Abstract
In this work, we studied the relaxation dynamics of coherences of different orders present in a system of two coupled nuclear spins. We used a previously designed model for intrinsic noise present in such systems which considers the Lindblad master equation for Markovian relaxation. We experimentally created zero-, single- and double-quantum coherences in several two-spin systems and performed a complete state tomography and computed state fidelity. We experimentally measured the decay of zero- and double-quantum coherences in these systems. The experimental data fitted well to a model that considers the main noise channels to be a correlated phase damping (CPD) channel acting simultaneously on both spins in conjunction with a generalised amplitude damping channel acting independently on both spins. The differential relaxation of multiple-quantum coherences can be ascribed to the action of a CPD channel acting simultaneously on both the spins.
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Acknowledgements
All experiments were performed on a Bruker Avance-III 600 MHz FT-NMR spectrometer at the NMR Research Facility at IISER Mohali.
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Singh, H., Arvind & Dorai, K. Using a Lindbladian approach to model decoherence in two coupled nuclear spins via correlated phase damping and amplitude damping noise channels. Pramana - J Phys 94, 160 (2020). https://doi.org/10.1007/s12043-020-02027-3
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DOI: https://doi.org/10.1007/s12043-020-02027-3
Keywords
- Nuclear magnetic resonance relaxation theory
- Multiple quantum coherences
- Lindblad master equation
- Markovian noisy channels