Skip to content
Licensed Unlicensed Requires Authentication Published by De Gruyter (O) January 26, 2021

Revisiting cross sections for proton induced reactions on natural lead between 10 and 80 MeV

  • Salim Gülez , Bhawna Pandey and Erik Strub EMAIL logo
From the journal Radiochimica Acta

Abstract

This work is focused on the natPb(p,xn)207Bi reaction to extend earlier works on proton induced reactions for the determination of cross sections of residual nuclides. 207Bi decay (half-life 31.55 years) was measured by γ-ray spectrometry in 42 lead foils which had been irradiated by high proton fluxes 20 years ago. Since then, all short-lived radionuclides produced during the irradiation have decayed, so the background is strongly reduced and the cross section could be measured more precisely than during the original measurements. The results are found to be in very good agreement with the historical record. Additionally, theoretical calculations with modern Monte Carlo based codes were performed to compare the calculations of various Bi, Tl and Pb reactions with the historical data and with additional data from literature. The deviations of the new data from both theoretical calculations using EMPIRE and TALYS are discussed.


Corresponding author: Erik Strub, Abteilung Nuklearchemie, Universität zu Köln, Zülpicher Str. 45, 50674Köln, Germany, E-mail:

  1. Author contribution: All the authors have accepted responsibility for the entire content of this submitted manuscript and approved submission.

  2. Research funding: No external funding was used for this work.

  3. Conflict of interest statement: The authors declare no conflicts of interest regarding this article.

References

1. Gloris, M. Protonen-induzierte Restkernproduktion in schweren Elementen bei mittleren Energien. Doctoral Thesis, University of Hannover, Germany, 1998.Search in Google Scholar

2. Sudbrock, F. Experimentelle und theoretische Studien zur Restkernproduktion bei Spallations-und Fragmentationsreaktionen. Doctoral Thesis, University of Cologne, Germany, 1998.Search in Google Scholar

3. Bodemann, R., Lange, H. J., Leya, I., Michel, R., Schiekel, T., Rösel, R., Herpers, U., Hofmann, H. J., Dittrich, B., Suter, M., Wölfli, W., Holmqvist, B., Condé, H., Malmborg, P. Production of residual nuclei by proton-induced reactions on C, N, O, Mg, AI and Si. Nucl. Instrum. Methods Phys. Res. B 1993, 82, 9. https://doi.org/10.1016/0168-583x(93)95077-i.Search in Google Scholar

4. Ammon, K., Leya, I., Lavielle, B., Gilabert, E., David, J. C., Herpers, U., Michel, R. Cross sections for the production of helium, neon and argon isotopes by proton-induced reactions on iron and nickel. Nucl. Instrum. Methods Phys. Res. B 2008, 266, 2. https://doi.org/10.1016/j.nimb.2007.10.024.Search in Google Scholar

5. Michel, R., Hansmann, D., Neumann, S., Glasser, W., Schuhmacher, H., Dangendorf, V., Nolte, R., Herpers, U., Smirnov, A. N., Ryzhov, I. V., Prokofiev, A. V., Malmborg, P., Kollár, D., Meulders, J. P. Excitation functions for the production of radionuclides by neutron-induced reactions on C, O, Mg, Al, Si, Fe, Co, Ni, Cu, Ag, Te, Pb, and U up to 180 MeV. Nucl. Instrum. Methods Phys. Res. B 2015, 343, 30. https://doi.org/10.1016/j.nimb.2014.11.006.Search in Google Scholar

6. Michel, R., Gloris, M., Protoschill, J., Herpers, U., Kuhnhenn, J., Sudbrock, F., Malmborg, P., Kubik, P. Cross sections for the production of radionuclides by proton-induced reactions on W, Ta, Pb and Bi from thresholds up to 2.6 GeV. J. Nucl. Sci. Technol. 2002, 39(Suppl. 2), 242. https://doi.org/10.1080/00223131.2002.10875084.Search in Google Scholar

7. Issa, S. A. M., Uosif, M. A. M., Michel, R., Herpers, U., Malmborg, P., Holmqvist, B. Proton-induced production of residual radionuclides in natRe up to 2590 MeV. Nucl. Instrum. Methods Phys. Res. B 2013, 298, 19. https://doi.org/10.1016/j.nimb.2013.01.001.Search in Google Scholar

