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Measurement of 14.54 ± 0.24 MeV neutron activation reaction cross sections of 93Nb, natMo with covariance analysis

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Abstract

The 93Nb(n,α)90mY, 93Nb(n,2n)92mNb and 92Mo(n,p)92mNb reaction cross sections have been measured relative to the 197Au(n,2n)196Au monitor reaction at the neutron energy of 14.54 ± 0.24 MeV. The neutrons were generated from the T(d,n)4He reaction using Purnima neutron generator. The experiment was done by using the method of activation in combination with an off-line \(\gamma\)-ray spectrometry technique. The uncertainties and correlations for the reaction cross sections were estimated with the use of covariance analysis by considering the partial uncertainties in individual attributes. The measured reaction cross sections have been analyzed by comparing with the data available in EXFOR compilation, various files of evaluated data and theoretically calculated values from TALYS-1.9.

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References

  1. Valentina Semkova R (2014) Measurement of neutron activation cross sections on Mo isotopes in the energy range from 7 to 15 MeV. EPJ Web Conf 66:03077

    Article  Google Scholar 

  2. Goldberg DC, Dicker G, Worcester SA (1972) Niobium and niobium alloys in nuclear power. Nucl Eng Des 22:95–123

    Article  CAS  Google Scholar 

  3. Susumu Amemiya Kei-ichi, Ishibashi T Katoh (1982) Neutron activation cross section of Molybdenum isotopes at 14.8 MeV. J Nucl Sci Technol 19(10):781–788

    Article  Google Scholar 

  4. Belgaid M, Said M, Allab M (1992) Measurement of 14.7 MeV neutron cross sections for several isotopes. J Radio Anal Nucl Chem Lett 166(6):493–502

    Article  CAS  Google Scholar 

  5. Konno C, Ikeda Y, Oishi K, Kawade K, Yamamoto H, Maekawa H (1993) Activation cross section measurements at neutron energy from 13.3 to 14.9 MeV. Report No. JAERI-1329

  6. Filatenkov AA (2016) Neutron activation cross sections measured at KRI in neutron energy region 13.4–14.9 MeV. INDC (CCP)-0460

  7. Molla NI, Miah RU, Rahman M, Ayesha A (1991) Excitation functions of some (n,p), (n,2n) and (n,alpha) reactions on nickel, zirconium and niobium isotopes in the energy range 13.63–14.83 MeV. In: Conference on nuclear data for science and technology, Juelich, p 355

  8. Woelfle R, Mannan A, Qaim SM, Liskien H, Widera R (1988) Excitation functions of 93Nb(n,2n)92mNb, 93Nb(n,α)90m,gY, 139La(n, α)136Cs and 181Ta(n,p)181Hf reactions in the energy range of 12.5–19.6 MeV. Appl Radiat Isot 39:407–412

    Article  CAS  Google Scholar 

  9. Yujiro Ikeda C, Konno K, Oishi T, Nakamura H, Miyade K, Kawade H, Yamamoto, Toshio Katoh (1988) Activation cross section measurement for fusion reactor structural materials at neutron energy from 13.3 to 15.0 MeV using FNS facility. JAERI report 1312

  10. Huang Jianzhou C, Yunfeng Z, Wenrong C (1977) Activation function of fast neutron induced nuclear reaction for Ni-58 and Nb-93. Atomic Energy Sci Technol 11(3):211

    Google Scholar 

  11. Turkiewicz J (1975) Preliminary values of cross sections for (n,a) reactions on the P-31, Mn-55, Co-59, As-75 and Nb-93. Priv comm

  12. Mannhart W, Schmidt D (2007) Measurement of neutron activation cross sections in the energy range from 8 to 15 MeV. Report of the Physikalisch-Technischen Bundesanstalt, Braunschweig

    Google Scholar 

  13. Kiraly B, Csikai J, Doczi R (2001) Validation of neutron data libraries by differential and integral cross sections. JAERI-Conf 6:283–288

    Google Scholar 

  14. Santry DC, Werner RD (1990) Cross sections for the 93Nb(n,2n)92mNb reaction. Can J Phys 68:582

    Article  CAS  Google Scholar 

  15. Lu Hanlin H, Jianzhou F, Peiguo C, Yunfeng Z Wenrong (1989) Measurement of cross sections for the (n,2n) reaction of Mn-55, Ni-58, Co-59, Nb-93, Ta-181 and Au-197. R, INDC(CPR)- No.16

  16. Csikai J (1982) Study of excitation function around 14 MeV neutron energy. Proce. of the Int. Conf. Antwerp J Nucl Sci and Technol 414-417. https://doi.org/10.1007/978-94-009-7099-1$4

