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Intensification of CO₂ capture by monoethanolamine solution containing TiO2 nanoparticles in a rotating packed bed
International Journal of Greenhouse Gas Control ( IF 3.9 ) Pub Date : 2019-12-16 , DOI: 10.1016/j.ijggc.2019.102933
Masoud Shirzadi Ahou Dashti , Mahdieh Abolhasani

This study investigates the mass transfer intensification in the absorption of carbon dioxide (CO₂) into a monoethanolamine (MEA) solution enhanced by TiO2 nanoparticles in a typical rotating packed bed (RPB). The overall volumetric gas phase mass transfer coefficients (KGa) were investigated in a counter-current RPB with blade packings. The effects of TiO2 and MEA concentrations, rotational speed, initial concentration of CO₂, gas and liquid flow rates on KGa were specified. The rotational speed had positive effects on KGa. It is deduced that TiO2 nanoparticles led to enhanced CO₂ capture efficiency of over 26.9 % and enhancement in KGa from 7.5%–96.1% for MEA based TiO2 suspension in comparison with MEA solution without nanoparticles. Therefore, TiO2 nanoparticles can augment the mass transfer coefficient and intensify the CO₂ absorption, even in a high-efficiency equipment like a high gravity RPB.



中文翻译:

在旋转填充床中通过含TiO 2纳米粒子的单乙醇胺溶液增强对CO 2的捕集

这项研究研究了在典型的旋转填充床(RPB)中二氧化碳(CO 2)吸收到由TiO 2纳米颗粒增强的单乙醇胺(MEA)溶液中的传质强化。气相总体积传质系数(ķG一种)在带有叶片填料的逆流RPB中进行了研究。TiO 2和MEA浓度,转速,CO 2初始浓度,气体和液体流速对ķG一种被指定。旋转速度对K G a产生积极影响。据推论,与不含纳米颗粒的MEA溶液相比,基于MEA的TiO 2悬浮液使TiO 2纳米颗粒提高了26.9%的CO 2捕集效率,并使K G a从7.5%–96.1%提高。因此,即使在诸如高重力RPB的高效设备中,TiO 2纳米颗粒也可以增加传质系数并增强CO 2的吸收。

更新日期:2019-12-17
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