Abstract
Fast speckle suppression is crucial for time-resolved full-field imaging with laser illumination. Here, we introduce a method to accelerate the spatial decoherence of laser emission, achieving speckle suppression in the nanosecond integration time scale. The method relies on the insertion of an intracavity phase diffuser into a degenerate cavity laser to break the frequency degeneracy of transverse modes and broaden the lasing spectrum. The ultrafast decoherence of laser emission results in the reduction of speckle contrast to 3% in less than 1 ns.
1 Introduction
Conventional lasers have a high degree of spatial coherence, manifesting coherent artifacts and cross-talk. One prominent example is speckle noise, which is detrimental to laser applications such as imaging, display, material processing, photolithography, optical trapping and more [1]. Several techniques have been developed to suppress speckle noise by incoherently integrating many uncorrelated speckle realizations, e.g., by using a moving diffuser or aperture [2], [3], [4], [5], [6], [7], [8], [9]. Typically, these methods are effective only at long integration times of a millisecond or longer.
Fast speckle suppression is essential for time-resolved imaging of moving targets or transient phenomena [10], [11], [12]. It can be achieved by using multimode lasers with low and tunable spatial coherence [13], [14], [15], [16], [17], [18], [19]. The decoherence time of such lasers, critical for fast speckle suppression in short integration times, is determined by the frequency spacing and linewidth of the individual lasing modes, as well as the total width of the emission spectrum
To reach low spatial coherence, a large number of transverse modes must lase simultaneously. This requires the modes to have a similar loss or quality factor, which can be achieved with a degenerate cavity laser (DCL) [21]. The DCL self-imaging configuration ensures that all transverse modes have an almost identical (degenerate) quality factor. Experimentally, it has been shown that N ≈ 320,000 transverse modes can lase simultaneously and independently in a solid-state DCL [22]. But the transverse modes are also nearly degenerate in frequency, which implies a longer decoherence (integration) time. In the short nanosecond time scale, the longitudinal modes play a critical role in spatial coherence reduction [11]. In particular, the spatiotemporal dynamics of a DCL having M longitudinal modes reduces the speckle contrast to
In this work, we develop a simple and robust method for ultrafast speckle suppression. We accelerate the spatial decoherence of a DCL by inserting a phase diffuser (random phase plate) into the cavity. The intracavity phase diffuser lifts the frequency degeneracy of transverse modes and broadens the lasing spectrum. Simultaneously, a large number of transverse modes manage to lase because of their high quality factors. The speckle contrast is reduced to 3% (below human perception level [23]) in less than 1 ns. The lasing threshold is slightly increased (5–10%) with the intracavity phase diffuser, and the output power is reduced by merely 15% over a wide range of pump levels. This work provides a simple and robust method for ultrafast speckle suppression.
2 Degenerate cavity laser configurations
Figure 1 schematically presents several different DCL configurations (details are given in Section 5.1). Figure 1A shows the basic DCL in a self-imaging condition [22]. It comprises of a high-reflectivity flat back mirror, a Nd:YAG gain medium optically pumped by a flash lamp, two spherical lenses of focal lengths f in a 4f telescope configuration and an output coupler. We calculate the transverse mode structure (see Section 5.2 for details) and plot the histogram of the frequency differences between the nth order transverse mode ωn and the fundamental mode ω0. The difference ωn − ω0 is normalized by the free spectral range (FSR = Δωl), which is the frequency spacing of longitudinal mode groups. The results shown in the center panel indicate that all the transverse modes in a perfect DCL are exactly degenerate in frequency. The quality factor as a function of the transverse mode index in the right panel exhibits a uniform distribution of high quality factors, indicating that all the transverse modes have an exactly identical (degenerate) quality factor. In this ideal case, despite the fact that many transverse modes are expected to lase, the spectral degeneracy slows down the spatial decoherence. Only when the photodetection integration time exceeds the coherence time given by the inverse of spectral linewidth of individual lasing modes, the degenerate modes become mutually incoherent and the speckle contrast decreases. Note that in practice such an ideal DCL cannot be realized due to the presence of misalignment errors, thermal effects and optical aberrations [24]. Therefore, the transverse lasing modes have slightly different frequencies, which in turn shorten the time of decoherence [22].