  17. Paulsen A, Widera R (1970) The (n,2n) excitation functions for 93Nb and 103Rh with special respect to the isomeric states in 92Nb and 102Rh. Z Physik 238:23–34

    Article  CAS  Google Scholar 

  18. Zhao Wenrong Lu, Hanlin Yu, Weixiang H, Xiaogang H Xiaolong (1998) Measurement of cross section for 92Mo(n,p)92mNb reaction and deduction of low energy neutron. INDC(CPR)-047/L

  19. Xiangzhong K, Yongchang W, Junqiang Y, Yang Jinkang (1996) The cross section measurements for the 92Mo(n,p)92mNb, 98Mo(n,p)98mNb and 94Mo(n,2n)93mMo reactions. Journal of Lanzhou Univ. ISSN: 0455–2059

  20. Liskien H, Wolfle R, Windera R, Qaim SM (1990) Excitation functions of (n,p) and (n,α) reactions on Molybdenum isotopes. Appl Radiat Isot 41:83–90

    Article  CAS  Google Scholar 

  21. Zhang Y, Zhao L, Kong X, Liu R, Jiang L (2012) Cross-sections for (n,2n) and (n,α) reactions on 55Mn isotopes around neutron energy 14 MeV. Radi Phys Chem 81:1563–1567

    Article  CAS  Google Scholar 

  22. IAEA-EXFOR Database. http://www-nds.iaea.org/exfor

  23. Otuka N, Dupont E, Semkova V, Pritychenko B, Blokhin AI, Aikawa M, Babykina S, Bossant M, Chen G, Dunaeva S, Forrest RA, Fukahori T, Furutachi N, Ganesan S, Ge Z, Gritzay OO, Herman M, Hlavac S, Zhuang Y (2014) Towards a more complete and accurate experimental nuclear reaction data library (EXFOR): International collaboration between nuclear reaction data centers (NRDC). Nucl Data Sheets 120:272–276

    Article  CAS  Google Scholar 

  24. Koning AJ, Hilaire S, Goriely S (2017) TALYS-1.9, A Nuclear Reaction Program (NRG-1755 ZG Petten, The Netherlands). http://www.talys.eu/download-talys/

  25. Sinha A, Roy T, Yogesh K, Ray N, Shukla M, Patel T, Bajpai S, Sarkar PS, Bishnoi S (2015) Experimental subcritical facility driven by D-D/D-T neutron generator at BARC, India. Nucl Instrum Meth Phys Res B 350:66–70

    Article  CAS  Google Scholar 

  26. Pasha I, Basavanna R, Yerranguntla SS, Suryanarayana SV, Naik H, Karkera M, Radha E, Pandikumar G, Sunitha AM, Sachhidananda HB (2019) Measurement of 67Zn(n,p)67Cu, 64Zn(n,2n)63Zn, 89Y(n,γ)90mY and 89Y(n,2n)88Y reaction cross sections at the neutron energy of 14.54 MeV with covariance analysis. J Radioanal Nucl Chem. https://doi.org/10.1007/s10967-019-06883-1

    Article  Google Scholar 

  27. Pasha I, Rudraswamy B, Yerranguntla SS, Suryanarayana SV, Naik H, Midhun CV, Tarun P (2020) Measurement of 14.54 MeV neutron induced reaction cross sections of Cr and Mn with covariance analysis. Radiochim Acta. https://doi.org/10.1515/ract-2019-3189

    Article  Google Scholar 

  28. Martin MJ (2013) Nuclear data sheets for A = 152*. Nucl Data Sheets 114:1497–1847

    Article  CAS  Google Scholar 

  29. NuDat 2.7 (2016) National Nuclear Data Center, Brookhaven National Laboratory. http://www.nndc.bnl.gov/nudat2

  30. Vidmar T (2005) EFFTRAN- A Monto Carlo efficiency transfer code for gamma-ray spectrometry. Nucl Instrum Methods Phys Res A 550:603–608

    Article  CAS  Google Scholar 

  31. Sheela SY, Naik H, Prasad KM, Ganesan S, Suryanarayana SV (2017) Detailed data sets related to covariance analysis of the measurement of cross section of 59Co(n,γ)60Co reaction relative to the cross section of 115In(n,γ)116mIn. Internal report, No. Mu/Stastics/DAE-BRNS/2017. https://doi.org/10.13140/RG.2.2.26729.49764

