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Quantify the contribution of chain length heterogeneity on block copolymer self-assembly Giant Pub Date : 2020-11-20 Yanxiao Sun; Rui Tan; Zhuang Ma; Dongdong Zhou; Jinbin Li; Deyu Kong; Xue-Hui Dong
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What is next in polymer-grafted plasmonic nanoparticles? Giant Pub Date : 2020-11-05 Hanyi Duan; Yiqun Yang; Yan Zhang; Chenglin Yi; Zhihong Nie; Jie He
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Mesoatom alloys via self-sorting approach of giant molecules blends Giant Pub Date : 2020-10-01 Yuchu Liu; Tong Liu; Xiao-yun Yan; Qing-Yun Guo; Jian Wang; Rongchun Zhang; Shuailin Zhang; Zebin Su; Jiahao Huang; Geng-Xin Liu; Wei Zhang; Wei Zhang; Takuzo Aida; Kan Yue; Mingjun Huang; Stephen Z.D. Cheng
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Understanding humidity-induced actuation in Antheraea pernyi silks Giant Pub Date : 2020-09-28 Zhen Wang; Shihui Lin; Jing Ren; Ying Pei; Min Chen; Zeming Qi; Zhengzhong Shao; Shengjie Ling
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Synthesis of High-Molecular-Weight Poly(ε-caprolactone) via Heterogeneous Zinc-Cobalt(III) Double Metal Cyanide Complex Giant Pub Date : 2020-09-29 Zi-Heng Liu; Yang Li; Cheng-Jian Zhang; Ying-Ying Zhang; Xiao-Han Cao; Xing-Hong Zhang
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Water-Mediated Through-Space-Conjugation of Aromatic Groups for Stimuli-Responsive Photoluminescence Giant Pub Date : 2020-09-26 Yang Yang; Haoke Zhang; Chin Yi Chen; Da Peng Liu; Ankit Raj; Hiro-o. Hamaguchi; Ben Zhong Tang; Yan Jun Lin; Chien Lung Wang; Xiao Song Wang
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Efficient room-temperature solid-state lithium ion conductors enabled by mixed-graft block copolymer architectures Giant Pub Date : 2020-09-11 Xiaoyu Ji; Mengxue Cao; Xiaowei Fu; Ruiqi Liang; An N. Le; Qiuting Zhang; Mingjiang Zhong
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Morphological and constituent viral-mimicking self-assembled nanoparticles promote cellular uptake and improve cancer therapeutic efficiency in vivo Giant Pub Date : 2020-08-31 Wenbo Zhang; Zihe Zhai; Shenyu Huang; Zhengwei Mao; Yixian Zhang; Changyou Gao
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An ultrathin polydiacetylene nanosheet as dual colorimetric and fluorescent indicator for lysophosphatidic acid, a cancer biomarker Giant Pub Date : 2020-09-03 Bojian Hu; Peiyi Wu
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Incorporation of fluorescent microgels inside calcite single crystals Giant Pub Date : 2020-08-16 Xinyi Jin, Jinqiao Xue, Dong Hee Kang, Yujing Liu, Jie Ren, Quan Wen, Dapeng Hu, Yan Yu, Wei Yang, Binyang Du, Myung-Han Yoon, Hanying Li
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Natural polyphenols in drug delivery systems: Current status and future challenges Giant Pub Date : 2020-08-07 Hui Wang, Changping Wang, Yuan Zou, Jingjing Hu, Yiwen Li, Yiyun Cheng
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Anisotropic ion transport in 2D polymer single crystal-based solid polymer electrolytes Giant Pub Date : 2020-08-07 Shan Cheng, Xiaowei Li, Yongwei Zheng, Derrick M. Smith, Christopher Y. Li
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Dynamic artificial light-harvesting systems based on rotaxane dendrimers Giant Pub Date : 2020-07-31 Wei-Jian Li, Xu-Qing Wang, Wei Wang, Zhubin Hu, Yubin Ke, Hanqiu Jiang, Chunyong He, Xueli Wang, Yi-Xiong Hu, Pei-Pei Jia, Panchao Yin, Jinquan Chen, Haitao Sun, Zhenrong Sun, Lin Xu, Hai-Bo Yang
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Manipulating small water droplets on a photo-switchable mat of fluorinated linear liquid crystal polymers Giant Pub Date : 2020-07-29 Xiao Zhang, Lang Qin, Yuyun Liu, Jia Wei, Yanlei Yu
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Reaction: Amplification of macromolecular helicity through self-assembly Giant Pub Date : 2020-07-03 By Kai-Chieh Yang, Puhup Puneet, Rong-Ming Ho
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Diving into the active, complex and living fairyland of precise biomacromolecular self-assemblies Giant Pub Date : 2020-04-27 Guosong Chen
