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Lignocellulose aerogel and amorphous silica nanoparticles from rice husks J. Leather Sci. Eng. Pub Date : 2021-01-15 Zichao Wei; Andrew T. Smith; William R. T. Tait; Jingjing Liu; Hao Ding; Hui Wang; Weixing Wang; Luyi Sun
Rice Husks (RHs) are one of the most abundant sources of biomass in the world due to rice consumption. Lignocellulose and silica are two of the main components of RHs, which allow RHs to be applied in different areas. Lignocellulose can be partially dissolved in 1-butyl-3-methylimidazolium chloride (BMIMCl), which is a simple way of competing with the traditional extraction methods that suffer from
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Advances in microbial remediation for heavy metal treatment: a mini review J. Leather Sci. Eng. Pub Date : 2021-01-15 Shipei Wang; Ting Liu; Xiao Xiao; Shenglian Luo
In recent years, microbiological treatment to remediate contamination by heavy metals has aroused public attention as such pollution has seriously threatens ecosystems and human health and impedes sustainable development. However, the aspect of actual industrial wastewater and solid waste remediation by microorganisms is not explored sufficiently. And what we focus on is technical field of microbial
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Current trends in leather science J. Leather Sci. Eng. Pub Date : 2020-12-15 Anthony D. Covington; William R. Wise
In preparing the second edition of ‘Tanning Chemistry. The Science of Leather.’, the literature was updated and the content was revised and reviewed. Here, the new findings are presented and discussed. Notable developments include the necessary rethinking of the mechanism of sulfide unhairing because of new understanding of the aqueous chemistry of sulfide species. Revision upwards of the value of
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Effects of collagen fiber addition on the combustion and thermal stability of natural rubber J. Leather Sci. Eng. Pub Date : 2020-12-15 Weixing Xu; Xintao Wu; Qilin Wen; Shuangyang Li; Yongjiao Song; Bi Shi
Collagen fiber (CF) and silane coupling agent-modified collagen fiber (MCF) were used as flame retardant filler for natural rubber (NR) modification. The combustion phenomena and properties of composites blended with different dosages of CF or MCF were compared to elucidate the flame retardant mechanism of the composites. The flame retardancy of NR can be enhanced effectively by increasing nitrogen
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Life cycle assessment and leather production J. Leather Sci. Eng. Pub Date : 2020-11-09 Diego Navarro; Jianhui Wu; Wei Lin; Pere Fullana-i-Palmer; Rita Puig
Leather industry is facing new trends on production and consumption patterns due to society concerns. Circular economy is proposing a transition from the current economic model to a more sustainable one, in which waste is designed out and resources will be reused and recycled as long as possible. In this transition, Life Cycle Assessment (LCA) is an important tool to help decision-making. In the present
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An insight into artisanal leather making in Ghana J. Leather Sci. Eng. Pub Date : 2020-11-09 Miriam Appiah-Brempong; Helen M. K. Essandoh; Nana Yaw Asiedu; Samuel Kwame Dadzie; Francis Warings Yao Momade
The production of leather from animal skins and hides through tanning processes began in the pre-historic ages. Despite the origination of new leather making techniques such as chrome tanning which is being employed extensively today, the traditional method of leather production primarily through vegetable tanning is still being practised mostly in artisanal tanneries in developing nations including
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Screening of additives to reduce grain damage risk on unhairing by proteinase K J. Leather Sci. Eng. Pub Date : 2020-10-09 Mei Chen; Mingfang Jiang; He Li; Haiming Cheng
Enzymatic unhairing is a cleaner strategy for leather-making. It is a potential alternative to the traditional hair-burning process. However, several shortcomings, such as uncontrolled enzymatic reaction, and risk of grain looseness and damage have restricted the broad application of enzymatic unhairing. In this work, metal ions and organic additives were screened for lessening the hydrolytic activity
