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Surface-imprinted polymers based on 3D printing resin for selective bacteria detection Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-03-05 Tamara M. Iakimova, Benjamin Heidt, Amy Q. Shen
Surface-imprinted polymers (SIPs) are biomimetic receptors that emulate the molecular recognition capabilities of antibodies but offer enhanced stability. Traditional contact imprinting for SIP fabrication is labor intensive and can produce inconsistent results due to the manual polymer synthesis. Laying the groundwork for future SIP imprinting with three-dimensional (3D) printers, our study pioneers
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Verification of Bell nonlocality by violating quantum monogamy relations Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-22 Yan-Han Yang, Xin-Zhu Liu, Xing-Zhou Zheng, Shao-Ming Fei, Ming-Xing Luo
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A three-minute gram-scale synthesis of amines via ultrafast “on-water” in continuo organolithium addition to imines Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-21 Jacopo Brucoli, Alessandra Puglisi, Sergio Rossi, Davide Gariboldi, Davide Brenna, Ivano Maule, Maurizio Benaglia
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Unleashing the benefits of smart grids by overcoming the challenges associated with low-resolution data Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-21 Rui Yuan, S. Ali Pourmousavi, Wen L. Soong, Andrew J. Black, Jon A.R. Liisberg, Julian Lemos-Vinasco
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Post-positioned gas spring enables ultra-high output power of hybrid thermoacoustic electric generators Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-21 Yuanhang Chen, Guoyao Yu, Yanyan Chen, Shunmin Zhu, Jing Luo, Yanlei Sun, Ercang Luo
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Coalescence and detachment of double bubbles on electrode surface in photoelectrochemical water splitting Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-20 Bo Zhang, Yechun Wang, Yuyang Feng, Canghao Zhen, Miaomiao Liu, Zhenshan Cao, Qiuyang Zhao, Liejin Guo
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Protective shielding films for atomic-level evaluation of lithium lanthanum zirconium oxide at room temperature Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-20 Haiming Sun, Kazuo Yamamoto
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Ultrafast synthesis of high-entropy carbides up to 3,273 K for superior oxidation resistance Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-14 Zihao Wen, Zhongyu Tang, Hong Meng, Lei Zhuang, Hulei Yu, Yanhui Chu
Exploiting the huge compositional space is significant in achieving the superior oxidation resistance of high-entropy carbides (HECs) yet is challenging with conventional synthesis techniques. Herein, we develop an ultrafast high-temperature synthesis apparatus to reach a heating temperature of 3,273 K within seconds. Based on this apparatus, the equiatomic 4- to 9-cation HECs of the IVB, VB, and VIB
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Predicting cell failure and performance decline in lithium-sulfur batteries using distribution of relaxation times analysis Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-14 Roby Soni, Ji Hu, James B. Robinson, Alexander J.E. Rettie, Thomas S. Miller
While lithium-sulfur (Li-S) batteries are a promising next-generation technology, their complex chemistry means they can degrade and fail via numerous mechanisms. To minimize or overcome these modes of failure, we must develop tools that can differentiate between chemical processes in the operating cell, reveal their effects on cell health, and monitor cells throughout their lifetimes. In this study
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Structure and applications of PIC-based polymers and hydrogels Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-14 Kaizheng Liu, Johannes Vandaele, Hongbo Yuan, Kerstin G. Blank, Roel Hammink, Paul H.J. Kouwer, Susana Rocha
Over the last decade, water-soluble polyisocyanopeptides (PICs) have emerged as a new class of biomimetic polymers. Analogous to biopolymers, PICs exhibit a semi-flexible nature; however, unlike their biological counterparts, they possess the unique advantage of being highly customizable. Hydrogels made of PICs have a fibrous and porous architecture and, consequently, unique mechanical properties.
