Ti-MOF single-crystals featuring an intracrystal macro–microporous hierarchy for catalytic oxidative desulfurization,Chemical Communications

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Ti-MOF single-crystals featuring an intracrystal macro–microporous hierarchy for catalytic oxidative desulfurization
Chemical Communications ( IF 4.9 ) Pub Date : 2023-01-18 , DOI: 10.1039/d2cc06473a
Shen Yu _{1,

2} , Yu Xiao ₁ , Zhan Liu _{1,

2,

3} , Jia-Min Lyu ₁ , Yi-Long Wang ₄ , Zhi-Yi Hu _{1,

3} , Yu Li ₁ , Ming-Hui Sun ₅ , Li-Hua Chen ₁ , Bao-Lian Su _{1,

5}

Affiliation

For the first time, we demonstrate a Ti-MOF (Ti-metal organic framework) single-crystal featuring an intracrystal macro–microporous hierarchy (Hier-NTU-9) by a vapor-assisted polymer-templated method. This Hier-NTU-9 possesses macropores (100–1000 nm) derived from polymer templates and enhanced transport ability of bulky molecules, exhibiting almost double the desulfurization activity compared to the conventional NTU-9.

中文翻译：

用于催化氧化脱硫的具有晶内大-微孔结构的 Ti-MOF 单晶

我们首次通过蒸汽辅助聚合物模板法展示了具有晶内大微孔结构 (Hier-NTU-9) 的 Ti-MOF（钛金属有机骨架）单晶。这种 Hier-NTU-9 具有源自聚合物模板的大孔 (100–1000 nm) 和增强的大分子传输能力，与传统的 NTU-9 相比，脱硫活性几乎翻了一番。

更新日期：2023-01-18

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