Abstract
Magneto-optical materials have become a key tool in functional nanophotonics, mainly due to their ability to offer active tuning between two different operational states in subwavelength structures. In the long-wavelength limit, such states may be considered as the directional forward- and back-scattering operations, due to the interplay between magnetic and electric dipolar modes, which act as equivalent Huygens sources. In this work, on the basis of full-wave electrodynamic calculations based on a rigorous volume integral equation (VIE) method, we demonstrate the feasibility of obtaining magnetically-tunable directionality inversion in spherical microresonators (THz antennas) coated by magneto-optical materials. In particular, our analysis reveals that when a high-index dielectric is coated with a magneto-optical material, we can switch the back-scattering of the whole particle to forward-scattering simply by turning off/on an external magnetic field bias. The validity of our calculations is confirmed by reproducing the above two-state operation, predicted by the VIE, with full-wave finite-element commercial software. Our results are of interest for the design of state-of-the-art active metasurfaces and metalenses, as well as for functional nanophotonic structures, and scattering and nanoantennas engineering.
1 Introduction
Following an increasing need for the deployment of active (tunable) photonic materials during recent years, magneto-optical-aided dielectric resonators have emerged as a valuable platform because of their unique and energy-efficient ability to control the propagation of optical waves. This is achieved through an external agent, mainly an external magnetic field, which alters the constitutive parameters of the magneto-optical material. Multi-fold enhancement of magneto-optical effects in Si nanodisks covered with thin nickel films, as well as in magneto-photonic array of nanodisks, has been experimentally demonstrated, for the development of active and nonreciprocal photonic nanostructures [1]. Magneto-optical materials have been successfully employed in cylindrical structures, such as infinite cylinders or arrays of such. In particular, their use was recently achieved in the context of active scattering, via the available Mie theory for infinite, two-dimensional circular gyroelectric/gyromagnetic cylinders whose solution can be separated into TE and TM modes [2]. Specifically, active control of directional scattering with a core–shell infinite cylinder driven by an external magnetic field, as well as in cylindrical reconfigurable meta-lattices, has been theoretically examined by breaking the degeneracy of the multipoles in the subwavelength regime, thereby allowing the splitted modes to interfere and lead to directional optical switching [3], [4]. In addition, a normally irradiated array of magneto-optical core–shell cylinders has resulted in tunable anomalous back-scattering, where the extinction mean free path is longer than the transport mean free path [5].
Magneto-optical effects have been studied for attaining all-optical modulation [6], by exploiting nonlinear optical effects in two-dimensional materials, including graphene which involves magneto-optical effects in its conductivity model [7], [8], in magneto-optical active plasmonic resonators [9], in the implementation of highly tunable terahertz filters with magneto-optical Bragg gratings [10], in high-index structures where a Si spherical nanoantenna encapsulates a magneto-optical garnet core giving rise to magnetic and electric resonances that dominate the long-wavelength spectrum [11], in spatially dispersive gyrotropic semiconductor spheres [12], in obtaining topologically robust ultraslow waves in the presence of absorption and scattering channels [13], in laser devices for Q-switching [14], in nickel–silicon metasurfaces [15], nickel-based nanodisk arrays [16], and in photonic crystals with magnetized epsilon-near-zero metamaterials [17] for achieving magneto-optical response enhancement. Although high-index dielectrics do not exhibit the intrinsic losses of plasmonic materials, magneto-plasmonic media may offer additional functionalities, such as e.g. tunable plasmon-driven Hall currents existing in silver-coated Bi:YIG spherical scatterers [18].
The objective of our present work is to theoretically and numerically establish the feasibility of obtaining functional directionality inversion in spherical particles in the THz regime with the aid of magneto-optical materials that obey a Drude–Lorentz dispersive model. A straightforward strategy to achieve tunable forward- and back-scattering functionality is to deposit a magneto-optical layer on top of a high-index material. In this way, the high-index core contributes the magnetic dipolar mode, while the magneto-optical shell can exhibit the necessary electric dipolar plasmon that interferes with the magnetic dipolar mode, thereby leading to the desired directionality inversion. By employing a rigorous VIE method developed for the electromagnetic scattering by highly inhomogeneous gyroelectric spheres [19], and by means of full-wave electrodynamic calculations, we demonstrate such a tunable scattering-directionality inversion.
