Abstract
A multi-dimensional, compressible fluid flow solver, valid in both channel and porous media, is derived by volume-averaging the Navier–Stokes equations. By selecting an appropriate average density/velocity pair, a continuous, stable solution is obtained for both pressure and velocity. The proposed model is validated by studying the pressure drop of two commonly used experimental setups to measure in-plane and through-plane permeability of fuel cell porous media. Numerical results show that the developed model is able to reproduce the experimentally measured pressure drop at varying flow rates. Further, it highlights that previously used methods of extracting permeability, which rely on the use of simplified one-dimensional models, are not appropriate when high flow rates are used to study the porous media. At high flow rates, channel–porous media interactions cannot be neglected and can result in incorrect permeability estimations. For example, at flow rates of 1 SLPM a discrepancy of 12% in pressure drop was observed when using previous permeability values instead of the values obtained in the article using the proposed 3D model. Given that at high flow rate one-dimensional models might not be appropriate, previous estimations of Forchheimer permeability might not be accurate. To illustrate the suitability of the numerical model to fuel cell applications, fluid flow bypass in serpentine and interdigitated fuel cell flow channels is also investigated.
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Amestoy, P., Duff, I., L’Excellent, J.: MUMPS multifrontal massively parallel solver version 2.0 (1998)
Auriault, J.: On the domain of validity of Brinkman’s equation. Transp. Porous Media 79(2), 215–223 (2009)
Badea, L., Discacciati, M., Quarteroni, A.: Numerical analysis of the Navier–Stokes/Darcy coupling. Numer. Math. 115(2), 195–227 (2010)
Bangerth, W., Hartmann, R., Kanschat, G.: deal.II—a general-purpose object-oriented finite element library. ACM Trans. Math. Softw. (TOMS) 33(4), 24 (2007)
Beavers, G., Joseph, D.: Boundary conditions at a naturally permeable wall. J. Fluid Mech. 30(1), 197–207 (1967)
Bernardi, C., Rebollo, T., Hecht, F., Mghazli, Z.: Mortar finite element discretization of a model coupling Darcy and Stokes equations. ESAIM: Math. Modell. Numer. Anal. 42(3), 375–410 (2008)
Burman, E., Hansbo, P.: A unified stabilized method for Stokes’ and Darcy’s equations. J. Comput. Appl. Math. 198(1), 35–51 (2007)
Carrigy, N., Pant, L., Mitra, S., Secanell, M.: Knudsen diffusivity and permeability of PEMFC microporous coated gas diffusion layers for different polytetrafluoroethylene loadings. J. Electrochem. Soc. 160(2), F81–F89 (2013)
Chidyagwai, P., Rivière, B.: On the solution of the coupled Navier–Stokes and Darcy equations. Comput. Methods Appl. Mech. Eng. 198(47–48), 3806–3820 (2009)
Cremonesi, M., Meduri, S., Perego, U.: Lagrangian–Eulerian enforcement of non-homogeneous boundary conditions in the Particle Finite Element Method. Comput. Part. Mech. 7(1), 41–56 (2020)
Darcy, H.: Recherches expérimentales relatives au mouvement de l’eau dans les tuyaux, vol. 1. Impr, Impériale (1857)
Davis, T.: Algorithm 832: Umfpack v4. 3—an unsymmetric-pattern multifrontal method. ACM Trans. Math. Softw. (TOMS) 30(2), 196–199 (2004)
Discacciati, M., Quarteroni, A.: Navier–Stokes/Darcy coupling: modeling, analysis, and numerical approximation. Rev. Mat. Complut. 22(2), 315–426 (2009)
Dobberschütz, S.: Effective behavior of a free fluid in contact with a flow in a curved porous medium. SIAM J. Appl. Math. 75(3), 953–977 (2015)
Donea, J., Huerta, A.: Finite Element Methods for Flow Problems, 1st edn. Wiley, New York (2003)
