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Intrinsic magnetism in superconducting infinite-layer nickelates
Nature Physics ( IF 19.6 ) Pub Date : 2022-08-01 , DOI: 10.1038/s41567-022-01684-y
Jennifer Fowlie , Marios Hadjimichael , Maria M. Martins , Danfeng Li , Motoki Osada , Bai Yang Wang , Kyuho Lee , Yonghun Lee , Zaher Salman , Thomas Prokscha , Jean-Marc Triscone , Harold Y. Hwang , Andreas Suter

The discovery of superconductivity in Nd0.8Sr0.2NiO2 (ref. 1) introduced a new family of layered nickelate superconductors that has now been extended to include a range of strontium doping2,3, praseodymium or lanthanum in place of neodymium4,5,6,7, and the five-layer compound Nd6Ni5O12 (ref. 8). A number of studies have indicated that electron correlations are strong in these materials9,10,11,12,13,14,15, a feature that often leads to the emergence of magnetism. Here we report muon spin rotation/relaxation studies of a series of superconducting infinite-layer nickelates. Regardless of the rare earth ion or doping, we observe an intrinsic magnetic ground state arising from local moments on the nickel sublattice. The coexistence of magnetism—which is likely to be antiferromagnetic and short-range ordered—with superconductivity is reminiscent of some iron pnictides16 and heavy fermion compounds17, and qualitatively distinct from the doped cuprates18.



中文翻译:

超导无限层镍酸盐的本征磁性

Nd 0.8 Sr 0.2 NiO 2超导性的发现(参考文献1)引入了一个新的层状镍酸盐超导体系列,现已扩展到包括一系列锶掺杂2,3、镨或镧代替钕4,5 ,6,7和五层化合物 Nd 6 Ni 5 O 12(参考文献8)。许多研究表明,这些材料中的电子相关性很强9,10,11,12,13,14,15,这个特征往往会导致磁性的出现。在这里,我们报告了一系列超导无限层镍酸盐的 μ 子自旋旋转/弛豫研究。无论稀土离子或掺杂如何,我们都观察到由镍亚晶格上的局部矩引起的固有磁基态。磁性(可能是反铁磁性和短程有序)与超导性的共存让人想起一些铁磷化物16和重费米子化合物17,并且在质量上与掺杂的铜酸盐18不同。

更新日期:2022-08-02
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