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A low-polarity small organic molecule with a stable keto form for photocatalytic H2 evolution
Chemical Communications ( IF 4.9 ) Pub Date : 2022-07-25 , DOI: 10.1039/d2cc03951f Qing Yang 1 , Cefei Zhang 1 , Fangli Yi 1 , Xinyu Li 1 , Yiqi Yuan 1 , Kewei Liu 1 , Hongmei Cao 1 , Hongjian Yan 1 , Zhishan Su 1
Chemical Communications ( IF 4.9 ) Pub Date : 2022-07-25 , DOI: 10.1039/d2cc03951f Qing Yang 1 , Cefei Zhang 1 , Fangli Yi 1 , Xinyu Li 1 , Yiqi Yuan 1 , Kewei Liu 1 , Hongmei Cao 1 , Hongjian Yan 1 , Zhishan Su 1
Affiliation
Five small organic molecules (SOMs) with different degrees of enol to keto tautomerism were synthesized for photocatalytic H2 evolution. The SOM possessing the highest activity features a stable keto form that greatly facilitates the flowing of the excited electrons toward the carbonyl O site where the reduction reaction occurs.
中文翻译:
一种具有稳定酮形式的低极性有机小分子,用于光催化析氢
合成了五种具有不同程度烯醇至酮互变异构的有机小分子 (SOM),用于光催化 H 2演化。具有最高活性的 SOM 具有稳定的酮形式,极大地促进了受激电子流向发生还原反应的羰基 O 位点。
更新日期:2022-07-29
中文翻译:
一种具有稳定酮形式的低极性有机小分子,用于光催化析氢
合成了五种具有不同程度烯醇至酮互变异构的有机小分子 (SOM),用于光催化 H 2演化。具有最高活性的 SOM 具有稳定的酮形式,极大地促进了受激电子流向发生还原反应的羰基 O 位点。