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A Pinch-Based Approach for Targeting Carbon Capture, Utilization, and Storage Systems
Industrial & Engineering Chemistry Research ( IF 4.2 ) Pub Date : 2019-02-14 , DOI: 10.1021/acs.iecr.8b06156
Sonal K. Thengane 1 , Raymond R. Tan 2 , Dominic C. Y. Foo 3 , Santanu Bandyopadhyay 4
Affiliation  

Carbon capture and storage (CCS) reduces carbon dioxide (CO2) emissions by sequestration of captured CO2 for long-term storage whereas carbon capture and utilization (CCU) offers resource conservation benefits by displacing the need for extracted CO2 from natural sources. The integration of these two results in a carbon capture, utilization, and storage (CCUS) system, which either uses CO2 for profitable applications or stores it in the reservoirs. One of the key problems in CCS systems is to optimally match the sources (e.g., CO2 captured from fossil-fueled power plants) and the sinks (e.g., available geological reservoirs for storing the captured CO2). In practice, the geological storage sites may be available at different times and have limitations on the maximum CO2 storage capacity and the injectivity rate, subject to other geological characteristics. This work proposes an improved pinch analysis-based methodology by simultaneously considering the injectivity constraints and variable availability of all sources and sinks. Two types of CO2 storage are considered in this work, that is, sinks with fixed life and sinks with fixed capacity. A new CCUS Mapping Diagram is presented to show the capture of CO2 to the individual sinks. Four illustrative examples demonstrate the applicability of the proposed methodology to the CCUS systems in which purity is not a constraint in CO2 utilization. In some cases, the improved methodology overcomes the pitfall of the previous method by identifying rigorous CCUS targets.

中文翻译:

一种针对目标的碳捕集,利用和存储系统的基于捏的方法

碳捕获和储存(CCS)通过将捕获的CO 2隔离以进行长期存储来减少二氧化碳(CO 2)排放,而碳捕获和利用(CCU)取代了从自然资源中提取CO 2的需求,从而节省了资源。两者的整合形成了碳捕集,利用和封存(CCUS)系统,该系统将CO 2用于有利可图的应用或将其存储在储层中。CCS系统中的关键问题之一是最佳地匹配来源(例如,从化石燃料发电厂捕获的CO 2)和汇(例如,用于存储捕获的CO 2的可用地质储层))。实际上,根据其他地质特征,地质封存地点可能在不同时间可用,并且对最大CO 2封存能力和注入速率有限制。这项工作提出了一种改进的基于捏分析的方法,同时考虑了所有源和汇的注入性约束和可变可用性。在这项工作中考虑了两种类型的CO 2储存,即具有固定寿命的水槽和具有固定容量的水槽。提出了一个新的CCUS映射图,以显示将CO 2捕集到各个汇的情况。四个说明性例子说明了所提出的方法论对CCUS系统的适用性,其中纯度不是CO的限制2利用率。在某些情况下,通过确定严格的CCUS目标,改进的方法克服了先前方法的陷阱。
更新日期:2019-02-14
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