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Visible-light-driven photocatalytic degradation of rhodamine B using Bi2WO6/GO deposited on polyethylene terephthalate fabric J. Leather Sci. Eng. Pub Date : 2020-10-09 Zoufei Du; Ce Cui; Sihang Zhang; Hongyan Xiao; Erhui Ren; Ronghui Guo; Shouxiang Jiang
The environmental repercussions of wastewater from the dye process mean that it is very important to obtain an eco-friendly photocatalyst that would degrade wastewater. Herein, bismuth tungstate/graphene oxide (Bi2WO6/GO) composites are fabricated through in-situ hydrothermal reaction and then the Bi2WO6/GO photocatalysts are deposited onto polyethylene terephthalate (PET) fabric. The obtained Bi2WO6/GO
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Characteristics of natural biopolymers and their derivative as sorbents for chromium adsorption: a review J. Leather Sci. Eng. Pub Date : 2020-08-30 Ruoshi Zhang; Yongqiang Tian
Chromium is widely used in industry, and improper disposal of wastewater and industrial residues containing excessive chromium can contaminate water and soil, endangering both environmental and human health. Natural biopolymers and their derivatives have been investigated for removal of chromium (Cr) from wastewater. Cellulose, lignin, tannin, chitin, chitosan, and polypeptides are abundant in nature
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Aluminum tanning of hide powder and skin pieces under microwave irradiation J. Leather Sci. Eng. Pub Date : 2020-08-25 Yue Liu; Bin Song; Jinwei Zhang; Carmen Gaidau; Haibin Gu
The application and mechanism study of microwave irradiation in traditional industries have attracted considerable attention owing to the unique thermal and athermal effects that could lead to unexpected benefits in high-efficiency and clean production. Herein, we report the investigation of the aluminum tanning under microwave irradiation upon using hide powder and skin pieces, respectively, as simulants
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Facile preparation of hierarchical porous polydopamine microspheres for rapid removal of chromate from the wastewater J. Leather Sci. Eng. Pub Date : 2020-08-25 Lin Xiang; Jiayou Lin; Qin Yang; Shaojian Lin; Sheng Chen; Bin Yan
Cr(VI) containing industrial wastewaters are highly toxic and carcinogenic, and severely threats living creatures and the environment. Therefore, it is highly desired yet challenging to develop an available and economical adsorbent for simultaneously detoxifying Cr(VI) anions to Cr(III) ions and removing them from the wastewater. Here we propose a facile method for rapid removal of Cr(VI) ions from
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Alternative uses for tannery wastes: a review of environmental, sustainability, and science J. Leather Sci. Eng. Pub Date : 2020-08-12 Cesar Vinicius Toniciolli Rigueto; Marieli Rosseto; Daniela Dal Castel Krein; Bruna Elisangela Pessini Ostwald; Lillian Avila Massuda; Bárbara Belém Zanella; Aline Dettmer
The manufacture of leather covers a wide productive chain and beyond contributes to the economic flow. The various stages of leather processing result in high volumes of solid waste. In Brazil, a daily generation of 375 tons of solid waste is estimated, and landfills are still the most used route to its destination. In this review, emphasis will be given to researches that have sought alternatives
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Factors affecting thermal stability of collagen from the aspects of extraction, processing and modification J. Leather Sci. Eng. Pub Date : 2020-08-05 Xiaoxia Zhang; Songcheng Xu; Lirui Shen; Guoying Li
Collagen, as a thermal-sensitive protein, is the most abundant structural protein in animals. Native collagen has been widely applied in various fields due to its specific physicochemical and biological properties. The beneficial properties would disappear with the collapse of the unique triple helical structure during heating. Understanding thermal stability of collagen is of great significance for
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Highly selective and sensitive colorimetric chemosensor based on tricarboyanine for detection of Ag+ in industrial wastewater J. Leather Sci. Eng. Pub Date : 2020-08-03 Xiaolong Zeng; Xuezhao Li; Wen Sun
An efficient fluorescent probe 1 based on tricarbocyanine derivative was designed and synthesized, which can detect Ag+ in real industrial wastewater. UV-Vis absorption and fluorescent emission spectra of probe 1 were carried out and indicated this probe can bind Ag+ via complexation reaction, then leading to a remarkable color change from blue to light red. Furthermore, probe 1 showed high sensitive
