Quantum Persistent Tennis Racket Dynamics of Nanorotors

Yue Ma, Kiran E. Khosla, Benjamin A. Stickler, and M. S. Kim
Phys. Rev. Lett. 125, 053604 – Published 31 July 2020
PDFHTMLExport Citation

Abstract

Classical rotations of asymmetric rigid bodies are unstable around the axis of intermediate moment of inertia, causing a flipping of rotor orientation. This effect, known as the tennis racket effect, quickly averages to zero in classical ensembles since the flipping period varies significantly upon approaching the separatrix. Here, we explore the quantum rotations of rapidly spinning thermal asymmetric nanorotors and show that classically forbidden tunneling gives rise to persistent tennis racket dynamics, in stark contrast to the classical expectation. We characterize this effect, demonstrating that quantum coherent flipping dynamics can persist even in the regime where millions of angular momentum states are occupied. This persistent flipping offers a promising route for observing and exploiting quantum effects in rotational degrees of freedom for molecules and nanoparticles.

  • Figure
  • Figure
  • Received 31 March 2020
  • Accepted 13 July 2020

DOI:https://doi.org/10.1103/PhysRevLett.125.053604

© 2020 American Physical Society

Physics Subject Headings (PhySH)

Atomic, Molecular & OpticalGeneral Physics

Authors & Affiliations

Yue Ma1, Kiran E. Khosla1, Benjamin A. Stickler1,2,*, and M. S. Kim1,†

  • 1QOLS, Blackett Laboratory, Imperial College London, London SW7 2AZ, United Kingdom
  • 2Faculty of Physics, University of Duisburg-Essen, 47048 Duisburg, Germany

  • *b.stickler@imperial.ac.uk
  • m.kim@imperial.ac.uk

Article Text (Subscription Required)

Click to Expand

Supplemental Material (Subscription Required)

Click to Expand

References (Subscription Required)

Click to Expand
Issue

Vol. 125, Iss. 5 — 31 July 2020

Reuse & Permissions
Access Options
Author publication services for translation and copyediting assistance advertisement

Authorization Required


×
×

Images

×

Sign up to receive regular email alerts from Physical Review Letters

Log In

Cancel
×

Search


Article Lookup

Paste a citation or DOI

Enter a citation
×