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Multifunctional Magnetic Oxide-MoS2 Heterostructures on Silicon
Advanced Materials ( IF 29.4 ) Pub Date : 2023-05-25 , DOI: 10.1002/adma.202302620
Allen Jian Yang 1 , Liang Wu 2 , Yanran Liu 1 , Xinyu Zhang 2 , Kun Han 3 , Ying Huang 4 , Shengyao Li 1 , Xian Jun Loh 5 , Qiang Zhu 5, 6 , Rui Su 1, 7, 8 , Ce-Wen Nan 9 , Xiao Renshaw Wang 1, 7
Affiliation  

Correlated oxides and related heterostructures are intriguing for developing future multifunctional devices by exploiting their exotic properties, but their integration with other materials, especially on Si-based platforms, is challenging. Here, van der Waals heterostructures of La0.7Sr0.3MnO3 (LSMO) , a correlated manganite perovskite, and MoS2 are demonstrated on Si substrates with multiple functions. To overcome the problems due to the incompatible growth process, technologies involving freestanding LSMO membranes and van der Waals force-mediated transfer are used to fabricate the LSMO-MoS2 heterostructures. The LSMO-MoS2 heterostructures exhibit a gate-tunable rectifying behavior, based on which metal-semiconductor field-effect transistors (MESFETs) with on-off ratios of over 104 can be achieved. The LSMO-MoS2 heterostructures can function as photodiodes displaying considerable open-circuit voltages and photocurrents. In addition, the colossal magnetoresistance of LSMO endows the LSMO-MoS2 heterostructures with an electrically tunable magnetoresponse at room temperature. This work not only proves the applicability of the LSMO-MoS2 heterostructure devices on Si-based platform but also demonstrates a paradigm to create multifunctional heterostructures from materials with disparate properties.

中文翻译:

硅基多功能磁性氧化物-MoS2 异质结构

相关氧化物和相关异质结构对于通过利用其奇异特性来开发未来的多功能器件很有趣,但它们与其他材料的集成,特别是在硅基平台上,具有挑战性。在这里,La 0.7 Sr 0.3 MnO 3 (LSMO)(一种相关的锰钙钛矿)和MoS 2的范德华异质结构在具有多种功能的Si基板上得到了证明。为了克服生长过程不相容的问题,采用独立式 LSMO 膜和范德华力介导转移技术来制造 LSMO-MoS 2异质结构。LSMO-MoS 2异质结构表现出栅极可调整流行为,基于此可以实现开关比超过10 4的金属半导体场效应晶体管(MESFET)。LSMO-MoS 2异质结构可以用作光电二极管,显示出相当大的开路电压和光电流。此外,LSMO的巨大磁阻赋予LSMO-MoS 2异质结构在室温下电可调的磁响应。这项工作不仅证明了LSMO-MoS 2异质结构器件在硅基平台上的适用性,而且展示了从具有不同特性的材料创建多功能异质结构的范例。
更新日期:2023-05-25
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