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Chromium and leather: a review on the chemistry of relevance for allergic contact dermatitis to chromium J. Leather Sci. Eng. Pub Date : 2020-07-15 Yolanda S. Hedberg
As other causes decline in importance, chromium-tanned leather has become a more important source for chromium allergy, which affects around 1% of the general population. The aim of this review is to give suggestions on how to minimize the risk of leather-related allergic contact dermatitis, which can be elicited in chromium-allergic persons by hexavalent and trivalent chromium released from leather
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Utilization of waste wool fibers for fabrication of wool powders and keratin: a review J. Leather Sci. Eng. Pub Date : 2020-07-03 Chunhua Zhang; Liangjun Xia; Jiajing Zhang; Xin Liu; Weilin Xu
Wool fiber contains approximately 95% keratinous proteins, which is one of the most abundant sources of structural protein. However, a large amount of wool waste is underutilized. Developing appropriate approaches to recycle wool waste and produce value-added products is vital for sustainable development and reducing environmental burden. Thus, this paper reviews the mechanical methods of fabricating
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Investigation of different pre-treatments of chromium leather shavings to improve biogas production J. Leather Sci. Eng. Pub Date : 2020-06-27 Carolina Scaraffuni Gomes; Jens-Uwe Repke; Michael Meyer
Chromium shavings are wet by-products of the leather industry, of which thousands of tons accrue worldwide during leather manufacture. Due to their chromium content, chromium shavings are responsible for the most important ecological challenges caused by the leather industry. They are stable towards temperatures of up to 110 °C and enzymatic degradation. This high stability is caused by the three-dimensional
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The supramolecular redox functions of metallomacromolecules J. Leather Sci. Eng. Pub Date : 2020-06-10 Didier Astruc
Metallomacromolecules are frequently encountered in redox proteins including metal-tanned hide collagen and play crucial roles involving supramolecular properties in biological electron-transfer processes. They are also currently found in non-natural families, such as: metallopolymers, metallodendrimers and metallodendronic polymers. This mini-review discusses the supramolecular redox functions of
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Progress and mechanism of breaking glycoconjugates by glycosidases in skin for promoting unhairing and fiber opening-up in leather manufacture. A review J. Leather Sci. Eng. Pub Date : 2020-05-22 Fengxiang Luo; Xiang Zhong; Mengchu Gao; Biyu Peng; Zhongzhen Long
The glycoconjugates, herein glyco-proteins, existing in animal skins are closely related to the effectiveness of unhairing and fiber opening-up. Glycosidases have been used in leather making processes to reduce pollutants and improve leather quality. But the selection of glycosidases is still blind because the related mechanisms are not well understood yet. Hence, the animal skin structures and glycoconjugates
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Differences in loading patterns between fast walking and jogging at the same speed in male adults J. Leather Sci. Eng. Pub Date : 2020-05-04 Ruoyi Li; Hao Liu; Mengyuan Guo; Jitka Badurova; Luming Yang; Haojun Fan
Fast walking and jogging are two common exercises for people to maintain health in daily life. But the differences in loading patterns of fast walking and jogging are still unclear. The purpose of this study was to compare loading patterns in fast walking and jogging at the same speed, and to identify how differences in foot mechanics influence plantar pressure distribution between the two modes of
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Influence of microwave on chromium complex composition in tanning liquor J. Leather Sci. Eng. Pub Date : 2020-04-16 Jinwei Zhang; Wuyong Chen; Carmen Gaidau
Since microwave irradiation could promote hydrolysis and olation of chromium tanning liquor, but the influence of microwave on chromium complex component in the liquor was still unknown. Chromium sulphate solution (0% basicity) and 33% basicity chromium tanning liquor were subjected microwave (MW) and water bath (WB) heating, and the samples without any warming were regarded as control. Ion exchange
