Skip to main content
Log in

Sequential Extraction of Plutonium from the Bottom Sediments of PA Mayak’s R-4 and R-17 Reservoirs

  • Published:
Moscow University Chemistry Bulletin Aims and scope

Abstract

The speciation of 238, 239, 240Pu in the bottom sediments of two reservoirs of PA Mayak are investigated. The maximum content of plutonium in reservoir R-17 is found in the residual fraction. In reservoir R-4, plutonium is distributed equally in the residual fraction and the fraction bound to organic matter. The fact that plutonium exists in physico-chemically immobile fractions indicate its low biological availability.

This is a preview of subscription content, log in via an institution to check access.

Access this article

Price excludes VAT (USA)
Tax calculation will be finalised during checkout.

Instant access to the full article PDF.

Fig.1.

Similar content being viewed by others

REFERENCES

  1. Stukalov, P.M., Vopr. Radiats. Bezop., 2000, vol. 1, p. 50.

    Google Scholar 

  2. Andreev, S.S., Popova, I.Ya., and Pryakhin, E.A., Vestn. Chelyabinsk.Gos. Univ., 2013, vol. 7, p. 85.

    Google Scholar 

  3. Stukalov, P.M., Radioaktivnoe Zagryaznenie promyshlennogo vodoema PO “Mayak” Staroe Boloto. Obzor rezul’tatov issledovatel’skikh rabot (1949–2006 gody) (Radioactive Pollution of Industrial Pond Mayak Staroe Boloto: Review of Research Results (1949–2006)), Ozersk, 2007, part 1.

  4. Kuz’menkova, N.V., Vlasova, I.E., Rozhkova, A.K., et al., Vopr. Radiats. Bezop., 2017, vol. 1, p. 54.

    Google Scholar 

  5. Slyunchev, O.M., Kozlov, P.V., Soldatov, B.V., et al., Vopr. Radiats. Bezop., 2007, vol. 2, p. 14.

    Google Scholar 

  6. Tessier, A., Campbell, P.G.C., and Bisson, M., Anal. Chem., 1979, vol. 51, p. 844.

    Article  CAS  Google Scholar 

  7. Fedotov, P.S. and Spivakov, B.Ya., Usp. Khim, 2008, vol. 77, p. 690.

    Article  Google Scholar 

  8. Bunzl, K., Schimmack, W., Schramel, P., and Suomela, M., Analyst, 1999, vol. 124, p. 1383.

    Article  CAS  Google Scholar 

  9. Schultz, M.K., Burnett, W.C., and Inn, K.G.W., J. Environ. Radioact., 1998, vol. 40, p. 155.

    Article  CAS  Google Scholar 

  10. Lucey, J.A., Gouzy, A., Boust, D., et al., Appl. Radiat. Isot., 2004, vol. 60, p. 379.

    Article  CAS  Google Scholar 

  11. Skipperud, L., Oughton, D., and Salbu, B., Sci. Total Environ., 2000, vol. 257, p. 81.

    Article  CAS  Google Scholar 

  12. Skipperud, L., Brown, J., Fifield, L.K., Oughton, D.H., and Salbu, B., J. Environ. Radioact., 2009, vol. 100, p. 290.

    Article  CAS  Google Scholar 

  13. Pavlotskaya, F.I., Novikov, A.P., Goryachenkova, T.A., et al., Radiokhimiya, 1998, vol. 40, p. 462.

    Google Scholar 

  14. Pryakhin, E.A., Tryapitsyna, G.A., Deryabina, L.V., et al., Vopr. Radiats. Bezop., 2011, vol. 2, p. 5.

    Google Scholar 

  15. Duff, M.C., in Plutonium in the Environment, Ser.: Radioactivity in the Environment, Amsterdam: Elsevier, 2001, vol. 1, p. 139.

  16. Rai, D., Serne, R.J., and Swanson, J.L., J. Environ. Qual., 1980, vol. 9, p. 417.

    Article  CAS  Google Scholar 

  17. Stukalov, P.M. and Simkina, N.A., Vopr. Radiats. Bezop., 2008, vol. 2, p. 44.

    Google Scholar 

  18. Pryakhin, E.A., Mokrov, Yu.G., Tryapitsina, G.A., et al., J. Environ. Radioact., 2016, vol. 151, p. 449.

    Article  CAS  Google Scholar 

  19. Ure, A.M., Quevauviller, Ph., Muntau, H., and Griepink, B., Int. J. Environ. Anal. Chem., 1993, vol. 51, p. 135.

    Article  CAS  Google Scholar 

  20. Rauret, G., López-Sánchez, J.F., Sahuquillo, A., Rubio, R., and Davidson, C., J. Environ. Monit., 1999, vol. 1, p. 57.

    Article  CAS  Google Scholar 

  21. Sheppard, M.I. and Thibault, D.H., Soil Sci. Soc. Am. J., 1992, vol. 56, p. 415.

    Article  CAS  Google Scholar 

  22. Kenna, T.C., J. Environ. Radioact., 2009, vol. 100, p. 547.

    Article  CAS  Google Scholar 

  23. Jenne, E.A., Adv. Chem., 1968, vol. 73, p. 337.

    Article  Google Scholar 

  24. Torres, R.A. and Choppin, G.R., Radiochim. Acta, 1984, vol. 35, p. 143.

    Article  CAS  Google Scholar 

  25. Kim, J.I., Buckau, G., Bryant, E., and Klenze, R., Radiochim. Acta, 1989, vol. 48, p. 135.

    CAS  Google Scholar 

  26. Livens, F.R., Baxter, M.S., and Allen, S.E., Soil Sci., 1987, vol. 144, p. 24.

    Article  CAS  Google Scholar 

  27. Blumenthal, G., Engels, S., Fitz, I., Haberditzl, W., Heckner, K.-H., Henrion, G., Landsberg, R., Schmidt, W., Scholz, G., Starke, P., Wilke, I., and Wilke, K.-Th., Anorganikum: Lehr- und Praktikumsbuch der anorganischen Chemie mit einer Einführung in die physikalische Chemie (Textbook of Theoretical and Practical Inorganic Chemistry with an Introduction to Physical Chemistry), Kolditz, L., Ed., Berlin: Verlag der Wissenschaften, 1984, vol. 2.

    Google Scholar 

  28. Lujanienė, G., Motiejūnas, S., and Šapolaitė, J., J. Radioanal. Nucl. Chem., 2007, vol. 274, p. 345.

    Article  Google Scholar 

Download references

Funding

This work was performed with the support of the Russian Science Foundation, project no. 16-13-00049.

Author information

Authors and Affiliations

Authors

Corresponding author

Correspondence to A. K. Rozhkova.

Ethics declarations

CONFLICT OF INTEREST

The authors declare that they do not have a conflict of interest.

COMPLIANCE WITH ETHICAL STANDARDS

The study was performed without the use of animals or people as subjects.

Additional information

Translated by P. Kuchina

About this article

Check for updates. Verify currency and authenticity via CrossMark

Cite this article

Rozhkova, A.K., Kangina, O.A., Kuzmenkova, N.V. et al. Sequential Extraction of Plutonium from the Bottom Sediments of PA Mayak’s R-4 and R-17 Reservoirs. Moscow Univ. Chem. Bull. 75, 125–129 (2020). https://doi.org/10.3103/S0027131420020121

Download citation

  • Received:

  • Revised:

  • Accepted:

  • Published:

  • Issue Date:

  • DOI: https://doi.org/10.3103/S0027131420020121

Keywords:

Navigation