead, manganese, molybdenum, titanium, lithium and strontium). Water exposed to RCA material exceeded aquatic ecosystem guidelines for aluminium by 50 times and lead by up to 12 times. RCA materials increased pH by up to 4.35 pH units and electrical conductivity (EC) by up to 11 times the starting EC (mean 27.9 µs cm–1). We suggest that RCA materials need to be used with caution in settings that could be exposed to water and flow to waterways of conservation value.


References

ADDA (Ash Development Association of Australia) (2009). Guide to the use of fly-ash in concrete in Australia. Fly-ash data reference sheet number 1. Wollongong, NSW, Australia. Available at http://www.adaa.asn.au/uploads/default/files/adaa-ref_data_sheet_1.pdf [verified 9 November 2019].

ANZECC (Australian and New Zealand Environment and Conservation Council) (2000). ‘Australian and New Zealand Guidelines for Fresh and Marine Waters. National Water Quality Management Strategy Paper No. 4.’ (Australian and New Zealand Environment and Conservation Council: Canberra, ACT, Australia.)

APHA (American Public Health Association) (2012). ‘Standard Methods for the Examination of Water and Wastewater.’ 22nd edn. (American Public Health Association: Washington, DC, USA.)

Australian Government (2020). Department of Agriculture, Water and the Environment. Environmental Protection and Biodiversity Conservation Act 1999. Available at https://www.environment.gov.au/epbc [verified 20 April 2020].

Belmer, N., Wright, I., and Tippler, C. (2015). Urban geochemical contamination of high conservation value upland swamps, Blue Mountains Australia. Water, Air, and Soil Pollution 226, 332.
Urban geochemical contamination of high conservation value upland swamps, Blue Mountains Australia.Crossref | GoogleScholarGoogle Scholar |

Belmer, N., Tippler, C., and Wright, I. A. (2018). Aquatic ecosystem degradation of high conservation value upland swamps, Blue Mountains Australia. Water, Air, and Soil Pollution 229, .
Aquatic ecosystem degradation of high conservation value upland swamps, Blue Mountains Australia.Crossref | GoogleScholarGoogle Scholar |

Blue Mountains City Council (BMCC) (2010). Soft-engineering solutions for swamp remediation: a ‘how-to’ guide. Available at https://www.bmcc.nsw.gov.au/sites/default/files/document/files/SWAMPREMEDMANUALSECTIONONEFINAL.pdf [verified 9 November 2019].

Blue Mountains City Council (BMCC) (2016). Fact sheet caring for Blue Mountains swamps. Available at https://www.bmcc.nsw.gov.au/documents/fact-sheet-blue-mountains-swamps-caring [verified 9 November 2019].

Borris, M., Österlund, H., Marsalek, J., and Viklander, M. (2017). An exploratory study of the effects of stormwater pipeline materials on transported stormwater quality. Water Science and Technology 76, 247–255.
An exploratory study of the effects of stormwater pipeline materials on transported stormwater quality.Crossref | GoogleScholarGoogle Scholar | 28726691PubMed |

Brulliard, C., Cain, R., Do, D., Dornom, T., Evans, K., Lim, B., Olesson, E., and Young, S. (2012). The Australian Recycling Sector. Department of Sustainability, Water, Population and Communities, Canberra, ACT, Australia. Available at https://www.environment.gov.au/system/files/resources/dc87fd71-6bcb-4135-b916-71dd349fc0b8/files/australian-recycling-sector.pdf [verified 9 November 2019].

Carroll, R., Reynolds, J. K., and Wright, I. A. (2020). Geochemical signature of urbanisation in Blue Mountains upland swamps. The Science of the Total Environment 699, 134393.
Geochemical signature of urbanisation in Blue Mountains upland swamps.Crossref | GoogleScholarGoogle Scholar | 31677467PubMed |

Chambers, L. G., Chin, Y.-P., Filippelli, G. M., Gardner, C. B., Herndon, E. M., Long, D. T., Lyons, W. B., Macpherson, G. L., McElmurry, S. P., McLean, C. E., Moore, J., Moyer, R. P., Neumann, K., Nezat, C. A., Soderberg, K., Teutsch, N., and Widom, E. (2016). Developing the scientific framework for urban geochemistry. Applied Geochemistry 67, 1–20.
Developing the scientific framework for urban geochemistry.Crossref | GoogleScholarGoogle Scholar |

Commonwealth Government (2019). Temperate highland peat swamps on sandstone. Species profile and threats database. Department of the Environment and Energy. Available at http://www.environment.gov.au/cgi-bin/sprat/public/publicshowcommunity.pl?id=32 [verified 9 November 2019].

Connor, N. P., Sarraino, S., Frantz, D. E., Bushaw-Newton, K., and Macavoy, S. E. (2014). Geochemical characteristics of an urban river: influences of an urban landscape. Applied Geochemistry 47, 209–216.
Geochemical characteristics of an urban river: influences of an urban landscape.Crossref | GoogleScholarGoogle Scholar |

Davies, P., Wright, I., Jonasson, O., and Findlay, S. (2010). Impact of concrete and PVC pipes on urban water chemistry. Urban Water Journal 7, 233–241.
Impact of concrete and PVC pipes on urban water chemistry.Crossref | GoogleScholarGoogle Scholar |

DECCW (NSW Department of Environment Climate Change & Water) (2010). Specification for supply of recycled material for pavements, earthworks and drainage. Goulburn Street, Sydney. Available at https://www.epa.nsw.gov.au/~/media/EPA/Corporate%20Site/resources/waste/100004-supply-recycled-material.ashx [verified 9 November 2019].