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Real-time quantum control of spin-coupling damping and application in atomic spin gyroscopes Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-13 Hongyu Pei, Lihong Duan, Longyan Ma, Shimiao Fan, Ze Cai, Zhihong Wu, Wenfeng Fan, Wei Quan
Integrating classical estimation and control theory with quantum systems holds potential for quantum measurement improvement. Here, we report a real-time linear quadratic regulator (LQR) optimal control for spin damping in electron-nuclear spin-coupling regime. The aim is a quicker response and enhanced noise suppression for precision quantum measurements. Using a Kalman quantum observer with electron
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Noble gas management with radiation-tolerant MOF for molten salt reactors Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-12 Alexander J. Robinson, Hannah M. Johnson, Saehwa Chong, Brian J. Riley, Mark K. Murphy, Parker Okabe, Praveen K. Thallapally
One of the advantages of molten salt reactors (MSRs) is their ability to dynamically release volatile fission products such as Kr and Xe from the fuel. In order to manage this consistent radioactive off-gas, unselective delay beds of activated carbon allow the decay of short-lived isotopes. An improved sorbent material would demonstrate both higher delay efficiency and selectivity for Xe over Kr for
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Ball-milling-enabled nickel-catalyzed radical relayed reductive cross-coupling Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-12 Chunying Fan, Bobo Wang, Tianle Wu, Qinchun Kang, Huishuang Wang, Jiajia Sun, Xiaofeng Wei
Nickel-catalyzed radical relayed dicarbofunctionalizations of olefins, utilizing carbon electrophiles as coupling partners, present a powerful strategy for the streamlined construction of aliphatic structures. However, traditional solution-phase methods encounter challenges such as the need for bulk solvents, limited coupling partners, long reaction times, and air-/moisture-sensitive reagents. As an
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Neutron diffraction from a microgravity-grown crystal reveals the active site hydrogens of the internal aldimine form of tryptophan synthase Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-12 Victoria N. Drago, Juliette M. Devos, Matthew P. Blakeley, V. Trevor Forsyth, Jerry M. Parks, Andrey Kovalevsky, Timothy C. Mueser
Pyridoxal 5′-phosphate (PLP), the biologically active form of vitamin B, is an essential cofactor in many biosynthetic pathways. The emergence of PLP-dependent enzymes as drug targets and biocatalysts, such as tryptophan synthase (TS), has underlined the demand to understand PLP-dependent catalysis and reaction specificity. The ability of neutron diffraction to resolve the positions of hydrogen atoms
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Visualization of electron beam-induced desintering of nanostructured ceramics at the atomic scale Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-12 Tanna E.R. Fiuza, Bruno Focassio, Jefferson Bettini, Gabriel R. Schleder, Murillo H.M. Rodrigues, João B. Souza Junior, Adalberto Fazzio, Rodrigo B. Capaz, Edson R. Leite
Mass diffusion and local tensile stress associated with electron beam irradiation can favor the desintering process. Here, we report the electron beam-induced desintering of ZrO thin films at the atomic scale with unprecedented spatial resolution using high-resolution transmission electron microscopy (HRTEM). Our results confirm earlier works in which desintering is driven by tensile stress acting
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Formation and stabilization of metastable halide perovskite phases for photovoltaics Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-09 Shuangyan Hu, Arnauld Robert Tapa, Xuechang Zhou, Shuping Pang, Monica Lira-Cantu, Haibing Xie
Halide perovskites are semiconductors that have impacted the photovoltaic field in single and multijunction devices. Among them, metastable FAPbI-based (FA, formamidinium) and CsPbI-based perovskites are frontrunner materials for perovskite solar cells. However, they face the same challenge; their photoactive black perovskite phases spontaneously transform into the yellow non-photoactive δ phases at
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Direct synthesis of iso-olefins from carbon dioxide hydrogenation via tandem catalysis Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-09 Qinqin Ji, Di Li, Jingting Hu, Pan Gao, Guangjin Hou, Yanting Liu, Dehui Deng
The direct production of iso-olefins using carbon dioxide and hydrogen is a promising alternative to traditional petrochemical routes, but it has not been fully achieved due to the lack of suitable catalysts and processes for the conversion. Herein, we report a tandem process for the direct synthesis of C-C iso-olefins from carbon dioxide and hydrogen. The process proceeds by hydrogenation of carbon
