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Electronic Transport in Two-Dimensional Materials
Annual Review of Physical Chemistry ( IF 14.7 ) Pub Date : 2018-04-20 00:00:00 , DOI: 10.1146/annurev-physchem-050317-021353
Vinod K. Sangwan 1 , Mark C. Hersam 1, 2
Affiliation  

Two-dimensional (2D) materials have captured the attention of the scientific community due to the wide range of unique properties at nanometer-scale thicknesses. While significant exploratory research in 2D materials has been achieved, the understanding of 2D electronic transport and carrier dynamics remains in a nascent stage. Furthermore, because prior review articles have provided general overviews of 2D materials or specifically focused on charge transport in graphene, here we instead highlight charge transport mechanisms in post-graphene 2D materials, with particular emphasis on transition metal dichalcogenides and black phosphorus. For these systems, we delineate the intricacies of electronic transport, including band structure control with thickness and external fields, valley polarization, scattering mechanisms, electrical contacts, and doping. In addition, electronic interactions between 2D materials are considered in the form of van der Waals heterojunctions and composite films. This review concludes with a perspective on the most promising future directions in this fast-evolving field.

中文翻译:


二维材料中的电子传输

二维(2D)材料由于在纳米级厚度上具有广泛的独特特性而引起了科学界的关注。尽管已经完成了对2D材料的重大探索性研究,但对2D电子传输和载流子动力学的理解仍处于起步阶段。此外,由于先前的评论文章提供了2D材料的一般概述,或者特别关注于石墨烯中的电荷传输,因此在这里,我们重点介绍了石墨烯后2D材料中的电荷传输机制,尤其着重于过渡金属二卤化碳和黑磷。对于这些系统,我们描述了电子传输的复杂性,包括带厚度和外部场的能带结构控制,波谷极化,散射机制,电触点,和掺杂。此外,二维材料之间的电子相互作用以范德华异质结和复合膜的形式考虑。这篇综述以对这个快速发展领域中最有希望的未来方向的观点作为结束。

更新日期:2018-04-20
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