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Hydrostatic-Pressure-Induced Reentrance of the Metallic State in the κ-(ET)2Hg(SCN)2Cl Quasi-Two-Dimensional Organic Conductor

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Abstract

On cooling below 30 K, the κ-(ET)2Hg(SCN)2Cl quasi-two-dimensional organic metal, which is in the quantum spin liquid state at liquid helium temperatures, undergoes a transition to the Mott insulator state. The application of a hydrostatic pressure p = 0.7 kbar stabilizes the metallic state and makes it possible to study the behavior of the interlayer magnetoresistance at liquid helium temperatures. The field dependence of the magnetoresistance exhibits an unlimited power-law growth, which indicates that the polaron mechanism contributes to the interlayer transport. The spectrum of observed magnetoresistance oscillations corresponds to the Fermi surfaces characteristic of conducting layers with the κ-type structure.

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References

  1. P. W. Anderson, Mater. Res. Bull. 8, 153 (1973).

    Article  Google Scholar 

  2. T.-H. Han, J. S. Helton, Sh. Chu, D. G. Nocera, J. A. Rodriguez-Rivera, C. Broholm, and Y. S. Lee, Nature (London, U.K.) 492, 406 (2012).

    Article  ADS  Google Scholar 

  3. J. S. Helton, K. Matan, M. P. Shores, E. A. Nytko, B. M. Bartlett, Y. Yoshida, Y. Takano, A. Suslov, Y. Qiu, J.-H. Chung, D. G. Nocera, and Y. S. Lee, Phys. Rev. Lett. 98, 107204 (2007).

    Article  ADS  Google Scholar 

  4. P. Mendels and F. Bert, J. Phys. Soc. Jpn. 79, 011001 (2010).

    Article  ADS  Google Scholar 

  5. M. A. de Vries, K. V. Kamenev, W. A. Kockelmann, J. Sanchez-Benitez, and A. Harrison, Phys. Rev. Lett. 100, 157205 (2008).

    Article  ADS  Google Scholar 

  6. J. S. Helton, K. Matan, M. P. Shores, E. A. Nytko, B. M. Bartlett, Y. Qiu, D. G. Nocera, and Y. S. Lee, Phys. Rev. Lett. 104, 147201 (2010).

    Article  ADS  Google Scholar 

  7. J. M. Williams, J. R. Ferraro, R. J. Thorn, K. D. Carlson, U. Geiser, H. H. Wang, A. M. Kini, and M. H. Whangbo, Organic Superconductors (Including Fullerenes) Synthesis, Structure, Properties and Theories (Prentice Hall, Englewood Cliffs, N.J., 1992).

    Google Scholar 

  8. T. Ishiguro, K. Yamaji, and G. Saito, Organic Superconductors (Springer, Berlin, 1998).

    Book  Google Scholar 

  9. L. Balents, Nature (London, U.K.) 464, 199 (2010).

    Article  ADS  Google Scholar 

  10. B. J. Powell and R. H. McKenzie, Rep. Prog. Phys. 74, 056501 (2011).

    Article  ADS  Google Scholar 

  11. K. Shimizu, K. Miyagawa, M. Kanoda, M. Maesato, and G. Saito, Phys. Rev. Lett. 91, 107001 (2003).

    Article  ADS  Google Scholar 

  12. N. Hassan, S. Cunningham, M. Mourigal, E. I. Zhilyaeva, S. A. Torunova, R. N. Lyubovskaya, J. A. Schlueter, and N. Drichko, Science (Washington, DC, U. S.) 360, 1101 (2018).

    Article  ADS  Google Scholar 

  13. R. B. Lyubovskii, R. N. Lyubovskaya, and O. A. Dyachenko, J. Phys. (France) 6, 1609 (1996).

    Article  Google Scholar 

  14. N. Drichko, R. Beyer, E. Rose, M. Dressel, A. Schlueter, S. A. Turunova, E. I. Zhilyaeva, and R. N. Lyubovskaya, Phys. Rev. B 89, 075133 (2014).

    Article  ADS  Google Scholar 

  15. N. M. Hassan, K. Thirunavukkuarasu, Z. Lu, D. Smirnov, E. I. Zhilyaeva, S. Turunova, R. N. Lyubovskaya, and N. Drichko, npj Quantum Mater. 5, 15 (2020).

    Article  ADS  Google Scholar 

  16. A. Lohle, E. Rose, S. Singh, R. Bayer, E. Tatra, T. Ivek, E. I. Zhylyaeva, R. N. Lyubovskaya, and M. Dressel, J. Phys.: Condens. Matter 29, 055601 (2017).

    ADS  Google Scholar 

  17. P. D. Grigoriev, Phys. Rev. B 88, 054415 (2013).

    Article  ADS  Google Scholar 

  18. P. D. Grigoriev, Phys. B (Amsterdam, Neth.) 407, 1932 (2012).

    Article  ADS  Google Scholar 

  19. M. V. Kartsovnik, Chem. Rev. 104, 5737 (2004).

    Article  Google Scholar 

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Correspondence to S. I. Pesotskii.

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Russian Text © The Author(s), 2020, published in Pis’ma v Zhurnal Eksperimental’noi i Teoreticheskoi Fiziki, 2020, Vol. 112, No. 9, pp. 623–625.

Funding

This work was supported by the Ministry of Science and Higher Education of the Russian Federation (state assignment no. AAAA-A19-119092390079-8, preparation of the samples) and by the Russian Foundation for Basic Research (project nos. 18-02-00308 and 18-02-00280, studies of physical characteristics).

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Lyubovskii, R.B., Pesotskii, S.I., Zverev, V.N. et al. Hydrostatic-Pressure-Induced Reentrance of the Metallic State in the κ-(ET)2Hg(SCN)2Cl Quasi-Two-Dimensional Organic Conductor. Jetp Lett. 112, 582–584 (2020). https://doi.org/10.1134/S0021364020210092

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  • DOI: https://doi.org/10.1134/S0021364020210092

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