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A simple approach with scale-up potential towards intrinsically flame-retardant bio-based co-plasticizer for PVC artificial materials J. Leather Sci. Eng. Pub Date : 2020-04-15 Yong Xu; Songhang Wang; Jinming Chang; Zhou Xu; Qi Zeng; Zhonghui Wang; Jun Yan; Yi Chen
As an imitation of genuine leather, polyvinyl chloride (PVC) artificial materials are versatile, but suffers from being flammable due to the presence of large amounts of combustible plasticizers. Under such circumstance, intrinsically flame-retardant plasticizers displaying dual functions have been a subject of intensive research interest. However, previous strategies attempting to covalently attach
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Interaction between retanning agents and wet white tanned by a novel bimetal complex tanning agent J. Leather Sci. Eng. Pub Date : 2020-04-15 Wanli Huang; Ying Song; Yue Yu; Ya-nan Wang; Bi Shi
A promising and practical chrome-free tanning system has been developed based on a novel Al–Zr bimetal complex tanning agent. However, to achieve satisfactory resultant leather, the retanning process that is compatible with this emerging tannage needs to be investigated systematically. This paper aims to explore the interaction between the bimetal complex tanned wet white and retanning agents. The
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Denatured proteins as a novel template for the synthesis of well-defined, ultra-stable and water-soluble metal nanostructures for catalytic applications J. Leather Sci. Eng. Pub Date : 2020-03-23 Chaojian Chen; David Yuen Wah Ng; Tanja Weil
The templated synthesis of noble metal nanoparticles using biomass, such as proteins and polysaccharides, has generated great interest in recent years. In this work, we report on denatured proteins as a novel template for the preparation of water-soluble metal nanoparticles with excellent stability even after high speed centrifugation or storage at room temperature for one year. Different noble metal
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Facile fabrication of functional cellulose paper with high-capacity immobilization of Ag nanoparticles for catalytic applications for tannery wastewater J. Leather Sci. Eng. Pub Date : 2020-03-20 Ruiquan Yu; Tianxiang Lan; Jing Jiang; Hao Peng; Ruifeng Liang; Gongyan Liu
It has been a research goal to develop macroscopic materials with an optimized surface structure to affix silver nanoparticles which could contaminate water and maximize their practical functions. Cellulose paper is a versatile biomass material valued for its abundance, low cost, biocompatibility, and natural composition. Until now, its potential application in water purification has not been adequately
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A leather coating with self-healing characteristics J. Leather Sci. Eng. Pub Date : 2020-02-29 Feifei Liang; Tianyou Wang; Haojun Fan; Jun Xiang; Yi Chen
Genuine leather is often coated before making daily necessities such as shoes, clothing, bags, sofas, car seats, etc., so as to impart leather products various colours, higher wear resistance and water resistance and so on. However, the coating of these products is often damaged in daily use which will decrease its aesthetic effect and practicability. Therefore, how to improve the scratch resistance
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Amphiphilic hyperbranched polymers: synthesis, characterization and self-assembly performance J. Leather Sci. Eng. Pub Date : 2020-02-06 Longfang Ren; Qiaoxuan Niu; Jing Zhao; Taotao Qiang
A series of amphiphilic hyperbranched polymers (AHP-s, the “s” refers to the algebra of AHP) were synthesized by the reaction between hydroxyl-terminated hyperbranched polymers (HBP-s, the “s” refers to the algebra of HBP) and palmitoyl chloride. FTIR, NMR and GPC were used to determine the structure of AHP-s, the results showed that AHP-s exhibits core-shell structure. The thermal properties of polymers
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RAMAN AND ATR-FTIR SPECTROSCOPY TOWARDS CLASSIFICATION OF WET BLUE BOVINE LEATHER USING RATIOMETRIC AND CHEMOMETRIC ANALYSIS J. Leather Sci. Eng. Pub Date : 2020-02-05 Megha Mehta; Rafea Naffa; Catherine Maidment; Geoff Holmes; Mark Waterland
