Abstract
Anthropogenic emissions of greenhouse gases into the atmosphere is inducing global warming, ocean acidification, polar ice melting, rise in sea level, droughts and hurricanes, thus threatening human health and the global economy. Therefore, there is a need to develop cost-effective technologies for CO2 capture. For instance, solution absorption is promising due to a large processing capacity, high flexibility and reliability, and rich experience in engineering applications. Nonetheless, actual commercial solutions, solvents and processes for CO2 capture suffer from slow reaction kinetics, low absorption capacity, high-energy consumption, susceptibility to corrosion, toxicity, low stability and high costs. Therefore, current research focuses on developing more economical, effective, green and sustainable technologies. Here we review 2015–2020 findings on CO2 capture using liquid absorption methods. Methods are based on various solutions, solvents and processes such as carbonate solution, ammonia solution, amine-based solution, ionic liquid, amino acid salt, phase changing absorbent, microcapsulated and membrane absorption, nanofluids and phenoxide salt solution. We discuss absorption performance, absorption mechanism, enhancement pathways and challenges. Amine- and NH3-based absorbents are widely used, yet they are limited by high regeneration energy, corrosiveness and degradation, reagent loss and secondary pollution caused by NH3 escape. Phase changing absorbents are getting more attention due to their lower cost and lower energy penalty. The incorporation of membrane and microencapsulation technologies to absorbing solvents could enhance CO2 absorption performance by reducing corrosion and increasing selectivity. Adding nanoparticles to solvents could improve CO2 absorption performance and reduce energy requirement. Besides, solvent blends and promoter-improved solvents performed better than single and non-promoted solvents because they combine the benefits of individual solvents and promoters.
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Abbreviations
- CCS:
-
Carbon capture and storage
- [Cho][Pro]:
-
(2-Hydroxyethyl)-trimethyl-ammonium (S)-2-pyrrolidine-carboxylic acid salt
- CO2 :
-
Carbon dioxide
- HER:
-
Hydrogen evolution reaction
- K2CO3 :
-
Potassium carbonate
- MWCNTs:
-
Multi-walled carbon nanotubes
- N2O:
-
Nitrous oxide
- OH groups:
-
Hydroxyl (–) groups
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This study was supported by the National Natural Science Foundation of China (Nos. U1710108; 51576094).
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Ochedi, F.O., Yu, J., Yu, H. et al. Carbon dioxide capture using liquid absorption methods: a review. Environ Chem Lett 19, 77–109 (2021). https://doi.org/10.1007/s10311-020-01093-8
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DOI: https://doi.org/10.1007/s10311-020-01093-8