In order to accelerate the spatial decoherence, the frequency spacing of the transverse modes has to be increased. Namely, the frequency degeneracy of the modes has to be broken. A conventional method for breaking the frequency degeneracy is detuning the cavity, e.g., translating the output coupler in the longitudinal (z) axis of the cavity, as shown in the configuration of Figure 1B. With a sufficient longitudinal displacement
In order to break the frequency degeneracy and increase the frequency spacings of the transverse modes, while minimizing their quality factor degradation, we explore a different approach, where we insert a static intracavity phase diffuser into the DCL, as shown in Figure 1C. The phase diffuser is placed next to the output coupler in order to maintain the self-imaging condition of the cavity. More details are given in Section 5.1. The intracavity phase diffuser is a computer-generated random phase plate made of glass. It introduces an optical phase delay that varies randomly from −π to π on a length scale of ≈200 μm (see Section 5.1). The center panel of Figure 1C shows that the transverse modes are spread over the entire FSR of the DCL, increasing the frequency spacings between them. In contrary to the misaligned cavity case, many transverse modes experience minor quality factor degradation. As a result, a large number of transverse modes are expected to lase over a wide spectrum of frequencies, accelerating the speckle suppression process.
3 Ultrafast speckle suppression
To demonstrate the efficiency of our method, we experimentally measure the speckle contrast for integration times in the range of 10−10 to 10−4 s. The output beam of the DCL is incident onto a thin diffuser placed outside the laser cavity. Then, the speckle intensity is measured by an InGaAs photodiode of 15 GHz bandwidth and an oscilloscope of 4 GHz bandwidth. See Section 5.1 for a detailed description of the experimental setup and the measurement scheme. Figure 2A shows the measured speckle contrast as a function of the photodetector’s integration time without and with an intracavity phase diffuser, at the pump power of three times the lasing threshold. By measuring the speckle contrast over many time windows of an equal length, we compute the mean contrast value and estimate the uncertainty that is shown by the shaded area. The lasing pulse is ∼100 μs long. To avoid the transient oscillations at the beginning of the lasing pulse, we analyze the emission after the laser reaches a quasi steady state. For the effects of lasing transients, see Supplementary material S1. Experimental data with a lower pump power are also presented in Supplementary material S2.
With the intracavity phase diffuser, the speckle contrast at short integration times (between 10−10 and 10−7 s) is significantly lower than that without the intracavity phase diffuser. Even when the integration time is as short as 10−9 s, the speckle contrast is already reduced to 3%. To understand this remarkable result, we numerically calculate the field evolution in a passive cavity with a simplified (1+1)D model. Nonlinear interactions of the lasing modes through the gain medium are neglected (see Section 5.2 for details about the numerical model). The calculated speckle contrast is plotted as a function of integration time τ in Figure 2B. When τ is shorter than the inverse of the emission spectrum width
Once
With an intracavity phase diffuser in the DCL, the gap between
To verify this explanation, we compare the power spectrum of emission intensity of the DCL with the intracavity phase diffuser to that without it. The power spectrum is obtained by Fourier transforming the time intensity signal of the emission. Figure 3 shows the measured and simulated power spectra, which reflect the frequency beating of the lasing modes. Without the intracavity phase diffuser (top row), the power spectrum features narrow distributions peaked at the harmonics of FSR = c/(2L) ≈ 128 MHz, where c is the speed of light, and L = 117 cm is the total optical length of the DCL. The narrow distributions centered at the harmonics of the FSR reveal a slight breaking of frequency degeneracy of the transverse modes, due to the inherent imperfections of the cavity. With the intracavity phase diffuser (bottom row), the power spectrum of emission intensity features many narrow peaks in between the harmonics of the FSR. As the transverse modes move further away from the frequency degeneracy, their frequency differences, which determine their beat frequencies, increase. Nevertheless, the longitudinal mode spacing is unchanged; thus, the peaks at the harmonics of the FSR remain in the power spectrum but appear narrower than that without the intracavity phase diffuser. The changes in the power spectrum indicate a frequency broadening of spatiotemporal modes by the intracavity phase diffuser. An ensemble of mutually incoherent lasing modes separated by frequency spacings in the range of ∼1 to ∼128 MHz leads to a faster decoherence rate on the time scale of ∼10−8 to ∼10−6 s. This observation is consistent with the behavior shown in Figure 2.
