Abstract
Polyimide membranes and network hybrid membranes exhibit high permeability despite good thermal and chemical stability, and high selectivity in gas mixture separation. In this study, the effect of nanoparticle distribution on the network polymer network, and changes in permeability, selectivity, and structure of the composite lattice membrane are investigated. According to the obtained permeability results, this increase in permeability was due to the increase of polymer network free volume and the formation of cavities in the nanoparticle-polymer interface. The significant results were that the permeability growth of gases with larger molecular size such as methane and nitrogen was higher than other gases. A comparison of the permeability growth of gases with the increasing volume fraction of nanoparticles confirms the dominance of the molecular sieve mechanism and the type of membrane transport mechanism change over polyimide and network Hybrid.
Funding source: National Natural Science Foundation of China
Award Identifier / Grant number: 21706169
Award Identifier / Grant number: 51603225
Funding source: Natural Science Foundation of Shanxi Province
Award Identifier / Grant number: 201701D221067
Award Identifier / Grant number: 201801D121083
Funding source: Doctoral Scientific Research Foundation of Taiyuan University of Science and Technology
Award Identifier / Grant number: 20162020
Acknowledgments
National Natural Science Foundation of China (Grant No.21706169). Natural Science Foundation of Shanxi Province(Grant No.201701D221067). Doctoral Scientific Research Foundation of Taiyuan University of Science and Technology (Grant No. 20162020), National Natural Science Foundation of China (Grant No. 51603225) Natural Science Foundation of Shanxi Province (Grant No. 201801D121083). The authors gratefully a Department of Chemical Engineering, Arak Branch, Islamic Azad University, Arak, Iran and Young Researchers and Elite Club, Gachsaran Branch, Islamic Azad University, Gachsaran
Author contribution: All the authors have accepted responsibility for the entire content of this submitted manuscript and approved submission.
Research funding: The study was funded by National Natural Science Foundation of China (Grant No. 21706169); Natural Science Foundation of Shanxi Province (Grant No. 201701D221067); Doctoral Scientific Research Foundation of Taiyuan University of Science and Technology (Grant No. 20162020); National Natural Science Foundation of China (Grant No. 51603225). Natural Science Foundation of Shanxi Province(Grant No. 201801D121083). The authors gratefully a Department of Chemical Engineering, Arak Branch, Islamic Azad University, Arak, Iran and Young Researchers and Elite Club, Gachsaran Branch, Islamic Azad University, Gachsaran.
Conflict of interest statement: The authors declare no conflicts of interest regarding this article.
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