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Anomalous dispersion of longitudinal optical phonons in oxygen-doped La2xSrxCuO4+δ

Tim Tejsner, Andrea Piovano, Ana Ţuţueanu, Astrid T. Rømer, Barrett O. Wells, Jean-Claude Grivel, Martin Boehm, and Linda Udby
Phys. Rev. B 101, 100504(R) – Published 25 March 2020
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Abstract

Inelastic neutron scattering has been used to study the in-plane Cu-O bond-stretching mode in oxygen-doped La1.94Sr0.06CuO4.035 (Tc=38K) and La2CuO4+δ (Tc=43K). Similar to results from optimally doped La1.85Sr0.15CuO4 (Tc=35K), we observe anomalous features in the dispersion of this half-breathing mode in the form of a softening halfway through the Brillouin zone. Considering the differences in electronic structure and local environment between the oxygen- and strontium-doped compounds with similar Tc, we rule out a connection between the phonon anomaly and structural instabilities related to the specific dopant type. We interpret the phonon anomaly as a signature of correlated charge fluctuations ubiquitous in optimally doped superconductors.

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  • Received 25 October 2019
  • Accepted 11 March 2020

DOI:https://doi.org/10.1103/PhysRevB.101.100504

©2020 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

Tim Tejsner1,2, Andrea Piovano1, Ana Ţuţueanu1,2, Astrid T. Rømer1, Barrett O. Wells3, Jean-Claude Grivel4, Martin Boehm1, and Linda Udby2

  • 1Institut Laue-Langevin, 71 Avenue des Martyrs, 38000 Grenoble, France
  • 2Nanoscience Center, Niels Bohr Institute, University of Copenhagen, DK-2100 Copenhagen, Denmark
  • 3Department of Physics, University of Connecticut, Storrs, Connecticut 06269, USA
  • 4Department of Energy Conversion and Storage, Technical University of Denmark, Frederiksborgvej 399, DK-4000 Roskilde, Denmark

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Issue

Vol. 101, Iss. 10 — 1 March 2020

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