• Open Access

Electron transport in dual-gated three-layer MoS2

Michele Masseroni, Tim Davatz, Riccardo Pisoni, Folkert K. de Vries, Peter Rickhaus, Takashi Taniguchi, Kenji Watanabe, Vladimir Fal'ko, Thomas Ihn, and Klaus Ensslin
Phys. Rev. Research 3, 023047 – Published 15 April 2021

Abstract

The low-energy band structure of few-layer MoS2 is relevant for a large variety of experiments ranging from optics to electronic transport. Its characterization remains challenging due to complex multiband behavior. We investigate the conduction band of dual-gated three-layer MoS2 by means of magnetotransport experiments. The total carrier density is tuned by voltages applied between MoS2 and both top and bottom gate electrodes. For asymmetrically biased top and bottom gates, electrons accumulate in the layer closest to the positively biased electrode. In this way, the three-layer MoS2 can be tuned to behave electronically like a monolayer. In contrast, applying a positive voltage on both gates leads to the occupation of all three layers. Our analysis of the Shubnikov–de Haas oscillations originating from different bands lets us attribute the corresponding carrier densities in the top and bottom layers. We find a twofold Landau level degeneracy for each band, suggesting that the minima of the conduction band lie at the ±K points of the first Brillouin zone. This is in contrast to band structure calculations for zero layer asymmetry, which report minima at the Q points. Even though the interlayer tunnel coupling seems to leave the low-energy conduction band unaffected, we observe scattering of electrons between the outermost layers for zero layer asymmetry. The middle layer remains decoupled due to the spin-valley symmetry, which is inverted for neighboring layers. When the bands of the outermost layers are energetically in resonance, interlayer scattering takes place, leading to an enhanced resistance and to magneto-interband oscillations.

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  • Received 14 January 2021
  • Revised 11 March 2021
  • Accepted 24 March 2021

DOI:https://doi.org/10.1103/PhysRevResearch.3.023047

Published by the American Physical Society under the terms of the Creative Commons Attribution 4.0 International license. Further distribution of this work must maintain attribution to the author(s) and the published article's title, journal citation, and DOI.

Published by the American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

Michele Masseroni1,*, Tim Davatz1, Riccardo Pisoni1, Folkert K. de Vries1, Peter Rickhaus1, Takashi Taniguchi2, Kenji Watanabe3, Vladimir Fal'ko4, Thomas Ihn1, and Klaus Ensslin1

  • 1Solid State Physics Laboratory, ETH Zürich, 8093 Zürich, Switzerland
  • 2International Center for Materials Nanoarchitectonics, 1-1 Namiki, Tsukuba 305-0044, Japan
  • 3Research Center for Functional Materials, 1-1 Namiki, Tsukuba 305-0044, Japan
  • 4National Graphene Institute, University of Manchester, Booth St. E. Manchester M13 9PL, United Kingdom

  • *masmiche@phys.ethz.ch

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Vol. 3, Iss. 2 — April - June 2021

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