Abstract
During thermal design in the first phases development, thermoelectric systems, such as thermoelectric generators, the most important parameter affecting the performance is thermal resistance of the components. This paper focusses on the thermal contact resistance (TCR), analyzing the influence of aging and temperature on different thermal interface materials (TIMs), i.e., thermal paste, graphite and indium. In previous papers, TCR has been studied depending on parameters such as surface roughness, bonding pressure, thermal conductivity and surface hardness. However, in thermoelectric applications, a relevant aspect to consider when choosing a TIM is aging due to thermal stress. The exposure of this type of material to high temperatures for long periods of time leads to deterioration, which causes an increase in the TCR impairing the conduction of the heat flow. Therefore, there is a need to study the behavior of TIMs exposed to temperatures typical in thermoelectric generators to make a correct selection of the TIM. It has been observed that exposure to temperatures of around 180°C induces a significant increase in the thermal impedance of the three TIMs under study, although this effect is much more relevant for thermal paste. The contact, comprising steel, thermal paste and ceramic, presents a 300% increase in the thermal impedance after 70 days of aging, whereas that exceeds 185% for the contact of aluminum, thermal paste and ceramic. In the tests with exposure temperature of 60°C, there is no observed decrease in the thermal impedance.
Similar content being viewed by others
Abbreviations
- ΔT :
-
Temperature difference between the fluxmeter surfaces in contact with the sample (°C)
- A :
-
Cross-sectional area of fluxmeter (m2)
- k A :
-
Aluminum thermal conductivity (W/m °C)
- k C :
-
Ceramic thermal conductivity (W/m °C)
- k fluxmeter :
-
Fluxmeter thermal conductivity (W/m °C)
- k S :
-
Steel thermal conductivity (W/m °C)
- L A :
-
Aluminum thickness (m)
- L c :
-
Ceramic thickness (m)
- L i :
-
Sensors position in the fluxmeter “i = 1 to 4” (m)
- L S :
-
Steel thickness (m)
- \( \dot{Q} \) :
-
Heat flow through the contact between fluxmeters (W)
- R c :
-
Thermal contact resistance, TCR (°C m2/W)
- T av :
-
Average sample temperature during the tests (°C)
- T i :
-
Temperature sensors in the fluxmeter “i = 1 to 6” (°C)
- T 3′ :
-
Bottom fluxmeter temperature in contact with the sample (°C)
- T 4′ :
-
Upper fluxmeter temperature in contact with the sample (°C)
- u(Zg):
-
Uncertainty of Global thermal impedance (°C m2/W)
- u(Ti):
-
Uncertainty of temperature sensors in the fluxmeter “i = 1 to 6” (°C)
- u(Li):
-
Uncertainty of sensors position in the fluxmeter “i= 1 to 4” (m)
- u(\( \dot{Q} \)):
-
Uncertainty of heat flow through the contact between fluxmeters (W)
- Z k :
-
Thermal impedance due to the conductivity (°C m2/W)
- Z g :
-
Global thermal impedance of the sample (°C m2/W)
References
P. Jaiswal and C.K. Dwivedi, Int. J. Innov. Technol. Creative Eng. (IJITCE) (2011). http://ia800305.us.archive.org/34/items/IJITCE/IJITCE_May3.pdf. Accessed 4 May 2011.
S. Narumanchi, M. Mihalic, K. Kelly, and G. Eesley, in ITHERM Conference Proceedings (2008). https://doi.org/10.1109/itherm.2008.4544297.
R. Prasher and C.P. Chiu, in Materials for Advanced Packaging. ed. By D. Lu and C. Wong (Springer, 2017), p. 511.
I. Hu, M. Shih, and G. Kao, in IMPACT´15 Conference Proceedings (2015). https://doi.org/10.1109/impact.2015.7365218.
G.K. Morris, M.P. Polakowski, L. Wei, M.D. Ball, M.G. Phillips, C. Mosey, and R.A. Lukaszewski, in IWIPD Conference Proceedings (2015). https://doi.org/10.1109/iwipp.2015.7295991.