DPIE (NSW Department of Planning, Industry and Environment) (2019). About the Biodiversity Conservation Act 2016. Available at https://www.environment.nsw.gov.au/topics/animals-and-plants/biodiversity/overview-of-biodiversity-reform [verified 10 April 2020].

Engelsen, C. J., van der Sloot, H. A., Wibetoe, G., Justnes, H., Lund, W., and Stoltenberg-Hansson, E. (2010). Leaching characterisation and geochemical modelling of minor and trace elements released from recycled concrete aggregates. Cement and Concrete Research 40, 1639–1649.
Leaching characterisation and geochemical modelling of minor and trace elements released from recycled concrete aggregates.Crossref | GoogleScholarGoogle Scholar |

Fryirs, K., Freidman, B., and Kohlhagen, T. (2012). The formation and geomorphic condition of upland swamps in the Blue Mountains: rehabilitation potential of these endangered ecosystems. In ‘Proceedings of the 6th Australian Stream Management Conference. Managing for Extremes’. 6–8 February 2012, Canberra, ACT. (Eds J. R. Grove and I. Rutherford.) pp. 1–8. (River Basin Management Society: Canberra.) Available at https://rbms.com.au/event/asm/6asm/ [verified 20 April 2020].

Fryirs, K., Freidman, B., Williams, R., and Jacobsen, G. (2014). Peatlands in eastern Australia? Sedimentology and age structure of temperate highland peat swamps on sandstone (THPSS) in the southern highlands and blue mountains, Australia. The Holocene 24, 1527–1538.
Peatlands in eastern Australia? Sedimentology and age structure of temperate highland peat swamps on sandstone (THPSS) in the southern highlands and blue mountains, Australia.Crossref | GoogleScholarGoogle Scholar |

Grella, C., Renshaw, A., and Wright, I. A. (2018). Invasive weeds in urban riparian zones: the influence of catchment imperviousness and soil chemistry across an urbanization gradient. Urban Ecosystems 21, 505–517.
Invasive weeds in urban riparian zones: the influence of catchment imperviousness and soil chemistry across an urbanization gradient.Crossref | GoogleScholarGoogle Scholar |

Jacques, D., Wang, L., Martens, E., and Mallants, D. (2010). Modelling chemical degradation of concrete during leaching with rain and soil water types. Cement and Concrete Research 40, 1306–1313.
Modelling chemical degradation of concrete during leaching with rain and soil water types.Crossref | GoogleScholarGoogle Scholar |

Jin, R., and Chen, Q. (2015). Investigation of concrete recycling in the US construction industry. Procedia Engineering 118, 894–901.
Investigation of concrete recycling in the US construction industry.Crossref | GoogleScholarGoogle Scholar |

Kaushal, S., Groffman, P., Likens, G., Belt, K., Stack, W., Kelly, V., Band, L., and Fisher, G. (2005). Increased salinization of fresh water in the northeastern United States. Proceedings of the National Academy of Sciences of the United States of America 102, 13517–13520.
Increased salinization of fresh water in the northeastern United States.Crossref | GoogleScholarGoogle Scholar | 16157871PubMed |

Kaushal, S. S., Duan, S., Doody, T. R., Haq, S., Smith, R. M., Newcomer Johnson, T. A., Newcomb, K. D., Gorman, J., Bowman, N., Mayer, P. M., Wood, K. L., Belt, K. T., and Stack, W. P. (2017). Human-accelerated weathering increases salinization, major ions, and alkalinization in fresh water across land use. Applied Geochemistry 83, 121–135.
Human-accelerated weathering increases salinization, major ions, and alkalinization in fresh water across land use.Crossref | GoogleScholarGoogle Scholar | 30220785PubMed |

Law, D., Setunge, S., Adamson, R., and Dutton, L. (2013). Effect of leaching from freshly cast concrete on pH. Magazine of Concrete Research 65, 889–897.
Effect of leaching from freshly cast concrete on pH.Crossref | GoogleScholarGoogle Scholar |

Limbachiya, M., Meddah, M. S., and Ouchagour, Y. (2012). Use of recycled concrete aggregate in fly-ash concrete. Construction & Building Materials 27, 439–449.

Mekhalfi, M., Amara, S., Robert, S., Carrière, F., and Gontero, B. (2014). Effect of environmental conditions on various enzyme activities and triacylglycerol contents in cultures of the freshwater diatom, Asterionella formosa (Bacillariophyceae). Biochimie 101, 21–30.
Effect of environmental conditions on various enzyme activities and triacylglycerol contents in cultures of the freshwater diatom, Asterionella formosa (Bacillariophyceae).Crossref | GoogleScholarGoogle Scholar | 24355202PubMed |

NSW Scientific Committee (2007). Blue Mountains swamps in the Sydney Basin bioregion: vulnerable ecological community listing. Available at https://www.environment.nsw.gov.au/topics/animals-and-plants/threatened-species/nsw-threatened-species-scientific-committee/determinations/final-determinations/2004-2007/blue-mountains-swamps-sydney-basin-bioregion-vulnerable-ecological-community-listing [verified 9 November 2019].

