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Experimental investigation and optimization of pool boiling heat transfer enhancement over graphene-coated copper surface

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Abstract

The current study presents an artificial neural network model used to predict the boiling heat transfer coefficient of different coating thicknesses of a graphene-coated copper surface in the pool boiling experimental setup for deionized water. The surface characterization has been carried out to study the structure, morphology and surface behavior. The investigations are carried out to evaluate the boiling heat transfer coefficient, heat flux and wall superheat for various thicknesses of nano-coated surfaces experimentally, and the obtained results are compared with those of the reported studies and existing empirical correlations. After that, these results are compared with the outputs such as current, heat flux, wall superheat and boiling heat transfer coefficient obtained using a MATLAB-based artificial neural network model with coating thickness, surface roughness and voltage as input variables. The admirable accuracies are obtained with the predicted optimal model outputs with experimental observation in each test case.

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Abbreviations

HTC:

Heat transfer coefficient (h) (kW m−2 K−1)

CHF:

Critical heat flux (W m−2)

Tn, To, Tp :

Temperature of copper heating block (°C)

Tq, Tr, Ts :

Calculated temperature of sample at different sections (°C)

T l :

Temperature of base fluid (°C)

T s :

Surface temperature of specimen (°C)

T :

Wall superheat (°C)

Qpq, Qqr, Qrs :

Heat flux at various sections (W m−2)

Kpq, Kqr, Krs :

Thermal conductivity of copper material at various sections (W m−1 K−1)

Apq, Aqr, Ars :

Cross-sectional area at various sections (m2)

xpq, ∆xrs, ∆xrs :

Thickness of surface at various sections (m)

k :

Thermal conductivity of the working fluid (W m−1 K−1)

Pr :

Prandtl number \(\left( {\frac{{\mu C_{\text{p}} }}{K}} \right)\)

C p :

Specific heat of the working fluid (kJ kg−1 K−1)

h fg :

Latent heat of vaporization of the working fluid (kJ kg−1)

q :

Pool boiling heat transfer (W m−2)

I :

Current (A)

AI:

Artificial intelligence

ANN:

Artificial neural networks

GEP:

Gene expression programming

SVR:

Support vector regression

IVR-ERVC:

In-vessel retention through extend reaction vessel cooling

CNT:

Carbon nanotubes

PEG:

Polyethylene glycol

Cu:

Copper

XRD:

X-ray diffraction

AFM:

Atomic force microscopy

SEM:

Scanning electron microscopy

DI:

De-ionized

d :

Interplanar spacing

h, k, l :

Miller indices

a, c :

Lattice constants

g :

Acceleration due to gravity (m s−2)

MLP:

Multilayer perceptron

Trainlm:

Levenberg–Marquardt backpropagation

Trainscg:

Scaled conjugate gradient backpropagation

Trainbfg:

BFGS quasi-Newton backpropagation

Traingda:

Gradient descent with adaptive learning rate backpropagation

Trainsig:

Hyperbolic tangent sigmoid transfer function

Logsig:

Log-sigmoid

MATLAB:

Matrix laboratory

MSE:

Mean square error

R :

Regression coefficient

MAPE:

Mean absolute percentage error

n :

Total number of output data

µ :

Viscosity (N s m−2)

σ :

Surface tension (N m−2)

ρ :

Density (kg m−3)

λ :

Wavelength (m)

s:

Surface

l:

Liquid

v:

Vapour

exp:

Experimental values

opt:

Predicted values

References

  1. Nukiyama S. The maximum and minimum values of the heat Q transmitted from metal to boiling water under atmospheric pressure. Int J Heat Mass Transf. 1966;9(12):1419–33.

    Google Scholar 

  2. Dharmendra M, Suresh S, Kumar CS, Yang Q. Pool boiling heat transfer enhancement using vertically aligned carbon nanotube coatings on a copper substrate. Appl Therm Eng. 2016;99:61–71.

    CAS  Google Scholar 

  3. Mehrotra AK, Nassar NN, Kasumu AS. A novel laboratory experiment for demonstrating boiling heat transfer. Educ Chem Eng. 2012;7(4):e210–8.

    Google Scholar 

  4. Parveen N, Zaidi S, Danish M. Comparative analysis for the prediction of boiling heat transfer coefficient of R134a in micro/mini channels using artificial intelligence (AI)-based techniques. Int J Model Simul. 2019. https://doi.org/10.1080/02286203.2018.1564809.

  5. Naphon P, Wiriyasart S, Arisariyawong T, Nakharintr L. ANN, numerical and experimental analysis on the jet impingement nanofluids flow and heat transfer characteristics in the micro-channel heat sink. Int J Heat Mass Transf. 2019;131:329–40.

