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A Better Understanding of How Polymer Composition Affects Sensing Performance of Molecularly Imprinted Photonic Polymer

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Abstract

Molecularly imprinted photonic polymer is an ideal sensory material due to high specificity and selectivity. Polymer composition plays a vital role in determining its sensing performance. For better understanding the effects of polymer composition, herein we reported the interactive effects of polymer composition on sensing performance by using Response surface methodology. We fabricated L-tryptophan molecularly imprinted photonic polymer by using maleic anhydride modified by β-cyclodextrin (MAH-β-CD) and acrylamide as dual functional monomers, N,N’-methylene bisacrylamide as cross-linker. A second-order polynomial model was proposed for describing the relationship between polymer composition and its sensing performance. This model reveled that MAH-β-CD and cross-linker were dominant in determining the sensing performance of demonstrated molecularly imprinted photonic polymer, and proved the existence of interactive effects of polymer composition on sensing performance, which have been ignored before and need to be considered in the future study of molecularly imprinted photonic polymer. It is anticipated that this work would provide an important guidance for rational design of molecularly imprinted photonic polymer.

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Funding

This work was funded by the National Nature Science Foundation of China (Grant no. 21571084), National First-Class Discipline Program of Light Industry Technology and Engineering (LIFE2018-19), and MOE and SAFEA for the 111 Project (B13025).

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Authors and Affiliations

  1. School of Mechanical Technology, Wuxi Institute of Technology, 214121, Wuxi, China

    Zhaokun Yang & Zhangyong Yu

  2. Key Laboratory of Synthetic and Biological Colloids, Ministry of Education, School of Chemical and Material Engineering, Jiangnan University, 214122, Wuxi, China

    Zhaokun Yang, Dongjian Shi, Shirong Liu & Mingqing Chen

Authors
  1. Zhaokun Yang
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  2. Zhangyong Yu
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  3. Dongjian Shi
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  4. Shirong Liu
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Correspondence to Zhangyong Yu or Mingqing Chen.

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Zhaokun Yang, Yu, Z., Shi, D. et al. A Better Understanding of How Polymer Composition Affects Sensing Performance of Molecularly Imprinted Photonic Polymer. Polym. Sci. Ser. B 63, 142–151 (2021). https://doi.org/10.1134/S1560090421020111

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  • DOI: https://doi.org/10.1134/S1560090421020111

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