8. Kuhnhenn, J., Herpers, U., Glasser, W., Michel, R., Kubik, P. W., Suter, M. Thin target cross sections for proton-induced formation of radionuclides from lead for Ep ≤ 71 MeV. Radiochim. Acta 2001, 89, 697. https://doi.org/10.1524/ract.2001.89.11-12.697.Search in Google Scholar

9. Kuhnhenn, J. Protonen-induzierte Erzeugung radioaktiver Restkerne in Blei und Bismut bei Energien bis 71 MeV. Doctoral Thesis, University of Cologne, Germany, 2001.Search in Google Scholar

10. Michel, R., Bodemann, R., Busemann, H., Dam, R., Gloris, M., Lange, H., Schnatz-Büttgen, M., Herpers, U., Schiekel, T., Sudbrock, F., Holmqvist, B., Conde, H., Malmborg, P., Suter, M., Dittrich-Hannen, B., Kubik, P.-W., Sinal, H., Filges, D. Cross sections for the production of residual nuclides by low- and medium-energy protons from the target elements C, N, O, Mg, Al, Si, Ca, Ti, V, Mn, Fe, Co, Ni, Cu, Sr, Y, Zr, Nb, Ba and Au. Nucl. Instruments Methods Phys. Res. B 1997, 129, 153. https://doi.org/10.1016/s0168-583x(97)00213-9.Search in Google Scholar

11. Schiekel, T., Sudbrock, F., Herpers, U., Gloris, M., Lange, H. J., Leya, I., Michel, R., Dittrich-Hannen, B., Synal, H. A., Suter, M., Kubik, P. W., Blann, M., Filges, D. Nuclide production by proton-induced reactions on elements (6 ≤ Ζ ≤ 29) in the energy range from 200 MeV to 400 MeV. Nucl. Instrum. Methods Phys. Res. B 1996, 114, 91. https://doi.org/10.1016/0168-583x(96)00145-0.Search in Google Scholar

12. Gloris, M., Michel, R., Herpers, U., Sudbrock, F., Filges, D. Production of residual nuclei from irradiation of thin Pb-targets with protons up to 1.6 GeV. Nucl. Instrum. Methods Phys. Res. B 1996, 113, 429. https://doi.org/10.1016/0168-583x(95)01325-3.Search in Google Scholar

13. Issa, S. A. M., Uosif, M. A. M., Michel, R., Flament, J. L., David, J. C., Leray, S., Herpers, U. The production of residual nuclides via 211, 1000, 1400 and 2530 MeV protons irradiation of natural uranium. J. Radioanal. Nucl. Chem. 2015, 305, 345. https://doi.org/10.1007/s10967-015-3985-9.Search in Google Scholar

14. Michel, R., Gloris, M., Lange, H. J., Leya, I., Lüpke, M., Herpers, U., Dittrich-Hannen, B., Rösel, R., Schiekel, T., Filges, D., Dragovitsch, P., Suter, M., Hofmann, H. J., Wölfli, W., Kubik, P. W., Baur, H., Wieler, W. Nuclide production by proton-induced reactions on elements (6 ≤ Z ≤ 29) in the energy range from 800 to 2600 MeV. Nucl. Instrum. Methods Phys. Res. B 1995, 103, 183. https://doi.org/10.1016/0168-583x(95)00566-8.Search in Google Scholar

15. Dittrich, B., Herpers, U., Lüpke, M., Michel, R., Hofmann, H. J., Wölfli, W. Determination of cross sections for the production of 7Be, 10Be and 22Na by high-energy protons. Radiochim. Acta 1990, 50, 11. https://doi.org/10.1524/ract.1990.50.12.11.Search in Google Scholar

16. Dittrich, B., Herpers, U., Hofmann, H. J., Wölfli, W., Bodemann, R., Lüpke, M., Michel, R., Dragovitsch, P., Filges, D. AMS measurements of thin-target cross sections for the production of 10Be and 26Al by high-energy protons. Nucl. Instrum. Methods Phys. Res. B 1990, 52, 588. https://doi.org/10.1016/0168-583x(90)90481-9.Search in Google Scholar

17. Gloris, M., Michel, R., Sudbrock, F., Herpers, U., Malmborg, P., Holmqvist, B. Proton-induced production of residual radionuclides in lead at intermediate energies. Nucl. Instrum. Methods Phys. Res. A 2001, 463, 593. https://doi.org/10.1016/s0168-9002(01)00174-7.Search in Google Scholar