    CAS  Google Scholar 

  6. Swain A, Das MK. ANFIS modeling of boiling heat transfer over tube bundles. In: Soft computing for problem solving. Springer; 2019; p. 433–40.

  7. Kim DE, Yu DI, Jerng DW, Kim MH, Ahn HS. Review of boiling heat transfer enhancement on micro/nanostructured surfaces. Exp Therm Fluid Sci. 2015;66:173–96.

    CAS  Google Scholar 

  8. Kumar CS, Kumar GU, Arenales MRM, Hsu C-C, Suresh S, Chen P-H. Elucidating the mechanisms behind the boiling heat transfer enhancement using nano-structured surface coatings. Appl Therm Eng. 2018;137:868–91.

    Google Scholar 

  9. Krishnan DV, Kumar GU, Suresh S, Thansekhar M, Iqbal U. Evaluating the scale effects of metal nanowire coatings on the thermal performance of miniature loop heat pipe. Appl Therm Eng. 2018;133:727–38.

    Google Scholar 

  10. Ray M, Bhaumik S. Nucleate pool boiling heat transfer of hydro-fluorocarbon refrigerant R134a on TiO2 nanoparticle coated copper heating surfaces. Heat Transf Eng. 2018;40:1–10.

    Google Scholar 

  11. Ray M, Bhaumik S. Structural properties of glancing angle deposited nanostructured surfaces for enhanced boiling heat transfer using refrigerant R-141b. Int J Refrig. 2018;88:78–90.

    CAS  Google Scholar 

  12. Jaikumar A, Kandlikar SG, Gupta A. Pool boiling enhancement through graphene and graphene oxide coatings. Heat Transf Eng. 2017;38(14–15):1274–84.

    CAS  Google Scholar 

  13. Seo H, Chu JH, Kwon S-Y, Bang IC. Pool boiling CHF of reduced graphene oxide, graphene, and SiC-coated surfaces under highly wettable FC-72. Int J Heat Mass Transf. 2015;82:490–502.

    CAS  Google Scholar 

  14. Lee MH, Heo H, Bang IC. Effect of thermal activity on critical heat flux enhancement in downward-hemispherical surface using graphene oxide coating. Int J Heat Mass Transf. 2018;127:1102–11.

    CAS  Google Scholar 

  15. Rishi AM, Gupta A, Kandlikar SG, editors. Improving liquid supply pathways on graphene oxide coated surfaces for enhanced pool boiling heat transfer performance. In: ASME 2018 16th international conference on nanochannels, microchannels, and minichannels. American Society of Mechanical Engineers; 2018.

  16. Ujereh S, Fisher T, Mudawar I. Effects of carbon nanotube arrays on nucleate pool boiling. Int J Heat Mass Transf. 2007;50(19–20):4023–38.

    CAS  Google Scholar 

  17. Park SD, Won Lee S, Kang S, Bang IC, Kim JH, Shin HS, et al. Effects of nanofluids containing graphene/graphene-oxide nanosheets on critical heat flux. Appl Phys Lett. 2010;97(2):023103.

    Google Scholar 

  18. Kim JM, Kim T, Kim J, Kim MH, Ahn HS. Effect of a graphene oxide coating layer on critical heat flux enhancement under pool boiling. Int J Heat Mass Transf. 2014;77:919–27.

    CAS  Google Scholar 

  19. Ahn HS, Kim JM, Kim MH. Experimental study of the effect of a reduced graphene oxide coating on critical heat flux enhancement. Int J Heat Mass Transf. 2013;60:763–71.

    CAS  Google Scholar 

  20. Su G, Fukuda K, Morita K, Pidduck M, Jia D, Matsumoto T, Akasaka R. Applications of artificial neural network for the prediction of flow boiling curves. J Nucl Sci Technol. 2002;39(11):1190–8.

    CAS  Google Scholar 

  21. Ertunc HM. Prediction of the pool boiling critical heat flux using artificial neural network. IEEE Trans Compon Packag Technol. 2006;29(4):770–7.

    CAS  Google Scholar 

  22. Das MK, Kishor N. Determination of heat transfer coefficient in pool boiling of organic liquids using fuzzy modeling approach. Heat Transf Eng. 2010;31(1):45–58.

    CAS  Google Scholar 

  23. Kishor N, Das MK. Soft computing techniques for prediction of boiling heat transfer coefficient of liquids on copper-coated tubes. Appl Artif Intell. 2010;24(3):210–32.