Surprisingly, the intracavity phase diffuser causes a significant speckle contrast reduction even when the integration time is shorter than 10−8 s, as seen in Figure 2A. Note that this behavior is not captured in the simulation (Figure 2B, green curve). To explain this effect, we analyze the entire experimentally measured power spectra [25]. The results are presented in Figure 4 both (A) without and (B) with the phase diffuser in the DCL.
Without the intracavity phase diffuser, the power spectrum envelope decays with increasing frequency. With the intracavity phase diffuser, the power spectrum exhibits an essentially constant envelope over the entire power detection range of 5 GHz. This difference indicates that the intracavity phase diffuser facilitates lasing in a broader frequency range. With the intracavity phase diffuser, the mutually incoherent lasing modes of frequency spacing well above 1 GHz accelerate the speckle reduction in the subnanosecond time scale. Due to the large number of lasing modes in the DCL, it is extremely difficult to simulate their nonlinear interactions with the gain material. Our numerical model does not account for spatial hole burning and mode competition for gain and thus cannot predict the lasing spectrum broadening induced by the intracavity diffuser. Therefore, the difference between the experimental and the numerical results in the ultrashort time regime is attributed to the absence of nonlinear lasing dynamics in the numerical model. Namely, the intracavity phase diffuser reduces mode competition for gain, allowing modes with wider frequency differences to lase simultaneously.
To complete this observation, we incorporate the diffuser-induced broadening of the lasing spectrum into the numerical model and calculate the spectral contrast as shown by the red curve in Figure 2B. Lasing with more longitudinal modal groups results in a more significant reduction of the speckle contrast at short integration times, in agreement to the experimental data in Figure 2A. This agreement confirms two distinct mechanisms for speckle contrast reduction by the intracavity diffuser. One is the increase of frequency spacing of the transverse modes within each longitudinal modal group, and the other is the broadening of the entire lasing spectrum and an increase in the total number of longitudinal modal groups that can lase. The former mechanism results in speckle reduction in the integration time range of 10−8 to 10−6 s, while the latter is responsible for speckle reduction in the range of 10−10 to 10−8 s.
Finally, we measure the total output power of the DCL without and with the intracavity phase diffuser. The lasing threshold is increased by 5−10% after the diffuser is inserted into the DCL. As shown in Section 5.4, the output power is reduced by about 15% over a wide range of pump levels from 1.2 times to 3.3 times the lasing threshold power.
4 Conclusion
In conclusion, we accelerate the spatial decoherence of a degenerate cavity laser (DCL) with an intracavity phase diffuser. In less than 1 ns, the speckle contrast is already reduced to 3%, below the human perception level. Such a light source, together with a time-gated camera, can be used for time-resolved full-field imaging of transient phenomena such as the dynamics of material processing [10] and tracking of moving targets [11], [22]. Our approach is general and will work more efficiently in terms of speckle reduction for compact multimode lasers that have a smaller number of lasing modes and a higher speckle contrast than our DCL. We plan to extend this work by further investigating how the intracavity phase diffuser modifies the nonlinear modal interactions and the spatiotemporal dynamics of a DCL [26].
5 Methods
5.1 Detailed experimental setup
Our experimental setup, shown in Figure 5, consists of two parts: (i) a DCL with a static intracavity phase diffuser and (ii) an imaging system to generate speckle with an external diffuser and to measure speckle contrast [11]. The DCL comprises a flat back mirror with 95% reflectivity, a Nd:YAG crystal rod of 10.9 cm length and 0.95 cm diameter, two spherical lenses of 5.08 cm diameter and f = 25 cm focal length and an output coupler with 80% reflectivity. Adjacent to the output coupler, the phase diffuser is placed inside the cavity. Lasing occurs at the wavelength of 1064 nm with optical pumping. The output beam is focused by a lens with a diameter of 2.54 cm and a focal length of f2 = 6 cm onto a thin diffuser with a 10° angular spread of the transmitted light. A photodetector with a 15 GHz bandwidth and 30 μm diameter is placed at a distance of 10 cm from the diffuser and records the scattered light intensity within a single speckle grain in time. We rotate the diffuser and repeat the time intensity trace measurement of a different speckle grain. In total, 100 time intensity traces are recorded.