Rahman, M. A., Imteaz, M., Arulrajah, A., and Disfani, M. M. (2014). Suitability of recycled construction and demolition aggregates as alternative pipe backfilling materials. Journal of Cleaner Production 66, 75–84.
Suitability of recycled construction and demolition aggregates as alternative pipe backfilling materials.Crossref | GoogleScholarGoogle Scholar |

Rahman, M. A., Imteaz, M. A., Arulrajah, A., Piratheepan, J., and Disfani, M. M. (2015a). Recycled construction and demolition materials in permeable pavement systems: geotechnical and hydraulic characteristics. Journal of Cleaner Production 90, 183–194.
Recycled construction and demolition materials in permeable pavement systems: geotechnical and hydraulic characteristics.Crossref | GoogleScholarGoogle Scholar |

Rahman, M. A., Imteaz, M. A., Arulrajah, A., Disfani, M. M., and Horpibulsuk, S. (2015b). Engineering and environmental assessment of recycled construction and demolition materials used with geotextile for permeable pavements. Journal of Environmental Engineering 141, .
Engineering and environmental assessment of recycled construction and demolition materials used with geotextile for permeable pavements.Crossref | GoogleScholarGoogle Scholar |

Serres, N., Braymand, S., and Feugeas, F. (2016). Environmental evaluation of concrete made from recycled concrete aggregate implementing life cycle assessment. Journal of Building Engineering 5, 24–33.
Environmental evaluation of concrete made from recycled concrete aggregate implementing life cycle assessment.Crossref | GoogleScholarGoogle Scholar |

Setunge, S., Nguyen, N., Alexander, B., and Dutton, L. (2009). Leaching of alkali from concrete in contact with waterways. Water Air and Soil Pollution Focus 9, 381–391.
Leaching of alkali from concrete in contact with waterways.Crossref | GoogleScholarGoogle Scholar |

Tippler, C., Wright, I., and Hanlon, A. (2012). Is catchment imperviousness a keystone factor degrading urban waterways? A case study from a partly urbanised catchment (Georges River, south-eastern Australia). Water, Air, and Soil Pollution 223, 5331–5344.
Is catchment imperviousness a keystone factor degrading urban waterways? A case study from a partly urbanised catchment (Georges River, south-eastern Australia).Crossref | GoogleScholarGoogle Scholar |

Tippler, C., Wright, I. A., Davies, P. J., and Hanlon, A. (2014). The influence of concrete on the geochemical qualities of urban streams. Marine and Freshwater Research 65, 1009–1017.
The influence of concrete on the geochemical qualities of urban streams.Crossref | GoogleScholarGoogle Scholar |

USEPA (2000). ‘Assigning Values to Non-detected/non-quantified Pesticide Residues in Human Health Food Exposure Assessments.’ Office of Pesticide Programs. (US Environmental Protection Agency: Washington, DC, USA.)

Wright, I., Davies, P., Findlay, S., and Jonasson, O. (2011). A new type of water pollution: concrete drainage infrastructure and geochemical contamination of urban waters. Marine and Freshwater Research 62, 1355–1361.
A new type of water pollution: concrete drainage infrastructure and geochemical contamination of urban waters.Crossref | GoogleScholarGoogle Scholar |

Wright, I. A., Khoury, R., Ryan, M. M., Belmer, N., and Reynolds, J. K. (2018). Laboratory study of impacts of concrete fragment sizes on wetland water chemistry. Urban Water Journal 15, 61–67.
Laboratory study of impacts of concrete fragment sizes on wetland water chemistry.Crossref | GoogleScholarGoogle Scholar |

Wu, H., Duan, H., Zheng, L., Wang, J., Niu, Y., and Zhang, G. (2016). Demolition waste generation and recycling potentials in a rapidly developing flagship megacity of South China: prospective scenarios and implications. Construction & Building Materials 113, 1007–1016.
Demolition waste generation and recycling potentials in a rapidly developing flagship megacity of South China: prospective scenarios and implications.Crossref | GoogleScholarGoogle Scholar |

Yang, J., Du, Q., and Bao, Y. (2011). Concrete with recycled concrete aggregate and crushed clay bricks. Construction & Building Materials 25, 1935–1945.
Concrete with recycled concrete aggregate and crushed clay bricks.Crossref | GoogleScholarGoogle Scholar |

Yu, Q., Nagataki, S., Lin, J., Saeki, T., and Hisada, M. (2005). The leachability of heavy metals in hardened fly ash cement and cement-solidified fly ash. Cement and Concrete Research 35, 1056–1063.
The leachability of heavy metals in hardened fly ash cement and cement-solidified fly ash.Crossref | GoogleScholarGoogle Scholar |