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Deciphering chiral structures in soft materials via resonant soft and tender X-ray scattering Giant Pub Date : 2020-07-28 Yu Cao, Chenrun Feng, Antal Jakli, Chenhui Zhu, Feng Liu
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Bio-inspired drag reduction: From nature organisms to artificial functional surfaces Giant Pub Date : 2020-07-25 Cunming Yu, Mengfei Liu, Chunhui Zhang, Hao Yan, Minghui Zhang, Qingshan Wu, Mingjie Liu, Lei Jiang
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Catalytic one-handed helix-induction and memory of amphiphilic poly(biphenylylacetylene)s in water Giant Pub Date : 2020-06-29 Tomoyuki Ikai, Kosuke Mizumoto, Ryoma Ishidate, Winald R. Kitzmann, Riho Ikeda, Chiaki Yokota, Katsuhiro Maeda, Eiji Yashima
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Anti-Freezing multiphase gel materials: Bioinspired design strategies and applications Giant Pub Date : 2020-06-27 Yichao Xu, Qinfeng Rong, Tianyi Zhao, Mingjie Liu
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Supramolecular Nanostructures Constructed from Cluster-based Hybrid Macromolecules Giant Pub Date : 2020-06-06 Jiancheng Luo, Xinyu Sun, Jia-Fu Yin, Panchao Yin, Tianbo Liu
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Self-Immolative nanoparticles for stimuli-triggered activation, covalent trapping and accumulation of in situ generated small molecule theranostic fragments Giant Pub Date : 2020-05-22 Zexuan Ding, Jie Cen, Yun Wu, Kai Zhong, Guhuan Liu, Jinming Hu, Shiyong Liu
Small molecule theranostic agents suffer from fast blood clearance whereas nanoparticle ones are incapable of molecular functions and often nondegradable. We propose to bridge the gap between nanoparticles and small molecule agents based on self-immolative polymers which undergo triggered cascade depolymerization at the chain level. Amphiphilic block copolymers containing side chain-functionalized
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Giant is different: Size effects and the nature of macromolecules Giant Pub Date : 2020-05-19 Wen-Bin Zhang, Stephen Z.D. Cheng
A century after Staudinger's Macromolecular Hypothesis, macromolecular science is entering a new era. In this perspective, we discuss size effects and the nature of macromolecules. With increasing molecular size, the complexity increases dramatically in terms of both primary chemical structure and assembled physical structure, as exemplified by the information-bearing molecules like DNA, RNA, and proteins
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Entropy-driven segregation and budding in hybrid vesicles of binary nanoparticle amphiphiles Giant Pub Date : 2020-05-19 Chelsey Lamar, Yijing Liu, Chenglin Yi, Zhihong Nie
Self-assembly of giant building blocks beyond conventional molecules offers tremendous opportunities for the fabrication of new-generation structural materials. This work describes the macroscopic colloidal segregation in the vesicular self-assembly of binary nanoparticle amphiphiles (NPAMs) consisting of block copolymer-grafted nanoparticles in solution. Depending on their relative size and concentration
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RNA can function as molecular chaperone for RNA folding Giant Pub Date : 2020-05-15 Zhi-Chao Lei, Xue Yin, Xinchang Wang, Guoliang Ke, Xiaoyu Cao, Chunhai Fan, Chaoyong James Yang, Haojun Liang, Zhong-Qun Tian
RNAs can mimic the information storage, replication and catalysis functions of DNAs and proteins, providing physical evidence for the widely accepted RNA world hypothesis that RNA alone constitutes earlier life forms. However, the currently found molecular chaperones for correcting RNA folding are proteins, which poses a question on whether RNA itself can avoid misfolding in the absence of proteins
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Supramolecular organic frameworks with ultralong phosphorescence via breaking π-Conjugated structures Giant Pub Date : 2020-05-15 Wei Yao, Chaoqun Ma, Huili Ma, Lishun Fu, Song Lu, Anqi Lv, Suzhi Cai, Xiaochun Hang, Manjeet Singh, Huifang Shi, Zhongfu An, Wei Huang