There is a substantial loss of value in bovine leather every year due to a leather quality defect known as “looseness”. Data show that 7% of domestic hide production is affected to some degree, with a loss of $35 m in export returns. This investigation is devoted to gaining a better understanding of tight and loose wet blue leather based on vibrational spectroscopy observations of its structural variations
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A facile preparation of a novel non-leaching antimicrobial waterborne polyurethane leather coating functionalized by quaternary phosphonium salt J. Leather Sci. Eng. Pub Date : 2020-01-16 Chunhua Wang; Jianhui Wu; Li Li; Changdao Mu; Wei Lin
The aim of this research is to develop a novel non-leaching antimicrobial waterborne polyurethane (WPU) leather coating material with covalently attached quaternary phosphonium salt (QPS). The structure of the QPS-bearing WPU has been identified, and their thermal stability, mechanical property, and antimicrobial performance have been investigated. The results reveal that the incorporation of QPS slightly
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The center of pressure progression characterizes the dynamic function of high-arched feet during walking J. Leather Sci. Eng. Pub Date : 2020-01-06 Bo Li; Qipeng Xiang; Xianyi Zhang
The medial longitudinal arch height has an effect on kinetic parameters during gait and might be related to the risk of injury. For the assessment of foot structures, the center of pressure (COP) trajectory is a more reliable and practical parameter than plantar pressure. This study aimed to clarify the COP trajectory and velocity characteristics in the medial-lateral and anterior-posterior direction
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Investigation of the solubility and dispersion degree of calf skin collagen in ionic liquids J. Leather Sci. Eng. Pub Date : 2019-11-11 Sicong Liu; Qian Li; Guoying Li
The dissolution of collagen in ionic liquids (ILs) was highly dependent on the polarity of ILs, which was influenced by their sorts and concentrations. Herein, the solubility and dispersion degree of collagen in two sorts of ILs, namely 1-ethyl-methylimidazolium tetrafluoroborate ([EMIM][BF4]) with low polarity and 1-ethyl-3-methylimidazolium acetate ([EMIM][Ac]) with high polarity in a concentration
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Quantitative and structural analysis of isotopically labelled natural crosslinks in type I skin collagen using LC-HRMS and SANS J. Leather Sci. Eng. Pub Date : 2019-10-31 Yi Zhang; Rafea Naffa; Christopher J. Garvey; Catherine A. Maidment; Sujay Prabakar
Collagen structure in biological tissues imparts its intrinsic physical properties by the formation of several covalent crosslinks. For the first time, two major crosslinks in the skin dihydroxylysinonorleucine (HLNL) and histidinohydroxymerodesmosine (HHMD), were isotopically labelled and then analysed by liquid-chromatography high-resolution accurate-mass mass spectrometry (LC-HRMS) and small-angle
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Kinetics and mechanism of thermal degradation of vegetable-tanned leather fiber J. Leather Sci. Eng. Pub Date : 2019-09-02 Jie Liu; Lan Luo; Yadi Hu; Fang Wang; Xuejing Zheng; Keyong Tang
Thermal degradation of vegetable-tanned leather fiber (VLF) was investigated by thermogravimetric analysis aiming to know the exact kinetics and degradation mechanism. The thermogravimetric (TG) and differential thermogravimetric (DTG) curves showed that decomposition of the VLF occurs mainly in the range of 150–600 °C, and the latter exhibits asymmetrical peak with a pronounced shoulder. The decomposition
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Collagen structure changes during chrome tanning in propylene carbonate J. Leather Sci. Eng. Pub Date : 2019-08-21 Yi Zhang; Jenna Kate Buchanan; Geoff Holmes; Bradley William Mansel; Sujay Prabakar
Green solvents, such as propylene carbonate (PC), can be used in leather processing to improve the efficiency of chrome tanning and reduce wastewater. Here we report a combined small-angle X-ray scattering (SAXS) and differential scanning calorimetry (DSC) study on PC and its efficacy as a carrier medium during chrome tanning. SAXS analysis on the collagen structure of chrome tanned leather using PC
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Regenerating leather waste for flexible pressure sensing applications J. Leather Sci. Eng. Pub Date : 2019-08-13 Jie Lei; Binghua Zou; Runan Zhang; Kang Zhang; Ruijie Xie; Weina Zhang; Jiansheng Wu; Sheng Li; Bing Zheng; Fengwei Huo