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High-power iontronics enabled by nanoconfined ion dynamics Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-08 Puguang Peng, Feiyao Yang, Xiang Li, Shaoxin Li, Zhonglin Wang, Di Wei
Tailoring ion dynamics within nanoconfined spaces presents a new approach for developing advanced iontronic devices. Using various nano-hierarchical materials with nanoconfined spaces can regulate anomalous ionic behaviors, but research on coupling interfacial reactions and ionic dynamics in nanoconfined spaces remains unclear, which limits their applications in energy harvesting. Here, we develop
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A facile two-photon red-emission fluorescent marker with a large Stokes shift for in vivo brain imaging of amyloid-beta aggregates Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-08 Miao Chen, Ziwei Zhang, Zhen Shi, Junyong Sun, Feng Gao
Efficient fluorescent probes for brain imaging of the progressive changes of amyloid-beta (Aβ) aggregates in Alzheimer’s disease (AD) are highly desired to track the occurrence and development of AD. Herein, a donor-acceptor-donor-type fluorescent probe (BTD-Aβ) is prepared using benzothiadiazole (BTD) scaffold as the acceptor, together with p-dimethylaminobenzene and p-hydroxybenzene as donors. The
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Construction of halogenated tetrasubstituted carbon centers through copper(I)-catalyzed asymmetric alkylation of 2-azaarylesters Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-07 Zi-Qing Wang, Zong-Ci Liu, Xiaoyu Huang, Liang Yin
Catalytic asymmetric alkylation of α-halogenated enolates is a challenging issue due to their extenuated nucleophilicity and the electrophilic and oxidative nature of the parent α-Cl/Br carbonyl compounds. Herein, by means of coordination-stabilized copper(I) α-F/Cl enolates as the nucleophiles, a catalytic asymmetric alkylation of 2-azaarylesters is achieved with a broad substrate scope on alkyl halides
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A toolbox for investigating liquid metal systems Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-07 Vaishnavi Krishnamurthi, Caiden J. Parker, Chung Kim Nguyen, Pierre H.A. Vaillant, Rosalie K. Hocking, Benedikt Haas, Andrew J. Christofferson, Salvy P. Russo, Ken Chiang, Aaron Elbourne, Torben Daeneke
The exceptional properties of liquid metals at room temperature, such as their fluidity, stretchability, deformability, and potential applications, have rapidly inspired the scientific community. At present, the main challenge is overcoming technical barriers associated with the characterization of liquid metal systems, which have resulted in their molecular structure remaining effectively unknown
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Enhanced retention and clean dewatering of nutrients in a slow-release organic silicon fertilizer Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-07 Gareth Griffiths, Michal M. Czachor, Jac Dimond, Christian J. Laycock, Alan J. Guwy
The development of sustainable fertilizers prepared from local and renewable resources is an increasingly urgent challenge faced by agricultural and food sectors globally. This challenge is complicated by the need to deliver nutrients directly to crops with minimal environmental impact. Here, we explore the characteristics of an organic silicon fertilizer prepared by treatment of digestate using potassium
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Development of 4D-bioprinted shape-morphing magnetic constructs for cartilage regeneration using a silk fibroin-gelatin bioink Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-06 Juhi Chakraborty, Julia Fernández-Pérez, Milad Takhsha Ghahfarokhi, Kenny A. van Kampen, Tim ten Brink, Jopeth Ramis, Maria Kalogeropoulou, Riccardo Cabassi, César de Julián Fernández, Franca Albertini, Carlos Mota, Sourabh Ghosh, Lorenzo Moroni
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Nematic superconductivity from selective orbital pairing in iron pnictide single crystals Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-06 Mason L. Klemm, Shirin Mozaffari, Rui Zhang, Brian W. Casas, Alexei E. Koshelev, Ming Yi, Luis Balicas, Pengcheng Dai
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Metastable polar orthorhombic local structure of hydrothermally grown HfO2 nanocrystals Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-06 Guan-Wen Liu, Wasif Zaheer, Luis Carrillo, Sarbajit Banerjee
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Dynamical and thermodynamical origins of motility-induced phase separation Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-05 Jie Su, Zhiyu Cao, Jin Wang, Huijun Jiang, Zhonghuai Hou
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High-throughput ab initio calculations and machine learning to discover SrFeO3-δ-based perovskites for chemical-looping applications Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-29 Ali Ramazani, Brett A. Duell, Eric J. Popczun, Sittichai Natesakhawat, Tarak Nandi, Jonathan W. Lekse, Yuhua Duan
