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Selective Stimulation in Laser-Induced Synthesis of Silver Nanoparticles in Nanoporous Glass

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Moscow University Physics Bulletin Aims and scope

Abstract

Laser-induced synthesis of metal nanoparticles by the method of supercritical deposition provides a wide range of opportunities for implementing various strategies. In the present work, based on the example of silver nanoparticles in the pores of Vycor glass, we demonstrate that irradiation at the plasmon resonance frequency initiates preferential synthesis of a target group. In the present case, the initial ensemble of seeds characterized by a plasmon band at 440 nm was sequentially irradiated at 532 nm and then at 637 nm. This two-stage selective treatment leads to the appearance of a well-defined second peak at \({\sim}600\) nm, which indicates significant growth of the mass fraction of the corresponding group of the particles that were initially missing. The results we obtained clearly demonstrate that the use of plasmon properties of the nanoparticles allows tuning of the properties of the synthesized ensemble in a targeted manner.

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Funding

Research on the synthesis and diagnostics of nanoparticles, including the preparation of nanoporous samples and direct experiments, was carried out with the financial support of the Russian Foundation for Basic Research, project no. 18-29-06056. An optical scheme that allows irradiation and diagnostics of samples in a cell with a supercritical fluid was created with the financial support of the Russian Foundation for Basic Research, project no. 19-02-00978. The laser sources used in this work are part of the CARS spectrometer created with the support of The Development Program of the Moscow State University.

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Authors and Affiliations

  1. Department Physics and International Laser Center, Moscow State University, 119991, Moscow, Russia

    V. G. Arakcheev & A. N. Bekin

  2. Institute of Photon Technologies, Federal Scientific Research Center Crystallography and Photonics, Russian Academy of Sciences, 108840, Troitsk, Moscow, Russia

    N. V. Minaev

  3. Department of Physics and International Laser Center, Moscow State University, 119991, Moscow, Russia

    V. B. Morozov

  4. Skobeltsin Institute of Nuclear Physics, Moscow State University, 119991, Moscow, Russia

    A. O. Rybaltovskii

Authors
  1. V. G. Arakcheev
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  2. A. N. Bekin
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  3. N. V. Minaev
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  4. V. B. Morozov
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  5. A. O. Rybaltovskii
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Corresponding author

Correspondence to V. G. Arakcheev.

Additional information

Translated by V. Alekseev

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Arakcheev, V.G., Bekin, A.N., Minaev, N.V. et al. Selective Stimulation in Laser-Induced Synthesis of Silver Nanoparticles in Nanoporous Glass. Moscow Univ. Phys. 75, 469–474 (2020). https://doi.org/10.3103/S0027134920050057

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  • DOI: https://doi.org/10.3103/S0027134920050057

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