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Recent advances in the synthesis of mesoporous materials and their application to lithium-ion batteries and hybrid supercapacitors

  • Invited Review Paper
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Abstract

The ever-growing demand for high performance energy storage systems has fueled the development of advanced electrode materials with light weight, high energy/power densities, and stable cycle life. Mesoporous materials play an important role in achieving these goals because of their unique features such as high surface area, tunable pore size, pore volume, and pore structures, as well as adjustable particle size and morphology. In this review, we summarize the recent progress in the synthesis of mesoporous materials and their applications in lithium-ion batteries (LIBs) and lithium-ion hybrid supercapacitors (Li-HSCs) over the past ten years. The block copolymer guided soft-template route is highlighted as a simple and versatile tool for designing mesoporous materials with controlled nano-and macrostructures without complicated synthetic procedures. The structural/morphological benefits of designed mesoporous materials translate into highly improved electrochemical performance in LIBs and Li-HSCs. Finally, future challenges and perspectives on the development of mesoporous materials in energy storage devices are provided, which will be useful both in academia and in industry.

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Acknowledgements

J.H. acknowledges the support of the National Research Foundation of Korea (NRF) grant funded by the Korea government (MSIT) (No. 2020R1F1A1065283). E.L. thanks the support of the KRICT projects (No. SI2011-30 and SI2061-313) from the Korea Research Institute of Chemical Technology (KRICT). C.J. acknowledges the support of the NRF grant funded by the Korea government (No. 2020R1G1A1101146).

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  1. These authors contributed equally.

Authors and Affiliations

  1. Chemical & Process Technology Division, Korea Research Institute of Chemical Technology (KRICT), 141 Gajeongro, Daejeon, 34114, Korea

    Eunho Lim

  2. Energy & Environment Division, Korea Institute of Ceramic Engineering and Technology (KICET), Jinju, Gyeongnam, 52851, Korea

    Jinyoung Chun

  3. School of Chemical Engineering & Materials Science, Chung-Ang University (CAU), 84 Heukseok-ro, Dongjak-gu, Seoul, 06974, Korea

    Changshin Jo

  4. Department of Chemical Engineering, Ajou University, Worldcupro 206, Suwon, 16499, Korea

    Jongkook Hwang

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  1. Eunho Lim
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Correspondence to Changshin Jo or Jongkook Hwang.

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Jongkook Hwang received his Ph.D. in department of chemical engineering from Pohang University of Science and Technology (POSTECH) in 2016. After his first post-doctoral training at Max Planck Institute of Colloids and Interfaces, he moved to Utrecht University where he worked on development of heterogeneous catalysts for preferential CO oxidation in H2. In 2020, he was appointed as an assistant professor in department of chemical engineering at Ajou University, Korea. His research interest is synthesis of nanoporous materials with well-defined structures and morphologies for energy- and catalytic applications.

Changshin Jo obtained his B.S. (2010) and Ph.D. (2016) degrees in Chemical Engineering from Pohang University of Science and Technology (POSTECH). After postdoctoral research at POSTECH (with Prof. Jinwoo Lee) and University of Cambridge (as Marie Sklodowska-Curie Fellow with Prof. Michael De Volder), he joined the faculty of the School of Chemical Engineering and Materials Science at Chung-Ang University. His current research interests focus on scalable synthesis of nanostructured materials for energy storage applications.

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Lim, E., Chun, J., Jo, C. et al. Recent advances in the synthesis of mesoporous materials and their application to lithium-ion batteries and hybrid supercapacitors. Korean J. Chem. Eng. 38, 227–247 (2021). https://doi.org/10.1007/s11814-020-0693-0

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