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Supercapacitive performance of ionic-liquid-intercalated two-dimensional Ti3C2Tx in redox electrolyte Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-30 Ashwini Jadhav, Plawan Kumar Jha, Mikko Salomäki, Sari Granroth, Pia Damlin, Carita Kvarnström
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Spontaneous assembly of bilayer perovskite crystals for built-in p-n homojunction Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-29 Ruihao Ma, Xiangjun Xu, Bowen Jin, Siwen Liu, Jinguo Cao, Shimin Wang, Erjing Wang, Liang Chu, Congcong Wu
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Producing naturally degradable room-temperature phosphorescent materials by covalently attaching lignin to natural polymers Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-01 Mengnan Cao, Fang Liu, Xinzhu Huo, Shouxin Liu, Jian Li, Shujun Li, Tony D. James, Zhijun Chen
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Condensation device design represents a critical step for solar-driven water evaporation toward practical applications Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-01 Zexiang Zhao, Chengbing Wang, Dan Wei, Fan Wang
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Cutaneous respiration inspired porous seawater electrodes Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-01 Tianzi Li, Lingling Xia, Yucen Li, Wei Zhang, Ming Hu
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A highly efficient heat-driven thermoacoustic cooling system Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-01 Lei Xiao, Kaiqi Luo, Zhanghua Wu, Jiaxin Chi, Jingyuan Xu, Limin Zhang, Jianying Hu, Ercang Luo
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Bionic metamaterial for multispectral-compatible camouflage of solar spectrum and infrared in the background of vegetation Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-01 Kai Xu, Linshuang Long, Wei Yang, Zizhen Huang, Hong Ye
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Amino-acid-specific thiol-ene coupling governs hydrogel crosslinking mechanism and cell behavior Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-02-01 Ke Yang, Kongchang Wei, Marine de Lapeyrière, Katharina Maniura-Weber, Markus Rottmar
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Producing sustainable room temperature phosphorescent materials using natural wood and sucrose Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-31 Wei-Ming Yin, Ben Dang, Yuanyuan Miao, Shujun Li, Jian Li, Shouxin Liu, Tony D. James, Zhijun Chen
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Bioreceptors as the key components for electrochemical biosensing in medicine Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-31 Xueqi Wang, Jianhua Zhou, Han Wang
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3D in situ heterogeneous SiC/mullite hollow constructs for broadband electromagnetic absorption Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-31 Changshun Wang, Qingchun Yang, Xingguo Gu, Annan Chen, Guizhou Liu, Shixiang Zhou, Zhaoqing Li, Chunze Yan, Yuheng Tian, Yusheng Shi, Jian Lu
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Spatially isolated dual-active sites enabling selective hydrogenation Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-31 Sai Zhang, Yongquan Qu
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Atomic structures of naphthalene dipeptide micelles unravel mechanisms of assembly and gelation Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-31 Ravi R. Sonani, Simona Bianco, Bart Dietrich, James Doutch, Emily R. Draper, Dave J. Adams, Edward H. Egelman
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Reviewing direct air capture startups and emerging technologies Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-31 Eryu Wang, Rahul Navik, Yihe Miao, Qi Gao, David Izikowitz, Lei Chen, Jia Li
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A four-electrode droplet triboelectric nanogenerator providing multimodal output Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-31 Peng He, Jing Ding, Le Lei, Wen-Quan Tao
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Physically based machine learning for hierarchical materials Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-30 Vincenzo Fazio, Nicola Maria Pugno, Orazio Giustolisi, Giuseppe Puglisi
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From fundamentals to future challenges for flexible piezoelectric actuators Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-30 Tianxiang Gao, Qingwei Liao, Wei Si, Yu Chu, Heyu Dong, Yinghao Li, Yaoyao Liao, Lei Qin
Flexible actuators, as the main components of soft robots and intelligent structures, can produce reversible mechanical deformations in response to external environmental stimuli such as light, electric fields, steam, and more. Piezoelectric flexible actuators, in particular, demonstrate clear advantages compared to other types of actuators due to their high precision, extremely fast response speed