18. Firestone, R. B., Shirley, V. S., Baglin, C. M., Chu, S. Y. F., Zipkin, J. Table of Isotopes, 8th ed.; John Wiley and Sons: New York, United States of America, 1996.Search in Google Scholar

19. Herman, M., Capote, R., Sin, M., Trkov, A., Carlson, B. V., Oblozinsky, P., Mattoon, C. M., Wienke, H., Hoblit, S., Cho, Y.-S., Nobre, G. P. A., Plujko, V., Zerkin, V. EMPIRE-3.2 Malta Modular System for Nuclear Reaction Calculations and Nuclear Data Evaluation Users Manual; Report INDC(NDS)-0603, IAEA: Vienna, Austria, 2013.10.2172/1108585Search in Google Scholar

20. Herman, M., Capote, R., Carlson, B. V., Obložinský, P., Sin, M., Trkov, A., Wienke, H., Zerkin, V. EMPIRE: nuclear reaction model code system for data evaluation. Nucl. Data Sheets 2007, 108, 2655. https://doi.org/10.1016/j.nds.2007.11.003.Search in Google Scholar

21. Koning, A. J., Rochman, D., Sublet, J. C., Dzysiuk, N., Fleming, M., van der Marck, S. TENDL: complete nuclear data library for innovative nuclear science and technology. Nucl. Data Sheets 2019, 155, 1. https://doi.org/10.1016/j.nds.2019.01.002.Search in Google Scholar

22. Ziegler, J. F., Biersack, J. P., Ziegler, M. D. SRIM the Stopping and Range of Ions in Matter, Chester; United States of America: Maryland, 2015.Search in Google Scholar

23. Biersack, J. P., Haggmark, L. G. A Monte Carlo computer program for the transport of energetic ions in amorphous targets. Nucl. Instrum. Methods 1980, 174, 257. https://doi.org/10.1016/0029-554x(80)90440-1.Search in Google Scholar

24. Kondev, F. G., Lalkovski, S. Nuclear data sheets for A = 207. Nucl. Data Sheets 2011, 112, 707. https://doi.org/10.1016/j.nds.2011.02.002.Search in Google Scholar

25. Ditrói, F., Tárkányi, F., Takács, S., Hermanne, A., Ignatyuk, A. V. Excitation functions of natPb(d,x) 206,205,204,203,202Bi, 203cum,202m,201cumPb and 202cum,201cumTl reactions up to 50 MeV. J. Radioanal. Nucl. Chem. 2014, 300, 1267. https://doi.org/10.1007/s10967-014-3056-7.Search in Google Scholar

26. Lagunas-Solar, M. C., Carvacho, O. F., Nagahara, L., Mishra, A., Parks, N. J. Cyclotron production of no-carrier-added 206Bi (6.24 d) and 205Bi (15.31 d) as tracers for biological studies and for the development of alpha-emitting radiotherapeutic agents. Int. J. Radiat. Appl. Instrum. Appl. Radiat. Isot. 1987, 38, 129. https://doi.org/10.1016/0883-2889(87)90008-6.Search in Google Scholar

27. Lagunas-Solar, M. C., Haff, R. P. Theoretical and experimental excitation functions for proton induced nuclear reactions on Ζ = 10 to Ζ = 82 target nuclides. Radiochim. Acta 1993, 60, 57. https://doi.org/10.1524/ract.1993.60.23.57.Search in Google Scholar

28. Lagunas-Solar, M. C., Little, F. E., Jungerman, J. A. Proton induced reactions on natural Pb targets. A potential new cyclotron method for 201Tl production. Int. J. Appl. Radiat. Isot. 1981, 32, 129. https://doi.org/10.1016/0020-708x(81)90158-7.Search in Google Scholar


Supplementary Material

The online version of this article offers supplementary material (https://doi.org/10.1515/ract-2020-0027).


Received: 2020-03-23
Accepted: 2021-01-10
Published Online: 2021-01-26
Published in Print: 2021-04-27

© 2021 Walter de Gruyter GmbH, Berlin/Boston

Downloaded on 19.4.2024 from https://www.degruyter.com/document/doi/10.1515/ract-2020-0027/html
Scroll to top button