Pressure sensor can be applied in a wide range of fields, such as voice recognition, human motions detection and artificial electronic skin, the sensing of which is greatly influenced by the flexibility and stretchability of substrate materials. Here, based on the piezoresistive effect, new kinds of flexible pressure sensors have been realized from a pair of flexible and biocompatible collagen films:
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Research progress on resource utilization of leather solid waste J. Leather Sci. Eng. Pub Date : 2019-08-02 Yanchun Li; Ruijun Guo; Wenhui Lu; Deyi Zhu
Leather making is the process of converting raw hides into leather. Amounts of solid waste containing hazardous and high value components are generated during this process. Therefore, the elimination of the potential pollution and resource utilization of leather solid waste are the primary research hotspots. Herein, we comprehensively review the recent advances in the resource utilization of leather
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Insights into functional polymer-based organic-inorganic nanocomposites as leather finishes J. Leather Sci. Eng. Pub Date : 2019-07-29 Qianqian Fan; Jianzhong Ma; Qunna Xu
Nowadays, the increasing demands from consumer challenges the traditional leather products. Traditional polymer leather finishes gradually lose their dominant position in the market. To address this issue, recent research effort has been devoted to developing polymer-based organic-inorganic nanocomposite leather finishes due to their various functional properties including antibacterial, self-cleaning
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Fractionational and structural characterization of lignin and its modification as biosorbents for efficient removal of chromium from wastewater: a review J. Leather Sci. Eng. Pub Date : 2019-07-29 Bing Wang; Yong-Chang Sun; Run-Cang Sun
The removal of chromium (Cr) from wastewater by various adsorbents has been investigated. As compared with the commercial activated carbon, the biosorbents with inexpensive and high adsorption capacities are developed from lignocellulosic wastes. Lignin, existing in lignocellulosic biomass, is the second most abundant resource in nature. Recently, lignin-based bio-sorbents were served as an advanced
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Homogeneous Zr and Ti co-doped SBA-15 with high specific surface area: preparation, characterization and application J. Leather Sci. Eng. Pub Date : 2019-07-29 Taotao Qiang; Yajuan Xia; Jing Zhao
A facile synthesis procedure is proposed to prepare homogeneous Zr and Ti co-doped SBA-15 (Zr-Ti-SBA-15) with high specific surface area of 876.0 m2 g− 1. Based on “masking mechanism” from tanning, lactic acid was used as masking agent to obtain the uniform distribution of Zr and Ti species in the SBA-15 framework. The obtained materials were characterized by powder X-ray diffraction (XRD), nitrogen
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Factors affecting mass transfer of protease in pelt during enzymatic bating process J. Leather Sci. Eng. Pub Date : 2019-07-29 Ying Song; Siqi Wu; Qian Yang; Hao Liu; Yunhang Zeng; Bi Shi
Bating pelt with protease is an important process, which removes unwanted non-collagenous proteins from the pelt and moderately disperse hide collagen network. However, the grain surface, may be excessively hydrolyzed during bating due to the longer retention time of protease in the grain than in the middle layer caused by the low mass transfer rate of protease in pelt. Here, the effects of protease
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Epoxidized methyl ricinoleate bio-plasticizer with a pendant acetate ester for PVC artificial material: circumventing existing limit on achievable migration resistance J. Leather Sci. Eng. Pub Date : 2019-07-29 Siyu Pan; Delong Hou; Gaofu Yang; Qiuping Xie; Sunxian Yan; Qi Zeng; Zhonghui Wang; Yi Chen; Haojun Fan
Processing polyvinyl chloride (PVC) artificial material requires plasticizer that softens the PVC coating. Currently, utilizing unsaturated fatty acid methyl esters to obtain epoxidized fatty acid methyl ester (EFAME) bio-plasticizers constitutes an environmentally responsible solution to substitute conventional ortho-phthalates that are endocrine disruptors or probable carcinogens. However, commercial