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Strained bilayer WSe2 with reduced exciton-phonon coupling

Burak Aslan, Minda Deng, Mark L. Brongersma, and Tony F. Heinz
Phys. Rev. B 101, 115305 – Published 23 March 2020
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Abstract

We investigate excitonic absorption and emission in bilayer WSe2 under tensile strain. We observe a redshift of 110 meV in the energy of the A exciton absorption peak (at the direct gap at the K point in the Brillouin zone) under 2.1% uniaxial tensile strain. In addition, under the same strain, the spectral linewidth of the A exciton at room temperature decreases by a factor of 2, from 70 to 36 meV. We show that this decrease is a result of suppression of phonon-mediated exciton scattering channels. This suppression is associated with the relative upshift under strain of the Q valley in the conduction band (involved in the indirect exciton emission), which is nearly degenerate with the K valley (involved in the A exciton). We analyze the strain-dependent absorption and photoluminescence spectra to determine the relative positions of these valleys and to infer intervalley scattering rates. Our model describes well the decrease and the distinct trends in the A exciton linewidth of monolayer and bilayer WSe2 under strain. The results show that strain can be used to tune, as well as to probe, the relative energies of band extrema and exciton scattering channels in two-dimensional semiconductors.

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  • Received 8 December 2019
  • Revised 21 January 2020
  • Accepted 6 February 2020

DOI:https://doi.org/10.1103/PhysRevB.101.115305

©2020 American Physical Society

Physics Subject Headings (PhySH)

Condensed Matter, Materials & Applied Physics

Authors & Affiliations

Burak Aslan1,*, Minda Deng2,3, Mark L. Brongersma1, and Tony F. Heinz2,3

  • 1Department of Materials Science and Engineering, and Geballe Laboratory for Advanced Materials, Stanford University, Stanford, California 94305, USA
  • 2Department of Applied Physics, Stanford University, Stanford, California 94305, USA
  • 3SLAC National Accelerator Laboratory, Menlo Park, California 94025, USA

  • *aslan@boun.edu.tr

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Issue

Vol. 101, Iss. 11 — 15 March 2020

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