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Ultrafast Quantum Relaxation Dynamics of Magnetically Ordered Systems with Spin Crossover in an Excited State under a Sudden Perturbation

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Abstract

A theoretical model based on the relaxation equation for the density matrix has been proposed to describe the ultrafast time dynamics of magnetically ordered systems with spin crossover in an excited state under a sudden perturbation. Oscillations of the magnetization, the population of the high-spin state, and the generation of local vibrons at a transition of the system from the light-excited Franck-Condon low-spin state to the highspin ground state.

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Funding

This work was supported by the Russian Science Foundation (project no. 18-12-00022).

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Authors and Affiliations

  1. Kirensky Institute of Physics, Federal Research Center KSC, Siberian Branch, Russian Academy of Sciences, Akademgorodok, Krasnoyarsk, 660036, Russia

    Yu. S. Orlov & S. G. Ovchinnikov

  2. Siberian Federal University, Krasnoyarsk, 660041, Russia

    Yu. S. Orlov, S. V. Nikolaev & S. G. Ovchinnikov

  3. Centro Universitario de Ciencias Exactas e Ingenierías (CUCEI), Universidad de Guadalajara, Guadalajara, Jalisco, 44420, Mexico

    A. I. Nesterov

Authors
  1. Yu. S. Orlov
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  2. S. V. Nikolaev
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  3. S. G. Ovchinnikov
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  4. A. I. Nesterov
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Corresponding author

Correspondence to Yu. S. Orlov.

Additional information

Russian Text © The Author(s), 2020, published in Pis’ma v Zhurnal Eksperimental’noi i Teoreticheskoi Fiziki, 2020, Vol. 112, No. 4, pp. 268–274.

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Orlov, Y.S., Nikolaev, S.V., Ovchinnikov, S.G. et al. Ultrafast Quantum Relaxation Dynamics of Magnetically Ordered Systems with Spin Crossover in an Excited State under a Sudden Perturbation. Jetp Lett. 112, 250–256 (2020). https://doi.org/10.1134/S0021364020160109

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  • DOI: https://doi.org/10.1134/S0021364020160109

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