The Thermal Electrochemical Co-drive System (TECS) has the advantages of high desorption rate and low energy consumption. However, the fluid flow and capture performance is still unknown in TECS. Thus, a comprehensive experiment and simulation work on TECS is performed to demonstrate the fluid flow and capture performance in a pilot-scale TECS. The reaction kinetics of the electrolyzed MEA-SG solution is discussed. A pilot-scale TECS is set up and gas-liquid two-phase flow model is developed for the TECS. According to the numerical computation and experiment, the gas-liquid two-phase flow field was analyzed under the thermal electrochemical co-drive conditions. The mechanism of CO₂ capture was clearly understood. The synergy of thermal desorption and electrochemical desorption was quantified numerically. The results showed that the temperature of TECS was reduced below 333 K and the energy consumption amount was determined at 1.3 G J/t to 2.1 G J/t, which is much lower than the conventional process. LNG cold energy reduced the desorption energy consumption.

热电联动系统（TECS）具有脱附率高，能耗低的优点。但是，在TECS中，流体的流动和捕获性能仍然未知。因此，在TECS上进行了全面的实验和仿真工作，以证明在中试规模的TECS中的流体流动和捕获性能。讨论了电解MEA-SG溶液的反应动力学。建立了中试规模的TECS，并为TECS建立了气液两相流模型。根据数值计算和实验，分析了热电化学共驱条件下的气液两相流场。CO ₂的作用机理捕获被清楚地理解。数值量化了热脱附和电化学脱附的协同作用。结果表明，TECS的温度降低到333 K以下，能耗确定为1.3 G J / t至2.1 G J / t，这远低于常规工艺。液化天然气冷能减少了解吸能量的消耗。