The intracavity phase diffuser (Figure 5B) is a computer-generated surface relief random phase plate of diameter 5.08 cm and thickness 2.3 mm. The angular spread of the transmitted light is
In the time-resolved speckle measurement, we use an InGaAs photodiode with 15 GHz bandwidth (Electro-Optics ET-3500). It is connected via a radiofrequency coaxial cable to a Keysight DSO9404A oscilloscope of 4 GHz bandwidth and up to 20 GS/s sampling rate (giga sample per second). The effective bandwidth of our detection system is thus limited to 4 GHz by the oscilloscope.
5.2 Numerical simulation
We simulate continuous wave propagation in a passive degenerate cavity with and without the intracavity phase diffuser. The cavity length and width are identical to those of the DCL in our experiment, except that the cross section is one dimensional in order to shorten the computation time. Without the intracavity phase diffuser, the field evolution matrix of a single round trip in the cavity is given as follows:
where MF is the field propagation matrix from the back mirror to the output coupler and MB from the output coupler to the back mirror and Mϵ represents a small axial misalignment of the DCL [24]. With the intracavity phase diffuser placed next to the output coupler, the field evolution matrix of a single round trip becomes:
where MPD represents the phase delay of the field induced by the phase diffuser for one round trip in the cavity. To construct MPD in our simulations, we use the spatial distribution of the phase delay taken from the measured profile in Figure 5B.
The matrices Mwo and Mw are diagonalized to obtain the eigenmodes of the cavity without and with the intracavity phase diffuser. A subset of the eigenmodes has high quality factors (low losses). Hence, they have low lasing threshold and correspond to the lasing modes. The total field in the cavity can be expressed as a sum of these modes:
where αm,n and ωm,n denote the amplitude and frequency of a mode, respectively, with a longitudinal index m and a transverse index n and ψn(x) represents the transverse field profile for the nth eigenmode. The phase ϕm,n(t) fluctuates randomly in time to simulate the spontaneous emission–induced phase diffusion that leads to spectral broadening [27]. The total number of transverse modes is N, and the number of longitudinal modes is 2M.
The optical gain spectrum is approximated as a Lorentzian function centered at
To generate an intensity speckle, we simulate the field propagation from the output coupler of the degenerate cavity to the external diffuser and then from the diffuser to the far field. The field intensity at the far field is used to compute the speckle contrast as a function of the integration time (see Methods 5.3).
5.3 Measurement of speckle contrast
We use the experimental setup in Figure 5A to measure the time-resolved intensity of a single speckle grain behind a diffuser that is placed outside of the DCL. Using the detection device, we record the intensity as a function of time with and without the phase diffuser inside the DCL. The time trace of the intensity is recorded at 100 spatial locations
where
5.4 Total output power of the DCL configurations
We experimentally measure the total output power of the DCL without and with the intracavity phase diffuser. As shown in Figure 6A, the total output power with the intracavity phase diffuser is slightly lower than that without it. In Figure 6B, we plot their ratio, which is about 0.85 for all the pump levels. Thus, the intracavity phase diffuser causes a power reduction of about
Funding source: US Air Force Office of Scientific Research
Award Identifier / Grant number: FA 9550-20-1-0129
Funding source: US-Israel Binational Science Foundation (BSF)
Award Identifier / Grant number: 2015509
Acknowledgments
The authors thank Arnaud Courvoisier and Ronen Chriki for their advice and help in the measurements. This work is partially funded by the US-Israel Binational Science Foundation (BSF) under grant no. 2015509. The work performed at Yale is supported partly by the US Air Force Office of Scientific Research under Grant No. FA 9550-20-1-0129, and the authors acknowledge the computational resources provided by the Yale High Performance Computing Cluster (Yale HPC). The research done at Weizmann is supported by the Israel Science Foundation.
Author contribution: All the authors have accepted responsibility for the entire content of this submitted manuscript and approved submission.
Research funding: This work is partially funded by the US-Israel Binational Science Foundation (BSF) under grant no. 2015509. The work performed at Yale is supported partly by the US Air Force Office of Scientific Research under Grant No. FA 9550-20-1-0129.
Conflict of interest statement: The authors declare no conflicts of interest regarding this article.
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Supplementary Material
The online version of this article offers supplementary material (https://doi.org/10.1515/nanoph-2020-0390).
© 2020 Simon Mahler et al., published by De Gruyter, Berlin/Boston
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