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Physical Properties of a Frustrated Quasi-One-Dimensional NaCuFe2(VO4)3 Magnet and Effect of Chemical Pressure Induced by the Substitution of Sodium for Lithium

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Abstract

The structural, thermal, static magnetic, and resonance properties of the low-dimensional NaCuFe2(VO4)3 compound obtained by the solid-phase synthesis have been investigated. In the temperature range of 110–300 K, the electron spin resonance in the X band with a g factor of 2.008 has been detected. The magnetic properties of a sample with a high frustration level in the paramagnetic, antiferromagnetic, and disordered states have been examined. A shift of the Néel temperature to the high-temperature region in an external magnetic field has been observed. The origin of the disordered magnetism in NaCuFe2(VO4)3 are discussed. The features of substitution of sodium for lithium on the physical properties of the ACuFe2(VO4)3 (A = Na, Li) system have been established. It is shown that the chemical pressure changes the crystal lattice parameters, spacings between magnetic ions, and crystallite size, which is reflected in the physical properties of the material.

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ACKNOWLEDGMENTS

The authors are grateful to the authorities of the Oak Ridge National Laboratory (USA) for presenting the opportunity of conducting neutron diffraction experiments and Matthias D. Frontzek for performing the measurements.

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Authors and Affiliations

  1. Kirensky Institute of Physics, Krasnoyarsk Scientific Center, Siberian Branch, Russian Academy of Sciences, 660036, Krasnoyarsk, Russia

    T. V. Drokina, G. A. Petrakovskii, O. A. Bayukov, M. S. Molokeev, A. M. Vorotynov, S. I. Popkov & D. A. Velikanov

  2. Siberian Federal University, 660041, Krasnoyarsk, Russia

    M. S. Molokeev & S. I. Popkov

Authors
  1. T. V. Drokina
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  2. G. A. Petrakovskii
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  3. O. A. Bayukov
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  4. M. S. Molokeev
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  5. A. M. Vorotynov
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  6. S. I. Popkov
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  7. D. A. Velikanov
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Correspondence to T. V. Drokina.

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Translated by E. Bondareva

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Drokina, T.V., Petrakovskii, G.A., Bayukov, O.A. et al. Physical Properties of a Frustrated Quasi-One-Dimensional NaCuFe2(VO4)3 Magnet and Effect of Chemical Pressure Induced by the Substitution of Sodium for Lithium. Phys. Solid State 62, 297–307 (2020). https://doi.org/10.1134/S1063783420020122

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  • DOI: https://doi.org/10.1134/S1063783420020122

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