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Emergent charge order in pressurized kagome superconductor CsV3Sb5
Nature ( IF 64.8 ) Pub Date : 2022-11-23 , DOI: 10.1038/s41586-022-05351-3
Lixuan Zheng 1 , Zhimian Wu 1 , Ye Yang 1 , Linpeng Nie 1 , Min Shan 1 , Kuanglv Sun 1 , Dianwu Song 1 , Fanghang Yu 1 , Jian Li 1 , Dan Zhao 1 , Shunjiao Li 1 , Baolei Kang 1 , Yanbing Zhou 1 , Kai Liu 1 , Ziji Xiang 1, 2 , Jianjun Ying 2 , Zhenyu Wang 2, 3 , Tao Wu 1, 2, 3, 4, 5 , Xianhui Chen 1, 2, 3, 4, 5
Affiliation  

The discovery of several electronic orders in kagome superconductors AV3Sb5 (A means K, Rb, Cs) provides a promising platform for exploring unprecedented emergent physics1,2,3,4,5,6,7,8,9. Under moderate pressure (<2.2 GPa), the triple-Q charge density wave (CDW) order is monotonically suppressed by pressure, while the superconductivity shows a two-dome-like behaviour, suggesting an unusual interplay between superconductivity and CDW order10,11. Given that time-reversal symmetry breaking and electronic nematicity have been revealed inside the triple-Q CDW phase8,9,12,13, understanding this CDW order and its interplay with superconductivity becomes one of the core questions in AV3Sb5 (refs. 3,5,6). Here, we report the evolution of CDW and superconductivity with pressure in CsV3Sb5 by 51V nuclear magnetic resonance measurements. An emergent CDW phase, ascribed to a possible stripe-like CDW order with a unidirectional 4a0 modulation, is observed between Pc1 0.58 GPa and Pc2 2.0 GPa, which explains the two-dome-like superconducting behaviour under pressure. Furthermore, the nuclear spin-lattice relaxation measurement reveals evidence for pressure-independent charge fluctuations above the CDW transition temperature and unconventional superconducting pairing above Pc2. Our results not only shed new light on the interplay of superconductivity and CDW, but also reveal new electronic correlation effects in kagome superconductors AV3Sb5.



中文翻译:

加压 kagome 超导体 CsV3Sb5 中的紧急电荷顺序

在 kagome 超导体 AV 3 Sb 5(A 表示 K、Rb、Cs)中发现了几个电子阶,为探索前所未有的新兴物理学1,2,3,4,5,6,7,8,9提供了一个有前途的平台。在中等压力 (<2.2 GPa) 下,三Q电荷密度波 (CDW) 阶被压力单调抑制,而超导性显示出类似双圆顶的行为,表明超导性和 CDW 阶之间存在不寻常的相互作用10,11 . 鉴于时间反转对称性破缺和电子向列性已在三Q CDW 相8,9,12,13中被揭示,了解这种 CDW 阶及其与超导性的相互作用成为 AV 3 Sb 5中的核心问题之一(参考文献3,5,6)。在这里,我们通过51 V 核磁共振测量报告了 CsV 3 Sb 5中 CDW 和超导性随压力的演变。在P c1  0.58 GPa 和P c2 之间观察到出现的 CDW 相,归因于具有单向 4a 0调制的可能的条纹状 CDW 阶 2.0 GPa,这解释了压力下的双圆顶状超导行为。此外,核自旋晶格弛豫测量揭示了 CDW 转变温度以上的与压力无关的电荷波动和P c2以上的非常规超导配对的证据。我们的结果不仅揭示了超导性和 CDW 的相互作用,而且揭示了 kagome 超导体 AV 3 Sb 5中新的电子相关效应。

更新日期:2022-11-23
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