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Giant voltage amplification from electrostatically induced incipient ferroelectric states
Nature Materials ( IF 41.2 ) Pub Date : 2022-08-25 , DOI: 10.1038/s41563-022-01332-z
Mónica Graf 1 , Hugo Aramberri 1 , Pavlo Zubko 2 , Jorge Íñiguez 1, 3
Affiliation  

Ferroelectrics subject to suitable electric boundary conditions present a steady negative capacitance response1,2. When the ferroelectric is in a heterostructure, this behaviour yields a voltage amplification in the other elements, which experience a potential difference larger than the one applied, holding promise for low-power electronics3. So far research has focused on verifying this effect and little is known about how to optimize it. Here, we describe an electrostatic theory of ferroelectric/dielectric superlattices, convenient model systems4,5, and show the relationship between the negative permittivity of the ferroelectric layers and the voltage amplification in the dielectric ones. Then, we run simulations of PbTiO3/SrTiO3 superlattices to reveal the factors most strongly affecting the amplification. In particular, we find that giant effects (up to tenfold increases) can be obtained when PbTiO3 is brought close to the so-called ‘incipient ferroelectric’ state.



中文翻译:

来自静电感应的初始铁电态的巨电压放大

铁电体受到合适的电边界条件呈现稳定的负电容响应1,2。当铁电体处于异质结构时,这种行为会在其他元素中产生电压放大,这些元素的电势差大于所施加的电势差,有望用于低功率电子设备3。到目前为止,研究主要集中在验证这种效果,而对如何优化它知之甚少。在这里,我们描述了铁电/电介质超晶格的静电理论,方便的模型系统4,5,并展示了铁电层的负介电常数与电介质层中的电压放大之间的关系。然后,我们运行 PbTiO 3 /SrTiO的模拟3 个超晶格揭示了对放大影响最强烈的因素。特别是,我们发现当 PbTiO 3接近所谓的“初始铁电”状态时可以获得巨大的效果(增加十倍) 。

更新日期:2022-08-25
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