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Nodeless superconductivity and its evolution with pressure in the layered dirac semimetal 2M-WS 2
npj Quantum Materials ( IF 5.7 ) Pub Date : 2019-09-10 , DOI: 10.1038/s41535-019-0189-5
Zurab Guguchia , Dariusz J. Gawryluk , Marta Brzezinska , Stepan S. Tsirkin , Rustem Khasanov , Ekaterina Pomjakushina , Fabian O. von Rohr , Joel A. T. Verezhak , M. Zahid Hasan , Titus Neupert , Hubertus Luetkens , Alex Amato

Recently, the transition metal dichalcogenide (TMD) system 2M-WS2 has been identified as a Dirac semimetal exhibiting both superconductivity with the highest Tc ~ 8.5 K among all the TMD materials and topological surface states. Here we report on muon spin rotation (μSR) and density functional theory studies of microscopic SC properties and the electronic structure in 2M-WS2 at ambient and under hydrostatic pressures (pmax = 1.9 GPa). The SC order parameter in 2M-WS2 is determined to have single-gap s-wave symmetry. We further show a strong negative pressure effect on Tc and on the SC gap Δ. This may be partly caused by the pressure induced reduction of the size of the electron pocket around the Γ-point. We also find that the superfluid density ns is weakly affected by pressure. The absence of a strong pressure effect on ns and the absence of a correlation between ns and Tc in 2M-WS2, in contrast to the other SC TMDs Td-MoTe2 and 2H-NbSe2, is explained in terms of its location in the optimal (ambient pressure) and above the optimal (under pressure) superconducting regions of the phase diagram and its large distance to the other possible competing or cooperating orders.



中文翻译:

分层狄拉克半金属2M-WS 2中的无节点超导性及其随压力的演化

最近,过渡金属二硫属化物(TMD)系统2M-WS 2已经被鉴定为狄拉克半金属兼具超导具有最高Ť Ç  〜8.5所有的TMD的材料和表面拓扑状态之间ķ。在这里,我们报告有关在室温和静水压力(p max  = 1.9 GPa)下2M-WS 2中的微观SC特性和电子结构的μ自旋旋转(μSR)和密度泛函理论研究。确定2M-WS 2中的SC阶参数具有单间隙s波对称性。我们进一步显示出对T c的强烈负压效应并且在SC间隙Δ上。这可能部分是由于压力引起的电子点在Γ点附近尺寸的减小而引起的。我们还发现,超流密度ñ小号弱受压力。没有强大的压力作用Ñ小号和不存在之间的相关性的Ñ小号Ť Ç在2M-WS 2,相比于其他SC TMD的Ť d -MoTe 2和2H-NbSe 2根据其在相图的最佳(环境压力)中和在最佳(负压)超导区域之上的位置以及与其他可能的竞争或合作顺序的较大距离来进行解释。

更新日期:2019-09-10
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