    Google Scholar 

  24. Hernandez Y, Lotya M, Rickard D, Bergin SD, Coleman JN. Measurement of multicomponent solubility parameters for graphene facilitates solvent discovery. Langmuir. 2009;26(5):3208–13.

    Google Scholar 

  25. Balandin AA, Ghosh S, Bao W, Calizo I, Teweldebrhan D, Miao F, Lau CN. Superior thermal conductivity of single-layer graphene. Nano Lett. 2008;8(3):902–7.

    CAS  PubMed  Google Scholar 

  26. Arao Y, Kubouchi M. High-rate production of few-layer graphene by high-power probe sonication. Carbon. 2015;95:802–8.

    CAS  Google Scholar 

  27. Jabbarzadeh F, Siahsar M, Dolatyari M, Rostami G, Rostami A. Fabrication of new mid-infrared photodetectors based on graphene modified by organic molecules. IEEE Sens J. 2014;15(5):2795–800.

    Google Scholar 

  28. Gupta S, Irihamye A. Probing the nature of electron transfer in metalloproteins on graphene-family materials as nanobiocatalytic scaffold using electrochemistry. AIP Adv. 2015;5(3):037106.

    Google Scholar 

  29. Jabbarzadeh F, Siahsar M, Dolatyari M, Rostami G, Rostami A. Modification of graphene oxide for applying as mid-infrared photodetector. Appl Phys B. 2015;120(4):637–43.

    CAS  Google Scholar 

  30. Siahsar M, Dolatyari M, Rostami A, Rostami G. Surface-modified graphene for mid-infrared detection. Graphene Mater Adv Appl. 2017. https://doi.org/10.5772/67490.

    Article  Google Scholar 

  31. Si Y, Samulski ET. Synthesis of water soluble graphene. Nano Lett. 2008;8(6):1679–82.

    CAS  PubMed  Google Scholar 

  32. Alaferdov AV, Gholamipour-Shirazi A, Canesqui MA, Danilov YA, Moshkalev SA. Size-controlled synthesis of graphite nanoflakes and multi-layer graphene by liquid phase exfoliation of natural graphite. Carbon. 2014;69:525–35.

    CAS  Google Scholar 

  33. Konios D, Stylianakis MM, Stratakis E, Kymakis E. Dispersion behaviour of graphene oxide and reduced graphene oxide. J Colloid Interface Sci. 2014;430:108–12.

    CAS  PubMed  Google Scholar 

  34. Johnson DW, Dobson BP, Coleman KS. A manufacturing perspective on graphene dispersions. Curr Opin Colloid Interface Sci. 2015;20(5–6):367–82.

    CAS  Google Scholar 

  35. Ayan-Varela M, Paredes JI, Guardia L, Villar-Rodil S, Munuera JM, Díaz-González M, Fernández-Sánchez CE, Martínez-Alonso A, Tascón JM. Achieving extremely concentrated aqueous dispersions of graphene flakes and catalytically efficient graphene-metal nanoparticle hybrids with flavin mononucleotide as a high-performance stabilizer. ACS Appl Mater Interfaces. 2015;7(19):10293–307.

    CAS  PubMed  Google Scholar 

  36. Hung YF, Cheng C, Huang CK, Yang CR. A facile method for batch preparation of electrochemically reduced graphene oxide. Nanomaterials. 2019;9(3):376.

    CAS  PubMed Central  Google Scholar 

  37. Kang DW, Shin HS. Control of size and physical properties of graphene oxide by changing the oxidation temperature. Carbon Lett. 2012;13(1):39–43.

    Google Scholar 

  38. Zhang TY, Zhang D. Aqueous colloids of graphene oxide nanosheets by exfoliation of graphite oxide without ultrasonication. Bull Mater Sci. 2011;34(1):25–8.

    Google Scholar 

  39. Ying JY, Benziger JB, Navrotsky A. Structural evolution of colloidal silica gels to glass. J Am Ceram Soc. 1993;76(10):2561–70.

    CAS  Google Scholar 

  40. Rivero PJ, Urrutia A, Goicoechea J, Zamarreño CR, Arregui FJ, Matías IR. An antibacterial coating based on a polymer/sol–gel hybrid matrix loaded with silver nanoparticles. Nanosc Res Lett. 2011;6(1):305.

    Google Scholar 

  41. Kline SJ. Describing uncertainty in single sample experiments. Mech Eng. 1953;75:3–8.

    Google Scholar 

  42. Andonovic B, Ademi A, Grozdanov A, Paunović P, Dimitrov AT. Enhanced model for determining the number of graphene layers and their distribution from X-ray diffraction data. Beilstein J Nanotechnol. 2015;6(1):2113–22.