El-Jarroudi, M., Er-Riani, M.: Homogenization of a two-phase incompressible fluid in crossflow filtration through a porous medium. Math. Methods Appl. Sci. 41(1), 281–302 (2018)
Erturk, E., Corke, T., Gökçöl, C.: Numerical solutions of 2-D steady incompressible driven cavity flow at high Reynolds numbers. Int. J. Numer. Methods Fluids 48(7), 747–774 (2005)
Feser, J., Prasad, A., Advani, S.: Experimental characterization of in-plane permeability of gas diffusion layers. J. Power Sources 162(2), 1226–1231 (2006)
Forchheimer, P.: Wasserbewegung durch boden. Z. Ver. dtsch. Ing. 45, 1782–1788 (1901)
Gebart, B.: Permeability of unidirectional reinforcements for RTM. J. Compos. Mater. 26(8), 1100–1133 (1992)
Ghia, U., Ghia, K., Shin, C.: High-Re solutions for incompressible flow using the Navier–Stokes equations and a multigrid method. J. Comput. Phys. 48(3), 387–411 (1982)
Gostick, J., Fowler, M., Pritzker, M., Ioannidis, M., Behra, L.: In-plane and through-plane gas permeability of carbon fiber electrode backing layers. J. Power Sources 162(1), 228–238 (2006)
Gray, W., Lee, P.: On the theorems for local volume averaging of multiphase systems. Int. J. Multiph. Flow 3(4), 333–340 (1977)
Gresho, P., Sani, R.: Incompressible Flow and the Finite Element Method. Volume 1: Advection–Diffusion and Isothermal Laminar Flow. Wiley, New York (1998)
Gurau, V., Bluemle, M., Castro, E.D., Tsou Jr., Y., Zawodzinski Jr., T., Mann Jr., J.A.: Characterization of transport properties in gas diffusion layers for proton exchange membrane fuel cells: 2. absolute permeability. J. Power Sources 165(2), 793–802 (2007)
Hashemi, F., Rowshanzamir, S., Rezakazemi, M.: CFD simulation of PEM fuel cell performance: effect of straight and serpentine flow fields. Math. Comput. Modell. 55(3–4), 1540–1557 (2012)
Hendrick, A., Erdmann, R., Goodman, M.: Practical considerations for selection of representative elementary volumes for fluid permeability in fibrous porous media. Transp. Porous Media 95(2), 389–405 (2012)
Howes, F., Whitaker, S.: The spatial averaging theorem revisited. Chem. Eng. Sci. 40(8), 1387–1392 (1985)
Hsu, C., Cheng, P.: Thermal dispersion in a porous medium. Int. J. Heat Mass Transf. 33(8), 1587–1597 (1990)
Hussaini, I., Wang, C.: Measurement of relative permeability of fuel cell diffusion media. J. Power Sources 195(12), 3830–3840 (2010)
Ismail, M., Damjanovic, T., Hughes, K., Ingham, D., Ma, L., Pourkashanian, M., Rosli, M.: Through-plane permeability for untreated and PTFE-treated gas diffusion layers in proton exchange membrane fuel cells. J. Fuel Cell Sci. Technol. 7(5), 051016 (2009)
Ismail, M., Damjanovic, T., Ingham, D., Ma, L., Pourkashanian, M.: Effect of polytetrafluoroethylene-treatment and microporous layer-coating on the in-plane permeability of gas diffusion layers used in proton exchange membrane fuel cells. J. Power Sources 195(19), 6619–6628 (2010)
Ismail, M., Borman, D., Damjanovic, T., Ingham, D., Pourkashanian, M.: On the through-plane permeability of microporous layer-coated gas diffusion layers used in proton exchange membrane fuel cells. Int. J. Hydrog. energy 36(16), 10392–10402 (2011)
Jian, Q., Ma, G., Qiu, X.: Influences of gas relative humidity on the temperature of membrane in PEMFC with interdigitated flow field. Renew. Energy 62, 129–136 (2014)
Levy, T., Sanchez-Palencia, E.: On boundary conditions for fluid flow in porous media. Int. J. Eng. Sci. 13(11), 923–940 (1975)
Li, S., Sundén, B.: Effects of gas diffusion layer deformation on the transport phenomena and performance of PEM fuel cells with interdigitated flow fields. Int. J. Hydrog. Energy 43(33), 16279–16292 (2018)
Liu, S., Masliyah, J.: Single fluid flow in porous media. Chem. Eng. Commun. 148(1), 653–732 (1996)