J. Due and A.J. Robinson, Appl. Therm. Eng. 50, 455 (2013).
R.A. Sayer, T.P. Koehler, S.M. Dalton, T.W. Grasser, and R.L. Akau, in ASME 2013 Summer Heat Transfer Conference Proceedings (2013). https://doi.org/10.1115/ht2013-17408.
J.-P. Ousten and Z. Khatir, in EPE Conference proceedings (2011). https://hal.archives-ouvertes.fr/hal-00628876. Accessed 4 Oct 2011.
V. Khuu, M. Osterman, A. Bar-Cohen, and M. Pecht, IEEE Trans. Device Mater. Reliab. 9, 379 (2009).
R. Skuriat, J.F. Li, P.A. Agyakwa, N. Mattey, P. Evans, and C.M. Johnson, Microelectron. Reliab. 53, 1933 (2013).
American Society for Testing and Materials, ASTM Standard D5470-06 (2006).
J. Liu, H. Feng, X. Luo, R. Hu, and S. Liu, in Int. Conf. Electron. Packag. Technol. High Density Packag. ICEPT-HDP Conference Proceedings (2010), pp. 116–120.
W. Zongren, Z. Weifang, and Y. Mingyuan, Adv. Mater. Res. 337, 774 (2011).
R.A. Sayer, Heat Transf. Eng. (2015). https://doi.org/10.1080/01457632.2014.932553.
N. Goel, A. Bhattacharya, J.A. Cervantes, R.K. Mongia, S.V. Machiroutu, H.L. Lin, Y.C. Huang, K.H. Fan, B.L. Denq, C.H. Liu, C.H. Lin, C.W. Tien, and J.H. Pan, Electron. Packag. Technol. Conf. Proc. Conf. (2008). https://doi.org/10.1109/EPTC.2008.4763637.
M.C. Kumar Swamy and Satyanarayan, J. Electron. Mater. (2019). https://doi.org/10.1007/s11664-019-07623-7.
T. Sakamoto, T. Iida, T. Sekiguchi, Y. Taguchi, N. Hirayama, K. Nishio, and Y. Takanashi, J. Electron. Mater. (2014). https://doi.org/10.1007/s11664-014-3165-7.
A. Rodríguez, J.G. Vián, and D. Astrain, Appl. Therm. Eng. (2009). https://doi.org/10.1016/j.applthermaleng.2009.03.005.
A. Rodríguez, D. Astrain, A. Martínez, E. Gubía, and F.J. Sorbet, J. Electron. Mater. (2013). https://doi.org/10.1007/s11664-013-2504-4.
A. Rodríguez, D. Astrain, A. Martínez, and P. Aranguren, J. Electron. Mater. (2014). https://doi.org/10.1007/s11664-014-3097-2.
P. Aranguren, D. Astrain, A. Rodríguez, and A. Martínez, Appl. Energy (2015). https://doi.org/10.1016/j.apenergy.2015.04.077.
D.P. Bentz and K.R. Prasad, Rep. No. Building and Fire Research Laboratory (BFRL)-NIST 7401, NIST, Gaithersburg, MD. Publisher: U.S. Department of Commerce (2007).
Acknowledgments
The authors are indebted to the Spanish Ministry of Economy and Competitiveness, and the European Regional Development Fund for economic support to this work, included in the RTI2018-093501-B-C22 research project.
Author information
Authors and Affiliations
Corresponding author
Additional information
Publisher's Note
Springer Nature remains neutral with regard to jurisdictional claims in published maps and institutional affiliations.
Rights and permissions
About this article
Cite this article
Rodríguez, A., Pérez-Artieda, G., Beisti, I. et al. Influence of Temperature and Aging on the Thermal Contact Resistance in Thermoelectric Devices. J. Electron. Mater. 49, 2943–2953 (2020). https://doi.org/10.1007/s11664-020-08015-y
Received:
Accepted:
Published:
Issue Date:
DOI: https://doi.org/10.1007/s11664-020-08015-y