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Optimizing grain boundary potential barriers for enhanced thermoelectric performance of NbFeSb alloy Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-30 Chang Tan, Adeel Abbas, Hongxiang Wang, Zhihao Li, Yuqing Sun, Yujie Zong, Hui Sun, Chunlei Wang, Hongchao Wang
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A vanadium-chromium redox flow battery toward sustainable energy storage Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-29 Xiaoyu Huo, Xingyi Shi, Yuran Bai, Yikai Zeng, Liang An
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Ultrasound-based separation of ethanol-water mixtures is economically advantageous and sustainable Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-29 Ji Woo Ha, Junli Liu, Hao Feng, Nikolaos V. Sahinidis, Hyerin Seo, Jeffrey J. Siirola, Jonggeol Na
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Pinacolborane-assisted superacid organocatalysis enabled direct access to cytotoxic alkyl N-Cbz amines Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-29 Woo Hee Kim, Seon Bin Song, Da Eun Lee, Prithwish Goswami, You Kyoung Chung, Sohyeong Choi, Won Hee Jung, Sang Un Choi, Shinwon Ham, Yujin Oh, Ki Hyun Kim, Joonsuk Huh, Han Yong Bae
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Unlocking the potential of post-consumer garments as a source of nanocellulose Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-29 Maria-Ximena Ruiz-Caldas, Varvara Apostolopoulou-Kalkavoura, Aji P. Mathew
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Host-guest self-assembly grafts into silica sub-surface for shear-stable interfaces Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-29 Yizhe Liu, Yang Wu, Zishuai Wu, Keling Hu, Meirong Cai, Xiaowei Pei, Wenbo Sheng, Feng Zhou
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Iron fluoride-lithium metal batteries in bis(fluorosulfonyl)imide-based ionic liquid electrolytes Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-29 Lorenz F. Olbrich, Albert W. Xiao, Maximilian Schart, Johannes Ihli, Guillaume Matthews, Mohan Sanghadasa, Mauro Pasta
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A general route to retooling hydrolytic enzymes toward plastic degradation Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-29 Susana M. Meza Huaman, Jake H. Nicholson, Alex P.S. Brogan
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A multi-band refinement technique for analyzing electronic band structure of thermoelectric materials Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-25 Bharti Agrawal, Johannes de Boor, Titas Dasgupta
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Insights into the host-guest systems of single-walled-carbon-nanotube-confined polyoxometalates Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-15 Sheng Zhu, Feng Yang
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Probing transference and field-induced polymer velocity in block copolymer electrolytes Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-10 Michael D. Galluzzo, Hans-Georg Steinrück, Christopher J. Takacs, Aashutosh Mistry, Lorena S. Grundy, Chuntian Cao, Suresh Narayanan, Eric M. Dufresne, Qingteng Zhang, Venkat Srinivasan, Michael F. Toney, Nitash P. Balsara
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Lithium-ion hopping weakens thermal stability of LiPF6 carbonate electrolytes Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-05 Kee Sung Han, Mal-Soon Lee, Namhyung Kim, Daiwon Choi, Sujong Chae, Jaegeon Ryu, GiovanniMaria Piccini, Roger Rousseau, Edwin C. Thomsen
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Synthesis of linear [7]- and [8]catenanes Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-05 Gray H. Harlan, Sheila L. Tran, Nathan D. Colley, Mark A. Nosiglia, Yipei Zhang, Jonathan C. Barnes
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Perfect detection of computer-generated text faces fundamental challenges Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-05 Martin Májovský, Martin Černý, David Netuka, Tomáš Mikolov
Recent advancements in large language models (LLMs) have sparked a debate on the detection of artificial intelligence (AI)-generated text, a concern especially prevalent among academic institutions and publishers. While current detection tools claim high accuracy rates, some studies point to their unreliability. This paper contends that efforts to detect AI writing are fundamentally flawed because
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Super-sensitive graphene nano-fabric drum at the macroscale Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-03 Shourui Ji, Yang Liu, Boyi Zhu, Xiaoshi Li, Yuhan Zhao, Tianrui Cui, Shuxuan Dong, Jinming Jian, Yilong Li, Yang Yi, Cheng Li, He Tian, Tian-Ling Ren
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Color-tunable organic light-emitting devices and their applications Cell Rep. Phys. Sci. (IF 8.9) Pub Date : 2024-01-03 Jiaming Zhang, Meina Han, Mengxin Xu, Letian Zhang, Shihao Liu, Wenfa Xie