Mahmoudi, A., Ramiar, A., Esmaili, Q.: Effect of inhomogeneous compression of gas diffusion layer on the performance of PEMFC with interdigitated flow field. Energy Convers. Manag. 110, 78–89 (2016)
Mangal, P., Dumontier, M., Carrigy, N., Secanell, M.: Measurements of permeability and effective in-plane gas diffusivity of gas diffusion media under compression. ECS Trans. 64(3), 487–499 (2014)
Mangal, P., Pant, L., Carrigy, N., Dumontier, M., Zingan, V., Mitra, S., Secanell, M.: Experimental study of mass transport in PEMFCs: through plane permeability and molecular diffusivity in GDLs. Electrochim. Acta 167, 160–171 (2015)
Nguyen, P., Berning, T., Djilali, N.: Computational model of a PEM fuel cell with serpentine gas flow channels. J. Power Sources 130(1–2), 149–157 (2004)
Orogbemi, O., Ingham, D., Ismail, M., Hughes, K., Ma, L., Pourkashanian, M.: Through-plane gas permeability of gas diffusion layers and microporous layer: effects of carbon loading and sintering. J. Energy Inst. 91(2), 270–278 (2018)
Pant, L., Mitra, S., Secanell, M.: Absolute permeability and Knudsen diffusivity measurements in PEMFC gas diffusion layers and micro porous layers. J. Power Sources 206, 153–160 (2012)
Park, J., Li, X.: An experimental and numerical investigation on the cross flow through gas diffusion layer in a PEM fuel cell with a serpentine flow channel. J. Power Sources 163(2), 853–863 (2007)
Park, J., Li, X.: An analytical analysis on the cross flow in a PEM fuel cell with serpentine flow channel. Int. J. Energy Res. 35(7), 583–593 (2011)
Pharoah, J.: On the permeability of gas diffusion media used in PEM fuel cells. J. Power Sources 144(1), 77–82 (2005)
Qin, Y., Liu, G., Chang, Y., Du, Q.: Modeling and design of PEM fuel cell stack based on a flow network method. Appl. Therm. Eng. 144, 411–423 (2018)
Rajagopal, K.: On a hierarchy of approximate models for flows of incompressible fluids through porous solids. Math. Models Methods Appl. Sci. 17(02), 215–252 (2007)
Saffman, P.: On the boundary condition at the surface of a porous medium. Stud. Appl. Math. 50(2), 93–101 (1971)
Saha, L., Oshima, N.: Prediction of flow crossover in the GDL of PEFC using serpentine flow channel. J. Mech. Sci. Technol. 26(5), 1315–1320 (2012)
Saha, S., Kurihara, E., Shi, W., Oshima, N.: Numerical study of pressure drop in the separator channel and gas diffusion layer of polymer electrolyte fuel cell and deformation effect of porous media. In: ASME 2008 6th International Conference on Nanochannels, Microchannels, and Minichannels, American Society of Mechanical Engineers, pp. 1317–1325 (2008)
Salahuddin, K., Oshima, N.: Numerical investigation of cross flow on the performance of polymer electrolyte fuel cell. J. Therm. Sci. Technol. 8(3), 586–602 (2013). https://doi.org/10.1299/jtst.8.586
Salahuddin, K., Nishimura, A., Oshima, N., Saha, L.: Numerical study of pressure drop mechanism and cross flow behavior in the gas channel and porous medium of a polymer electrolyte membrane fuel cell. J. Therm. Sci. Technol. 8(1), 209–224 (2013)
Santamaria, A., Cooper, N., Becton, M., Park, J.: Effect of channel length on interdigitated flow-field PEMFC performance: a computational and experimental study. Int. J. Hydrog. Energy 38(36), 16253–16263 (2013)
Secanell, M., Putz, A., Wardlaw, P., Zingan, V., Bhaiya, M., Moore, M., Zhou, J., Balen, C., Domican, K.: OpenFCST: an open-source mathematical modelling software for polymer electrolyte fuel cells. ECS Trans. 64(3), 655–680 (2014)
Srinivasan, S., Rajagopal, K.: A thermodynamic basis for the derivation of the Darcy, Forchheimer and Brinkman models for flows through porous media and their generalizations. Int. J. Non-Linear Mech. 58, 162–166 (2014)