Development of crystalline porous materials with luminescent properties have gradually attracted attention for their potential applications in drug delivery, bioimaging, photoelectronic and so on. To date, it is a formidable challenge to rationally design porous phosphorescent materials. Herein, we have reported a chemical strategy of breaking π-conjugated structures of phosphorescent molecules by
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pH-responsive Frame-Guided Assembly with hydrophobicity controllable peptide as leading hydrophobic groups Giant Pub Date : 2020-05-15 Chao Wang, Yiyang Zhang, Yu Shao, Xiancheng Tian, Jiafang Piao, Yuanchen Dong, Dongsheng Liu
Frame-Guided Assembly (FGA) strategy has been recently reported to prepare vesicles with customized shapes and sizes. However, the effects of the interaction between leading hydrophobic groups (LHGs) and amphiphiles on the thermodynamic and kinetic control of the FGA process haven't been fully understood. In this work, we employed the pH low-insertion peptide (pHLIP) as the LHGs because its interaction
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Competitive cation−π interactions between small cations and polycations with phenyl groups in poly(cation−π) hydrogels Giant Pub Date : 2020-04-29 Hailong Fan, Honglei Guo, Jiahui Wang, Jian Ping Gong
Although cation−π interactions play a critical role in biological systems, experimental studies in aqueous environments are limited due to a lack of suitable systems and methods. The recent success in synthesizing water-soluble poly(cation−π) bearing adjacent cationic/aromatic residues provides excellent systems for studying cation−π interactions in aqueous environments. In this study, we investigated
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Grafting density-induced smectic A to hexagonal columnar transition in mesogen-free isotactic liquid crystalline polyethers with n-dodecylsulfonyl side groups Giant Pub Date : 2020-04-23 Man-Hin Kwok, Caleb A. Bohannon, Jordan L. Crooks, Ruipeng Li, Bin Zhao, Lei Zhu
Highly dipolar mesogen-free liquid crystalline polymers are excellent candidates for achieving large spontaneous polarization under relatively low electric fields for advanced electrical and optical applications. In this report, the effect of grafting density of n-dodecylsulfonyl side chains on the mesogen-free liquid crystalline self-assembly of comb-like isotactic poly(oxypropylene) was studied.
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Supramolecular spheres assembled from covalent and supramolecular dendritic crowns dictate the supramolecular orientational memory effect mediated by Frank–Kasper phases Giant Pub Date : 2020-04-06 Ning Huang, Mohammad R. Imam, Monika J. Sienkowska, Mihai Peterca, Marian N. Holerca, Daniela A. Wilson, Brad M. Rosen, Benjamin E. Partridge, Qi Xiao, Virgil Percec
A supramolecular orientational memory (SOM) effect that provides access to complex columnar hexagonal architectures that cannot be designed by any other methodology was recently reported by our laboratory. This SOM concept is encountered upon heating and cooling a hexagonal columnar periodic array via a Frank–Kasper phase that is generated from supramolecular spheres. Here, a library of twenty-four
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Fine-tuned order-order phase transitions in giant surfactants via interfacial engineering Giant Pub Date : 2020-04-06 Wenpeng Shan, Wei Zhang, Mingjun Huang, Yuyang Ji, Ruimeng Zhang, Rui Zhang, Zebin Su, Hao Liu, Xueyan Feng, Dong Guo, Jiahao Huang, Tong Liu, Tao Li, Jialin Mao, Chrys Wesdemiotis, An-Chang Shi, Stephen Z.D. Cheng
Thermotropic order-order phase transitions (OOTs) in block copolymers are not commonly observed in the strong segregation region. Phase separation of giant surfactants composed of hydrophilic molecular nanoparticles (MNPs) as heads and hydrophobic flexible polymer chains as tails occurs generally in the strong segregation region. By introducing a rigid molecular segment at the junction point of the