    CAS  PubMed  PubMed Central  Google Scholar 

  43. Andonovic B, Grozdanov A, Paunović P, Dimitrov AT. X-ray diffraction analysis on layers in graphene samples obtained by electrolysis in molten salts: a new perspective. Micro Nano Lett. 2015;10(12):683–5.

    CAS  Google Scholar 

  44. Amaro-Gahete J, Benítez A, Otero R, Esquivel D, Jiménez-Sanchidrián C, Morales J, Caballero A, Romero-Salguero FJ. A comparative study of particle size distribution of graphene nanosheets synthesized by an ultrasound-assisted method. Nanomaterials. 2019;9(2):152.

    CAS  PubMed Central  Google Scholar 

  45. Simón M, Benítez A, Caballero A, Morales J, Vargas O. Untreated natural graphite as a graphene source for high-performance li-ion batteries. Batteries. 2018;4(1):13.

    Google Scholar 

  46. Jaikumar A. Multiscale mechanistic approach to enhance pool boiling performance for high heat flux applications; 2017. Thesis. Rochester Institute of Technology.

  47. Das S, Saha B, Bhaumik S. Experimental study of nucleate pool boiling heat transfer of water by surface functionalization with crystalline TiO2 nanostructure. Appl Therm Eng. 2017;113:1345–57.

    CAS  Google Scholar 

  48. Suryanarayana C. Experimental techniques in materials and mechanics. Boca Raton: CRC Press; 2011.

    Google Scholar 

  49. Suryanarayana C, Norton MG. X-ray diffraction: a practical approach. Berlin: Springer; 2013.

    Google Scholar 

  50. Zhang BJ, Kim KJ. Nucleate pool boiling heat transfer augmentation on hydrophobic self-assembly mono-layered alumina nano-porous surfaces. Int J Heat Mass Transf. 2014;73:551–61.

    CAS  Google Scholar 

  51. Jo H, Ahn HS, Kang S, Kim MH. A study of nucleate boiling heat transfer on hydrophilic, hydrophobic and heterogeneous wetting surfaces. Int J Heat Mass Transf. 2011;54(25–26):5643–52.

    CAS  Google Scholar 

  52. Jo H, Kim S, Kim H, Kim J, Kim MH. Nucleate boiling performance on nano/microstructures with different wetting surfaces. Nanosc Res Lett. 2012;7(1):242.

    Google Scholar 

  53. Das S, Saha B, Bhaumik S. Experimental study of nucleate pool boiling heat transfer of water by surface functionalization with SiO2 nanostructure. Exp Therm Fluid Sci. 2017;81:454–65.

    CAS  Google Scholar 

  54. Rohsenow WM. A method of correlating heat transfer data for surface boiling of liquids. Cambridge: MIT Division of Industrial Corporation; 1951.

    Google Scholar 

  55. Li Y-Y, Chen Y-J, Liu Z-H. A uniform correlation for predicting pool boiling heat transfer on plane surface with surface characteristics effect. Int J Heat Mass Transf. 2014;77:809–17.

    CAS  Google Scholar 

  56. Li N, Betz AR. Boiling performance of graphene oxide coated copper surfaces at high pressures. J Heat Transf. 2017;139(11):111504.

    Google Scholar 

  57. Akbari A, Fazel SAA, Maghsoodi S, Kootenaei AS. Pool boiling heat transfer characteristics of graphene-based aqueous nanofluids. J Therm Anal Calorim. 2019;135(1):697–711.

    CAS  Google Scholar 

  58. Basheer IA, Hajmeer M. Artificial neural networks: fundamentals, computing, design, and application. J Microbiol Methods. 2000;43(1):3–31.

    CAS  PubMed  Google Scholar 

  59. Najafi G, Ghobadian B, Tavakoli T, Buttsworth D, Yusaf T, Faizollahnejad M. Performance and exhaust emissions of a gasoline engine with ethanol blended gasoline fuels using artificial neural network. Appl Energy. 2009;86(5):630–9.

    CAS  Google Scholar 

  60. Ismail HM, Ng HK, Queck CW, Gan S. Artificial neural networks modelling of engine-out responses for a light-duty diesel engine fuelled with biodiesel blends. Appl Energy. 2012;92:769–77.

    Google Scholar 

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Gajghate, S.S., Barathula, S., Das, S. et al. Experimental investigation and optimization of pool boiling heat transfer enhancement over graphene-coated copper surface. J Therm Anal Calorim 140, 1393–1411 (2020). https://doi.org/10.1007/s10973-019-08740-5

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  • DOI: https://doi.org/10.1007/s10973-019-08740-5

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