2 Methods
The setup of the subwavelength spherical antenna that will enable active directionality inversion is depicted in Figure 1. It consists of a high-index isotropic dielectric core of radius R1 and permittivity
A general way to describe the permittivity properties of the core–shell structure is by means of the inhomogeneous cartesian permittivity tensor
where r is the radial distance in the spherical coordinate system. Therefore, Eq. (1) comprises a two-branch function with
In Eq. (2),
where
where
where
.
In Eq. (6), Re denotes the real part, the asterisk complex conjugation, while
3 Engineering functional spherical terahertz antennas for directionality inversion
The engineering of a setup for active directionality-inversion, is achievable by utilizing a magneto-optical material deposited on a high-index dielectric. Once the structure is manufactured, its geometrical parameters—i.e., radius R2 and
Figure 2A depicts the normalized scattering cross section
Figure 2B depicts the scattering-asymmetry parameter g in the same spectral window as in Figure 2A. With reference to the black curve—which corresponds to
To further proceed in the design of active tuning, in Figure 2D we plot a two-dimensional mapping of g versus
To better elucidate the optical response at the MD–LSP intersection in Figure 2C, as well as the spreading of its spectral shape where multiple peaks appear, we examine all terms that play a role in Eq. (5). Particularly, when magnetized, the sphere exhibits both uniaxial (birefringent) and gyrotropic optical response, as evident from Eq. (1) for
In Figure 2F we plot the normalized (to unity) polar/bistatic (far field) scattering cross section
Next, the effect of
Focusing on the forward-scattering operation depicted by Figure 3A–C (bottom subfigures/red curves), when the
Next we calculate the working bandwidth for our setup. For the designed device with
Up to this point, the setup is stimulated by a plane wave which impinges parallel to the orientation of the external magnetic field. In Figure 5 we examine how the switching performance is affected due to a relative orientation between
In Figure 6 we plot the near-fields and in particular the normalized magnitude
4 Scalability to the nano regime
Recently, it was experimentally demonstrated that static magnetic field-assisted resonant topological cavities, provide a platform for the implementation of photonic waveguides in the quantum regime [34]. In addition, it was theoretically and experimentally observed that graphene-based inhomogeneous strains can induce pseudomagnetic effects in the optical regime that are similar to the magnetic effects produced by the magneto-optical devices in the THz regime [35]. In particular, such effective magnetic fields can reach thousands of Tesla, exceeding standard laboratory values [36]. As a consequence, this would also increase the working bandwidth of the proposed device at the nanoscale, since the latter is linearly dependent on the magnetic field [20]. This rescaling observation led us to apply our analytical model in the THz regime, and export various intrinsic properties being scalable to shorter wavelengths.
5 Conclusion
In summary, we have shown that by judiciously designing a high-index spherical microresonator coated by an active magneto-optical material, full directionality inversion can be achieved. Based on analytical calculations and corroborating full-wave electrodynamic simulations, we have shown that by actively tuning the constitutive parameters of the magneto-optical coating by means of an external magnetic bias, tunable forward- and back-scattering functionality occurs. Our design is based on a Drude–Lorentz dispersive coating operating above its plasma frequency. The permittivity properties of the magneto-optic material change from those of an isotropic material, in the absence of magnetic field, to those of a gyroelectric one when the magnetic field is applied. Our results may allow the flexible and with low energy cost active switching of emerging metasurface and metalenses devices for applications like beam steering [37], as well as tunable nanophotonic structures such as magneto-metasurface devices for one-way transmission and sensing [38], or functional metamaterials like magneto-optical core–shell-based composed metamaterial devices for optical memory control [39].
Funding source: Hellenic Foundation for Research and Innovation (HFRI), General Secretariat for Research and Technology (GSRT)
Award Identifier / Grant number: 1819
Acknowledgement
G.P.Z., E.A., K.B., and K.L.T. were supported by the General Secretariat for Research and Technology (GSRT) and the Hellenic Foundation for Research and Innovation (HFRI) under Grant No. 1819.
Research funding: This work was supported by Hellenic Foundation for Research and Innovation (HFRI), General Secretariat for Research and Technology (GSRT) (No. 1819).
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