  32. Geraldo LP, Smith DL (1990) Covariance analysis and fitting of germanium gamma-ray detector efficiency calibration data. Nucl Instrum Methods Phys Res A 290:499–508

    Article  Google Scholar 

  33. Pasha I, Rudraswamy B, Radha E, Sathiamoorthy V (2018) Efficiency of high-purity germanium detector at characteristic gamma energies of 198Au and 58Co and covariance analysis. Radiat Prot Environ 41:110–114

    Article  Google Scholar 

  34. Geraldo LP, Smith DL (1989) least square methods and covariance matrix applied to the relative efficiency calibration of a Ge(Li) detector. Inst de Pesquisas Energeticas e Nulea res 243:1–16

    Google Scholar 

  35. Millsap DW, Landsberger S (2015) Self-attenuation as a function of gamma ray energy in naturally occurring radioactive material in the oil and gas industry. Appl Radiat Isot 97:21–433

    Article  CAS  Google Scholar 

  36. Nowotny R (1998) XMuDat photon attenuation data on PC. IAEA Report IAEA-NDS 195. http://www-nds.iaea.org/publications/iaea-nds

  37. Capote R, Zolotarev KI, Pronyaev VG, Trkov A (2012) Updating and extending the IRDF-2002 dosimetry library. http://www-nds.iaea.org/IRDFF/

  38. Yerraguntla SS, Naik H, Karantha MP, Ganesan S, Suryanarayana SV, Badwar S (2017) Measurement of 59Co(n,γ)60Co reaction cross sections at the effective neutron energies of 11.98 and 15.75 MeV. J Radio Anal Nucl Chem 314(1):457–465

    Article  CAS  Google Scholar 

  39. Pasha I, Basavanna R, Yerranguntla SS, Suryanarayana SS, Meghna K, Naik H, Prasad MK, Danu LS, Saroj B, Petel T, Rajeev K (2019) 93Nb(n,2n)92mNb, 93Nb(n,α)90mY and 92Mo(n,p)92mNb reactions at 14.78 MeV and covariance analysis. J Radioanal Nucl Chem 320:561–568

    Article  CAS  Google Scholar 

  40. Meghna Karkera, Yerraguntla SS, Punchithaya S, Suryanarayana SV, Karantha MP, Nail H, Ganesan S, Dhanu LS, Kumar R, Deo K, Raj D, Patel T, Bishnoi S, Kannan U (2019) Detailed covariance analysis in the measurement of cross sections for the 232Th(n,2n)231Th reaction at the effective neutron energy of 10.49 ± 0.003 MeV, 14.46 ± 0.26 MeV, 18.36 ± 0.24 MeV and 15.03 ± 0.003 MeV using the 7Li(p,n) and 3H(d,n) reaction neutron sources. Internal report No.MAHE/STATSTICS/DAE-BRNS/2019/5

  41. Zabrodskaya SV, Ignatyuk AV, Koscheev VN (2007) Nuclear constants. ROSFOND-2010, pp 1–2

  42. Sublet J-Ch, Koning AJ, Forrest RA, Kopecky J (2004) The JEFF-3.1/A. In: Proceedings of of international conference on nuclear data for science and technology

  43. Sublet J-Ch, Packer LW, Kopecky J, Forrest RA, Koning AJ, Rochman DA (2010) The European activation file: EAF-2010 neutron-induced cross section. CCFE-R (10) 05

  44. Zsolnay EM, Capote Noy R, Nolthenius HJ, Trkov A (2014) International reactor dosimetry and fusion file (IRDF 1.05). http://www-nds.iaea.org/IRDFF/

  45. An International collaboration of NEA data bank participating countries (2017) The joint evaluated fission and fusion File (JEFF). http://www.oecd-nea.org

  46. Shibata K, Iwamoto N, Kunieda S, Minato F, Iwamoto O (2016) Activation cross-section file for decommissioning of LWRs. In: JAEA-conference, pp 47–52

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Acknowledgements

One of the author (IP) would like to thank Department of Atomic Energy & Board of Research in Nuclear Sciences (DAE-BRNS) for major research project (Sanction No. 36(6)/14/ 92/2014-BRNS/2727). The author (IP), thanks the staff of Purnima neutron generator, BARC, Mumbai for their kind cooperation for the operation of accelerator.

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Pasha, I., Basavanna, R., Yerranguntla, S.S. et al. Measurement of 14.54 ± 0.24 MeV neutron activation reaction cross sections of 93Nb, natMo with covariance analysis. J Radioanal Nucl Chem 325, 863–868 (2020). https://doi.org/10.1007/s10967-020-07261-y

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