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Non-Lorentzian Local Density of States in Coupled Photonic Crystal Cavities Probed by Near- and Far-Field Emission

Daniele Pellegrino, Dario Balestri, Nicoletta Granchi, Matteo Ciardi, Francesca Intonti, Francesco Pagliano, Andrei Yu. Silov, Frank W. Otten, Tong Wu, Kevin Vynck, Philippe Lalanne, Andrea Fiore, and Massimo Gurioli
Phys. Rev. Lett. 124, 123902 – Published 26 March 2020
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Abstract

Recent theories proposed a deep revision of the well-known expression for the Purcell factor, with counterintuitive effects, such as complex modal volumes and non-Lorentzian local density of states. We experimentally demonstrate these predictions in tailored coupled cavities on photonic crystal slabs with relatively low optical losses. Near-field hyperspectral imaging of quantum dot photoluminescence is proved to be a direct tool for measuring the line shape of the local density of states. The experimental results clearly evidence non-Lorentzian character, in perfect agreement with numerical and theoretical predictions. Spatial maps with deep subwavelength resolution of the real and imaginary parts of the complex mode volumes are presented. The generality of these results is confirmed by an additional set of far-field and time-resolved experiments in cavities with larger modal volume and higher quality factors.

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  • Received 16 August 2019
  • Accepted 3 March 2020

DOI:https://doi.org/10.1103/PhysRevLett.124.123902

© 2020 American Physical Society

Physics Subject Headings (PhySH)

Atomic, Molecular & Optical

Authors & Affiliations

Daniele Pellegrino1, Dario Balestri2,3, Nicoletta Granchi2,3, Matteo Ciardi2, Francesca Intonti2,3, Francesco Pagliano1,4, Andrei Yu. Silov1, Frank W. Otten1, Tong Wu5, Kevin Vynck5, Philippe Lalanne5, Andrea Fiore1, and Massimo Gurioli2,3

  • 1Department of Applied Physics and Institute for Photonic Integration, Eindhoven University of Technology, 5600 MB Eindhoven, Netherlands
  • 2Department of Physics, University of Florence, via Sansone 1, I-50019 Sesto Fiorentino (FI), Italy
  • 3European Laboratory for Nonlinear Spectroscopy, via Nello Carrara 1, I-50019, Sesto Fiorentino (FI), Italy
  • 4nanoPHAB, Groene Loper 19, P.O.Box 513, 5612 AP Eindhoven, The Netherlands
  • 5LP2N, Institut d’Optique Graduate School, CNRS, Univ. Bordeaux, 33400 Talence, France

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Issue

Vol. 124, Iss. 12 — 27 March 2020

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