Sun, L., Oosthuizen, P., McAuley, K.: A numerical study of channel-to-channel flow cross-over through the gas diffusion layer in a PEM-fuel-cell flow system using a serpentine channel with a trapezoidal cross-sectional shape. Int. J. Therm. Sci. 45(10), 1021–1026 (2006)
Tamayol, A., McGregor, F., Bahrami, M.: Single phase through-plane permeability of carbon paper gas diffusion layers. J. Power Sources 204, 94–99 (2012)
Urquiza, J., N’dri, D., Garon, A., Delfour, M.: Coupling stokes and darcy equations. Appl. Numer. Math. 58(5), 525–538 (2008)
Vafai, K., Tien, C.: Boundary and inertia effects on flow and heat transfer in porous media. Int. J. Heat Mass Transf. 24(2), 195–203 (1981)
Whitaker, S.: Advances in theory of fluid motion in porous media. Ind. Eng. Chem. 61(12), 14–28 (1969)
Whitaker, S.: The forchheimer equation: a theoretical development. Transp. Porous Media 25(1), 27–61 (1996)
Whitaker, S.: The Method of Volume Averaging, vol. 13. Springer, Berlin (1999)
Xu, H.: Experimental measurement of mass transport parameters of gas diffusion layer and catalyst layer in PEM fuel cell. Master’s thesis, University of Alberta (2019)
Yu, L., Ren, G., Qin, M., Jiang, X.: Transport mechanisms and performance simulations of a PEM fuel cell with interdigitated flow field. Renew. Energy 34(3), 530–543 (2009)
Zhang, S., Reimer, U., Beale, S., Lehnert, W., Stolten, D.: Modeling polymer electrolyte fuel cells: a high precision analysis. Appl. Energy 233, 1094–1103 (2019a)
Zhang, X., Zhang, X., Taira, H., Liu, H.: Error of Darcy’s law for serpentine flow fields: dimensional analysis. J. Power Sources 412, 391–397 (2019b)
Acknowledgements
The authors would also like to thank the Natural Sciences and Engineering Research Council of Canada (NSERC), the Automotive Fuel Cell Cooperation (AFCC) Corp., and International Cooling Towers (ICT) for their financial support.
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Appendix: Lid-Driven Cavity Flow Test Case
Appendix: Lid-Driven Cavity Flow Test Case
A standard benchmark problem for testing Navier–Stokes equations is the lid-driven cavity flow problem (Donea and Huerta 2003; Cremonesi et al. 2020), which consists in the flow of an isothermal fluid in a square cavity, as shown in Fig. 19. The fluid contained inside the cavity is set into motion by the top wall which is sliding at constant velocity from left to right, while the other sides are fixed.
The steady-state compressible numerical solution is computed at Re = 1000 on a \(128 \times 128\) grid by using \(Q_1\) and \(Q_2\) approximations for density and velocity, respectively. The tolerance of the Newton method is set to \(10^{-10}\). The fluid flow patterns generated in this computation are shown in Fig. 20a, b. The streamlines depicted in Fig. 20a show the formation of three vortexes, which have been already observed in previous numerical studies Donea and Huerta (2003), Ghia et al. (1982), Erturk et al. (2005), Cremonesi et al. (2020).
The numerical results are compared to those previously obtained by Ghia et al. (1982). Figure 21 shows the variation of the horizontal and vertical velocity components along the vertical and horizontal centerlines (i.e., \(y/L = 0.5\) and \(x/L = 0.5\)), respectively. The computational results obtained by the present model are in very good agreement with the available numerical data.
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Jarauta, A., Zingan, V., Minev, P. et al. A Compressible Fluid Flow Model Coupling Channel and Porous Media Flows and Its Application to Fuel Cell Materials. Transp Porous Med 134, 351–386 (2020). https://doi.org/10.1007/s11242-020-01449-2
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DOI: https://doi.org/10.1007/s11242-020-01449-2